Coulomb drag experiments in which the inter-layer resistivity is measured are important as they provide information on the Coulomb interactions in bilayer systems. When the layer densities are low correlation effects become significant to account for the quantitative description of experimental results. We investigate systematically various models of effective inter-layer interactions in a bilayer system and compare our results with recent experiments. In the low density regime, the correlation effects are included via the intra- and inter-layer local-field corrections. We employ several theoretical approaches to construct static local-field corrections. Our comparative study demonstrates the importance of including the correlation effects accurately in the calculation of drag resistivity. Recent experiments performed at low layer densities are adequately described by effective inter-layer interactions incorporating static correlations.
We investigate interaction effects in transport phenomena in bilayer graphene (BLG). For the minimal conductivity in pristine BLG, we find that the conductivity assumes a constant value in the limit $T\to 0$, with the first correction being $\propto \sqrt{T}$. This has to be contrasted from the standard $1/T^2$ in Fermi liquids (neglecting additional logarithms and above all disorder). We furthermore study the Coulomb drag resistivity between two BLGs in the whole range from deep within the Fermi liquid regime all the way to the charge neutrality (CN) point. We find that in the Fermi liquid re…
Nonreciprocal perfect Coulomb drag in electron-hole bilayers: coherent exciton superflow as a diode
Tsung-Dao Lee Institute & School of Physics and Astronomy, Shanghai Jiao Tong University（上海交大李政道研究所与物理与天文学院）；Shanghai Branch, Hefei National Laboratory（合肥国家实验室上海分部）
We study the frictional drag between carriers in two bilayer graphene flakes separated by a 2 $-$ 5 nm thick hexagonal boron nitride dielectric. At temperatures ($T$) lower than $\sim$ 10 K, we observe a large anomalous negative drag emerging predominantly near the drag layer charge neutrality. The anomalous drag resistivity increases dramatically with reducing {\it T}, and becomes comparable to the layer resistivity at the lowest {\it T} = 1.5 K. At low $T$ the drag resistivity exhibits a breakdown of layer reciprocity. A comparison of the drag resistivity and the drag layer Peltier coefficie…
Coupled 2D sheets of electrons and holes are predicted to support novel quantum phases. Two experiments of Coulomb drag in electron-hole (e-h) double bilayer graphene (DBLG) have reported an unexplained and puzzling sign reversal of the drag signal. However, we show that this effect is due to the multiband character of DBLG. Our multiband Fermi liquid theory produces excellent agreement and captures the key features of the experimental drag resistance for all temperatures. This demonstrates the importance of multiband effects in DBLG: they have a strong effect not only on superfluidity, but al…
Coulomb drag experiments can give us information about the interaction state of double-layer systems. Here, we demonstrate anomalous Coulomb drag behaviours in a two-dimensional electron-electron bilayer system constructed by stacking atomically thin MoS2 on opposite sides of thin dielectric layers of boron nitride. In the low temperature regime, the measured drag resistance does not follow the behaviour predicted by the Coulomb drag models of exchanging momenta and energies with the particles in Fermi-liquid bilayer systems. Instead, it shows an upturn to higher and higher values. We investig…
The mechanisms of optical activity and quantum transport of twisted bilayer graphene are studied. The formation of unique electron states in the bilayer systems is studied using an effective continuum model. Such states are shown to support the correlation of transverse motions of electrons in two graphene layers. Because of the chiral structure of the atomic lattices, the contribution of such drag correlations is incompletely cancelled, thus resulting in a drag term of the optical conductivity tensor. We show that the drag term of the conductivity is the manifestation of the spatial dispersio…
Coulomb drag between parallel quantum wells provides a uniquely sensitive measurement of electron correlations since the drag response depends on interactions only. Recently it has been demonstrated that a new regime of strong interactions can be accessed for devices consisting of two monlolayer graphene (MLG) crystals, separated by few layer hexagonal boron-nitride. Here we report measurement of Coulomb drag in a double bilayer graphene (BLG) stucture, where the interaction potential is anticipated to be yet further enhanced compared to MLG. At low temperatures and intermediate densities a ne…
Umklapp-Enhanced Interlayer Valley Drag in Moiré Bilayers
