An intrinsically stable type-I optical parametric oscillator was built with a periodically poled KTiOPO4 (PPKTP) crystal to generate a stable bright, continuous-wave, broadband phase-squeezed beam. A 3.2 dB sensitivity enhancement of optical interferometry was demonstrated on weak electrooptic modulation signals within a 20 MHz squeezing bandwidth. This also realized a channel capacity increase beyond that of coherent optical communication.
We report measurements of time-frequency entangled photon pairs and heralded single photons at telecommunications wavelengths, generated using a periodically-poled, lithium niobate on insulator (LNOI) waveguide pumped optically by a diode laser. We achieve a high Coincidences-to-Accidentals Ratio (CAR) at high pair brightness, a low value of the conditional self-correlation function [$g^{(2)}$(0)], and high two-photon energy-time Franson interferometric visibility, which demonstrate the high quality of the entangled photon pairs and heralded single photons.
Significant successes have recently been reported in the study of the generation of spectrally pure state in group-velocity-matched (GVM) nonlinear crystals. However, the GVM condition can only be realized in limited kinds of crystals and at limited wavelengths. Here, we investigate pure state generation in the isomorphs of PPKTP crystal: i.e., periodically poled RTP, KTA, RTA and CTA crystals. By numerical simulation, we find that these crystals from the KTP family can generate pure photons with high spectral purity (over 0.8), wide tunability (more than 400 nm), reasonable nonlinearity at a …
We theoretically investigated spectrally uncorrelated biphotons generated in a counter-propagating spontaneous parametric downconversion (CP-SPDC) from periodically poled MTiOXO4 (M = K, Rb, Cs; X = P, As) crystals. By numerical calculation, it was found that the five crystals from the KTP family can be used to generate heralded single photons with high spectral purity and wide tunability. Under the type-0 phase-matching condition, the purity at 1550 nm was between 0.91 and 0.92, and the purity can be maintained over 0.90 from 1500 nm to 2000 nm wavelength. Under the type-II phase-matching con…
Low-noise quantum frequency conversion in periodically-poled nonlinear crystals has proved challenging when the pump wavelength is shorter than the target wavelength. This is - at least in large part - a consequence of the parasitic spontaneous parametric down-conversion of pump photons, whose efficiency is increased by fabrication errors in the periodic poling. Here we characterise the poling quality of commercial periodically-poled bulk potassium titanyl phosphate (ppKTP) by measuring the sum-frequency generation (SFG) efficiency over a large phase mismatch range from 0 to more than 400$π$. …
We present a detailed numerical investigation of five nonlinear materials and their properties regarding photon-pair creation using parametric downconversion. Periodic poling of ferroelectric nonlinear materials is a convenient way to generate collinearly propagating photon pairs. Most applications and experiments use the well-known potassium titanyl phosphate (KTiOPO4, ppKTP) and lithium niobate (LiNbO3, ppLN) crystals for this purpose. In this article we provide a profound discussion on the family of KTP-isomorphic nonlinear materials, including KTP itself but also the much less common CTA (…
Lithium niobate (LN), dubbed by many as the silicon of photonics, has recently risen to the forefront of chip-scale nonlinear optics research since its demonstration as an ultralow-loss integrated photonics platform. Due to its significant quadratic nonlinearity ($χ^{(2)}$), LN inspires many important applications such as second-harmonic generation (SHG), spontaneous parametric down-conversion, and optical parametric oscillation. Here, we demonstrate high-efficiency SHG in dual-resonant, periodically poled z-cut LN microrings, where quasi-phase matching is realized by field-assisted domain eng…
Broadband bright biphotons from periodically poled triple-resonance metasurface
Songshan Lake Materials Laboratory（松山湖材料实验室）；ARC Centre of Excellence for Transformative Meta-Optical Systems (TMOS), Department of Electronic Materials Engineering, Research School of Physics, Australian National University（澳大利亚国立大学变革性超光学系统卓越中心（TMOS）电子材料工程系物理研究学院）；School of Physics, Nanjing University（南京大学物理学院）；Institute of Applied Physics, Abbe Center of Photonics, Friedrich Schiller University Jena（耶拿弗里德里希·席勒大学应用物理研究所阿贝光子学中心）；Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所）
The absence of the single-photon nonlinearity has been a major roadblock in developing quantum photonic circuits at optical frequencies. In this paper, we demonstrate a periodically-poled thin film lithium niobate microring resonator (PPLNMR) that reaches 5,000,000%/W second harmonic conversion efficiency---almost 20-fold enhancement over the state-of-the-art---by accessing its largest $χ^{(2)}$ tensor component $d_{33}$ via quasi-phase matching. The corresponding single photon coupling rate $g/2π$ is estimated to be 1.2 MHz, which is an important milestone as it approaches the dissipation rat…
Nonlinear optical processes of spatially structured light, including optical vortex and vector optical fields, have stimulated a lot of interesting physical effects and found a variety of important applications ranging from optical imaging to quantum information processing. However, high harmonic generation of vector optical fields with space-varying polarization states is still a challenge. Here we demonstrate third harmonic generation of spatially structured light including vector optical fields, in a nonlinear Sagnac interferometer containing a carefully designed quasi-periodically poled po…
