arXivDaily arXiv每日学术速递 周一至周五更新
北美退伍军人节(Veterans Day),12 日无更新
arXiv 0706.0602cond-mat.str-el
收藏

Ga取代Mn对金属锰氧化物光学性质的影响

Effect of Mn substitution by Ga on the optical properties of a metallic manganite

A. Nucara, P. Maselli, M. Del Bufalo, M. Cestelli Guidi, J. Garcia, P. Orgiani, L. Maritato, P. Calvani

摘要:

在金属锰氧化物如La(2/3)Sr(1/3)MnO(3)中,Mn(+3)被Ga(+3)取代稀释了铁磁有序,并局部消除了Jahn-Teller畸变,而不会严重影响晶体结构。因此,人们可以跟踪由Ga引起的电荷动力学的变化,直到铁金属锰氧化物变成绝缘体。本文通过五个La(2/3)Sr(1/3)Mn(1-x)Ga(x)O(3)样品的红外反射率,详细研究了这一现象,x从0增加到0.30,温度为50 < T < 320 K。将测量的光学参数与磁化强度M(x,T)联系起来的简单模型很好地描述了等离子体频率、散射率和沿金属-绝缘体转变的中红外吸收的行为。

英文摘要:

In a metallic manganite like La(2/3)Sr(1/3)MnO(3), the substitution of Mn(+3) by Ga(+3) dilutes the ferromagnetic order and locally cancels the Jahn-Teller distortion, without heavily affecting the crystal structure. One can thus follow the changes in the charge dynamics induced by Ga, until the ferro-metallic manganite is turned into an insulator. Here this phenomenon is studied in detail through the infrared reflectivity of five samples of La(2/3)Sr(1/3)Mn(1-x)Ga(x)O(3), with x increasing from 0 to 0.30 and for 50 < T < 320 K. A simple model which links the measured optical parameters to the magnetization M(x, T) well describes the behavior of the plasma frequency, the scattering rate, and the mid-infrared absorption along the metal-to-insulator transition.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