Institute of Mathematical Sciences（数学科学研究所）；Tata Institute of Fundamental Research（塔塔基础研究所）；Indiana University（印第安纳大学）；Indian Institute of Technology - Kanpur（坎普尔印度理工学院）
Quantized spin waves, or magnons, in a magnetic insulator are assumed to interact weakly with the surroundings, and to flow with little dissipation or drag, producing exceptionally long diffusion lengths and relaxation times. In analogy to Coulomb drag in bilayer two dimensional electron gases, in which the contribution of the Coulomb interaction to the electric resistivity is studied by measuring the interlayer resistivity (transresistivity), we predict a nonlocal drag of magnons in a ferromagnetic bilayer structure based on semiclassical Boltzmann equations. Nonlocal magnon drag depends on m…
Several recent experiments have reported an anomalous temperature dependence of the Coulomb drag effect in electron-hole bilayers. Motivated by these puzzling data, we study theoretically a low-density electron-hole bilayer, where electrons and holes avoid quantum degeneracy by forming excitonic molecules. We describe the ionization-recombination crossover between the electron-hole plasma and exciton gas and calculate both the intralayer and drag resistivity as a function of temperature. The latter exhibits a minimum followed by a sharp upturn at low temperatures in a qualitative agreement wit…
We present measurements of Coulomb drag in an ambipolar GaAs/AlGaAs double quantum well structure that can be configured as both an electron-hole bilayer and a hole-hole bilayer, with an insulating barrier of only 10 nm between the two quantum wells. The Coulomb drag resistivity is a direct measure of the strength of the interlayer particle-particle interactions. We explore the strongly interacting regime of low carrier densities (2D interaction parameter $r_s$ up to 14). Our ambipolar device design allows comparison between the effects of the attractive electron-hole and repulsive hole-hole i…
We report Coulomb drag measurements on GaAs-AlGaAs electron-hole bilayers. The two layers are separated by a 10 or 25nm barrier. Below T$\approx$1K we find two features that a Fermi-liquid picture cannot explain. First, the drag on the hole layer shows an upturn, which may be followed by a downturn. Second, the effect is either absent or much weaker in the electron layer, even though the measurements are within the linear response regime. Correlated phases have been anticipated in these, but surprisingly, the experimental results appear to contradict Onsager's reciprocity theorem.
We consider a hydrodynamic description of transport for generic two dimensional electron systems that lack Galilean invariance and do not fall into the category of Fermi liquids. We study magnetoresistance and show that it is governed only by the electronic viscosity provided that the wavelength of the underlying disorder potential is large compared to the microscopic equilibration length. We also derive the Coulomb drag transresistance for double-layer non-Fermi liquid systems in the hydrodynamic regime. As an example, we consider frictional drag between two quantum Hall states with half-fill…
We theoretically calculate the interaction-induced frictional Coulomb drag resistivity between two graphene monolayers as well as between two graphene bilayers, which are spatially separated by a distance "$d$". We show that the drag resistivity between graphene monolayers can be significantly affected by the intralayer momentum-relaxation mechanism. For energy independent intralayer scattering, the frictional drag induced by inter-layer electron-electron interaction goes asymptotically as $ρ_D \sim T^2/n^4d^6$ and $ρ_D \sim T^2/n^2d^2$ in the high-density ($k_F d \gg 1$) and low-density ($k_F…
We have fabricated bilayer-graphene double layers separated by a thin ($\sim$20 nm) boron nitride layer and performed Coulomb drag and counterflow thermoelectric transport measurements. The measured Coulomb drag resistivity is nearly three orders smaller in magnitude than the intralayer resistivities. The counterflow Seebeck coefficient is found to be well approximated by the difference between Seebeck coefficients of individual layers and exhibit a peak in the regime where two layers have opposite sign of charge carriers. The measured maximum counterflow power factor is $\sim$ 700 $μ$W/K$^2$c…
We study a bilayer structure consisting of an antiferromagnetic insulator and a normal metal. An electron current is driven in the normal metal with direction parallel to the interface between the materials. Due to interfacial exchange coupling between the localized spins in the antiferromagnet and the itinerant electrons in the normal metal, a magnon current can then be induced in the antiferromagnet. Using an uncompensated antiferromagnetic interface, creating an asymmetry in the interfacial coupling to the two degenerate magnon modes, we find that it is possible to generate a magnon spin-cu…