The amplified spontaneous emission from a superluminescent diode was frequency doubled in a periodically poled lithium niobate waveguide crystal. The temporally incoherent radiation of such a superluminescent diode is characterized by a relatively broad spectral bandwidth and thermal-like photon statistics, as the measured degree of second order coherence, g$^{(2)}$(0)=1.9$\pm$0.1, indicates. Despite the non-optimized scenario in the spectral domain, we achieve six orders of magnitude higher conversion efficiency than previously reported with truly incoherent light. This is possible by using s…
Optical orbital angular momentum (OAM), as an important degree of freedom of light, has been attracted extensive attention, due to its intrinsic feature of natural discrete infinite dimension. Manipulation of OAM spectra is crucial for many impressive applications from classical to quantum realms, in particular, nonlinear manipulation of OAM spectra. Here we realized the nonlinear manipulation of OAM spectra by using the simultaneous second- and third-harmonic generation in a single nonlinear crystal of quasi-periodically poled potassium titanyl phosphate, for fundamental waves with a variety …
Prospective integrated quantum optical technologies will combine nonlinear optics and components requiring cryogenic operating temperatures. Despite the prevalence of integrated platforms exploiting $χ^{(2)}$-nonlinearities for quantum optics, for example used for quantum state generation and frequency conversion, their material properties at low temperatures are largely unstudied. Here, we demonstrate the first second harmonic generation in a fiber-coupled lithium niobate waveguide at temperatures down to 4.4K. We observe a reproducible shift in the phase-matched pump wavelength within the te…
A continuous-wave (CW) broadband high-level optical quadrature squeezer is essential for high-speed large-scale fault-tolerant quantum computing on a time-domain-multiplexed continuous-variable optical cluster state. CW THz-bandwidth squeezed light can be obtained with a waveguide optical parametric amplifier (OPA); however, the squeezing level have been insufficient for applications of fault-tolerant quantum computation because of degradation of the squeezing level due to their optical losses caused by the structural perturbation and pump-induced phenomena. Here, by using mechanical polishing…
Integrated photon-pair sources on periodically poled thin-film lithium tantalate
National University of Singapore（新加坡国立大学）；Centre for Quantum Technologies, National University of Singapore（新加坡国立大学量子技术中心）；A ∗ STAR Quantum Innovation Centre (Q.InC), Agency for Science, Technology and Research (A ∗ STAR)（新加坡科技研究局（A*STAR）量子创新中心）
Quantum squeezing in an all-resonant periodically poled lithium niobate microresonator
University of California, Berkeley（加州大学伯克利分校）；Ming Hsieh Department of Electrical and Computer Engineering, University of Southern California（南加州大学明海电气与计算机工程学院）；Materials Sciences Division, Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室材料科学部）
We demonstrate vacuum squeezing at the D1 line of atomic rubidium (795 nm) with a tunable, doubly-resonant, monolithic sub-threshold optical parametric oscillator in periodically-poled Rb-doped potassium titanyl phosphate. The squeezing appears to be undiminished by a strong dispersive optical nonlinearity recently observed in this material.
Gaussian mode coupling of spectrally broadband photons from bulk spontaneous parametric down-conversion: A spatial-spectral mode analysis of fiber coupling
Fraunhofer Institute for Applied Optics and Precision Engineering（弗劳恩霍夫应用光学和精密工程研究所）；Friedrich Schiller University Jena, Institute of Applied Physics, Abbe Center of Photonics（耶拿弗里德里希·席勒大学应用物理学院阿贝光子学中心）
We experimentally demonstrate a source of polarization entangled photon-pairs based on a single periodically-poled potassium titanyl phosphate (PPKTP) crystal pumped with a broadband, free running laser diode.The crystal is placed within a linear beam-displacement interferometer, and emits photon-pairs based ontype-0 spontaneous parametric downconversion (SPDC). We observe pair rates of 0.56 Mpairs/s/mW in a single spatial mode with a polarization visibility of 97.7% over a spectral range of 100 nm. This experiment demonstrates a pathway towards observing Gigacount rates of polarization entang…
We demonstrate a polarization-entangled photon-pair source obtained via a type-II non-collinear quasi-phase-matched spontaneous parametric down-conversion process with a 10-mm periodically poled KTiOPO$_4$ crystal, which is as stable and wavelength-tunable as the well-known Sagnac configuration scheme. A brightness of 4.2 kHz/mW is detected and a concurrence of 0.975 is estimated using quantum state tomography. Without loss of entanglement and brightness, the photon-pair wavelengths are tunable through control of the crystal temperature. This improvement is achieved using the non-collinear con…
We present a new approach to engineering broadband sources of entangled photon pairs for quantum interferometry. The source is based on quasi-phase-matched spontaneous parametric down conversion in a titanium diffused periodically poled lithium niobate waveguide with a strongly-chirped poling period. The proposed non-standard asymmetric poling mitigates phase distortions associated with the process of chirping. Asymmetric poling significantly broadens the entangled source bandwidth while preserving high visibility quantum interferometric sensing.
