We derive general conditions for 100 percent frequency conversion in any doubly resonant nonlinear cavity, for both second- and third-harmonic generation via chi2 and chi3 nonlinearities. We find that conversion efficiency is optimized for a certain critical power depending on the cavity parameters, and assuming reasonable parameters we predict 100 percent conversion using milliwatts of power or less. These results follow from a semi-analytical coupled-mode theory framework which is generalized from previous work to include both chi2 and chi3 media as well as inhomogeneous (fully vectorial) cavities, analyzed in the high-efficiency limit where down-conversion processes lead to a maximum efficiency at the critical power, and which is verified by direct finite-difference time-domain (FDTD) simulations of the nonlinear Maxwell equations. Explicit formulas for the nonlinear coupling coefficients are derived in terms of the linear cavity eigenmodes, which can be used to design and evaluate cavities in arbitrary geometries.
How to utilize topological microcavities to control quantum emission is one of the ongoing research topics in the optical community. In this work, we investigate the emission of quantum emitters in doubly-resonant topological Tamm microcavity, which can simultaneously achieve dual resonances at two arbitrary wavelengths according to the needs of practical application. To achieve the enhancement of quantum emission in such cavities, we have exploited the tunable doubly-resonant modes, in which one of resonant modes corresponds to the pump laser wavelength and the other one is located at the emi…
We describea theoretical analysis of the nonlinear dynamics of third-harmonic generation ($ω\to3ω$) via Kerr ($\chithree$) nonlinearities in a resonant cavity with resonances at both $ω$ and $3ω$. Such a doubly resonant cavity greatly reduces the required power for efficient harmonic generation, by a factor of $\sim V/Q^2$ where $V$ is the modal volume and $Q$ is the lifetime, and can even exhibit 100% harmonic conversion efficiency at a critical input power. However, we show that it also exhibits a rich variety of nonlinear dynamics, such as multistable solutions and long-period limit cycles.…
We present a versatile numerical algorithm for computing resonances of open dielectric cavities. The emphasis is on the generality of the system's configuration, i.e. the geometry of the (main) cavity (and possible inclusions) and the internal and external dielectric media (homogeneous and inhomogeneous). The method is based on a scattering formalism to obtain the position and width of the (quasi)-eigenmodes. The core of the method lies in the scattering S-matrix and its associated delay Q-matrix which contain all the relevant information of the corresponding scattering experiment. For instanc…
Second-order nonlinear effects, such as second-harmonic generation, can be strongly enhanced in nanofabricated photonic materials when both fundamental and harmonic frequencies are spatially and temporally confined. Practically designing low-volume and doubly resonant nanoresonators in conventional semiconductor compounds is challenging owing to their intrinsic refractive index dispersion. In this work we review a recently developed strategy to design doubly resonant nanocavities with low mode volume and large quality factor by localized defects in a photonic crystal structure. We build on thi…
Second harmonic generation in nonlinear materials can be greatly enhanced by realizing doubly-resonant cavities with high quality factors. However, fulfilling such doubly resonant condition in photonic crystal (PhC) cavities is a long-standing challenge, because of the difficulty in engineering photonic bandgaps around both frequencies. Here, by implementing a second-harmonic bound state in the continuum (BIC) and confining it with a heterostructure design, we show the first doubly-resonant PhC slab cavity with $2.4\times10^{-2}$ W$^{-1}$ conversion efficiency under continuous wave excitation.…
We present a multimode laser-linewidth theory for arbitrary cavity structures and geometries that contains nearly all previously known effects and also finds new nonlinear and multimode corrections, e.g. a bad-cavity correction to the Henry $α$ factor and a multimode Schawlow--Townes relation (each linewidth is proportional to a sum of inverse powers of all lasing modes). Our theory produces a quantitatively accurate formula for the linewidth, with no free parameters, including the full spatial degrees of freedom of the system. Starting with the Maxwell--Bloch equations, we handle quantum and …
Waveplates having spatially varying fast-axis orientation and retardance provide an elegant and easy way to locally manipulate different attributes of light beams namely, polarization, amplitude and phase, leading to the generation of exotic structured light beams. The fabrication of such doubly inhomogeneous waveplates (d-plates) is more complex, compared to that of singly inhomogeneous waveplates (s-plates) having uniform retardance, which can be easily fabricated by different means such as photoalignment of liquid crystals, metasurfaces etc. Here, exploiting the SU(2) formalism, we establis…
We study the formation of localized patterns arising in doubly resonant dispersive optical parametric oscillators. They form through the locking of fronts connecting a continuous-wave and a Turing pattern state. This type of localized pattern can be seen as a slug of the pattern embedded in a homogeneous surrounding. They are organized in terms of a homoclinic snaking bifurcation structure, which is preserved under the modification of the control parameter of the system. We show that, in the presence of phase mismatch, localized patterns can undergo oscillatory instabilities which make them br…
It is shown that non-centrosymmetric materials with bulk second-order nonlinear susceptibility can be used to generate strongly antibunched radiation at an arbitrary wavelength, solely determined by the resonant behavior of suitably engineered coupled microcavities. The proposed scheme exploits the unconventional photon blockade of a coherent driving field at the input of a coupled cavity system, where one of the two cavities is engineered to resonate at both fundamental and second harmonic frequencies, respectively. Remarkably, the unconventional blockade mechanism occurs with reasonably low …
Photonic nanostructures simultaneously maximizing spectral and spatial overlap between fundamental and second-harmonic confined modes are highly desirable for enhancing second-order nonlinear effects in nonlinear media. These conditions have thus far remained challenging to satisfy in photonic crystal cavities because of the difficulty in designing a band gap at the second-harmonic frequency. Here, we solve this issue by using instead a bound state in the continuum at that frequency, and we design a doubly-resonant photonic crystal slab cavity with strongly improved figures of merit for nonlin…
We propose a scheme for efficient cavity-enhanced nonlinear THz generation via difference-frequency generation (DFG) processes using a triply resonant system based on photonic crystal cavities. We show that high nonlinear overlap can be achieved by coupling a THz cavity to a doubly-resonant, dual-polarization near-infrared (e.g. telecom band) photonic-crystal nanobeam cavity, allowing the mixing of three mutually orthogonal fundamental cavity modes through a chi(2) nonlinearity. We demonstrate through coupled-mode theory that complete depletion of the pump frequency - i.e., quantum-limited con…
Interactions between solid-state quantum emitters and cavities are important for a broad range of applications in quantum communication, linear optical quantum computing, nonlinear photonics, and photonic quantum simulation. These applications often require combining many devices on a single chip with identical emission wavelengths in order to generate two-photon interference, the primary mechanism for achieving effective photon-photon interactions. Such integration remains extremely challenging due to inhomogeneous broadening and fabrication errors that randomize the resonant frequencies of b…
The paper explores a theoretical possibility of resonant amplification of electromagnetic modes generated by a nonlinear effect in Euler-Heisenberg electrodynamics. Precisely, we examine the possibility of the amplification for the third harmonics induced by a single electromagnetic mode in radiofrequency cavity, as well as the generation of signal mode of combined frequencies induced by two pump modes ($ω_1$ and $ω_2$) in the cavity. Solving inhomogeneous wave equations for the signal mode, we formulate two resonant conditions for a cavity of arbitrary shape, and apply the obtained formalism …