We show that Coulomb drag in hydrodynamic bilayer systems leads to additional viscosity terms in the hydrodynamic equations, i.e., the drag and drag-Hall viscosities, besides the well-known kinematic and Hall viscosities. These new viscosity terms arise from a change of the stress tensor due to the interlayer Coulomb interactions. All four viscosity terms are tunable by varying the applied magnetic field and the electron densities in the two layers. At certain ratios between the electron densities in the two layers, the drag viscosity dramatically changes the longitudinal transport resulting i…
We propose a phenomenological model that describes counterflow and drag experiments with quantum Hall bilayers in a ν_T=1 state. We consider the system consisting of statistically distributed areas with local total filling factors ν_{T1}>1 and ν_{T2}<1. The excess or deficit of electrons in a given area results in an appearance of vortex excitations. The vortices in quantum Hall bilayers are charged. They are responsible for a decay of the exciton supercurrent, and, at the same time, contribute to the conductivity directly. The experimental temperature dependence of the counterflow and drive r…
By applying a self-consistent Hartree-Fock approximation, we show that the mechanism of dynamical symmetry breaking can account for the insulating phase that develops about the charge neutrality point of twisted bilayer graphene around the magic angle. ($i$) If the Coulomb interaction is screened by metallic gates, the opening of a gap between the lowest-energy valence and conduction bands proceeds through the breakdown of chiral symmetry at strong coupling. Increasing the dielectric screening, however, we find a critical coupling at which chiral symmetry breaking is suppressed, triggering a v…
Exciton condensation in an electron-hole bilayer system of monolayer transition metal dichalcogenides is analyzed at three different levels of theory to account for screening and quasiparticle renormalization. The large effective masses of the transition metal dichalcogenides place them in a strong coupling regime. In this regime, mean field (MF) theory with either an unscreened or screened interlayer interaction predicts a room temperature condensate. Interlayer and intralayer interactions renormalize the quasiparticle dispersion, and this effect is included in a GW approximation. The renorma…
Electron interactions in undoped bilayer graphene lead to instability of the gapless state, `which-layer' symmetry breaking, and energy gap opening at the Dirac point. In contrast to single layer graphene, the bilayer system exhibits instability even for arbitrarily weak interaction. A controlled theory of this instability for realistic dynamically screened Coulomb interactions is developed, with full acount of dynamically generated ultraviolet cutoff. This leads to an energy gap that scales as a power law of the interaction strength, making the excitonic instability readily observable.
Interlayer exciton condensates between second Landau level orbitals in double bilayer graphene
Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室）；University of California, Berkeley（加州大学伯克利分校）；Harvard University（哈佛大学）；National Institute for Material Science（国立材料研究所）
We develop a theory for quantum phases and quantum multicriticality in bilayer graphene in the presence of an explicit energy gap in the non-interacting spectrum by extending previous renormalization group (RG) analyses of electron-electron interactions in gapless bilayer graphene at finite temperature to include the effect of an electric field applied perpendicular to the sample. We determine the possible outcomes of the resulting RG equations, represented by "fixed rays" along which ratios of the coupling constants remain constant and map out the leading instabilities of the system for an in…
The static dielectric function in AA-stacked bilayer graphene (BLG), subjected to an electric field applied perpendicular to layers, is calculated analytically within the random phase approximation (RPA). This result is used to calculate the screened Coulomb interaction and the electrical conductivity. The screened Coulomb interaction, which here can be tuned by the perpendicular electric field, shows a power-law decay as $1/(γ^{2}+V^2)$ at long-distance limit where $V$ and $γ$ are the electrical potential and the inter-layer hopping energy respectively, indicating that the Coulomb interaction…
Quantifying superlubricity of bilayer graphene from the mobility of interface dislocations
University of Illinois at Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校）；Material Research Laboratory, University of Illinois at Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校材料研究实验室）
Correlated charge inhomogeneity breaks the electron-hole symmetry in two-dimensional (2D) bilayer heterostructures which is responsible for non-zero drag appearing at the charge neutrality point. Here we report Coulomb drag in novel drag systems consisting of a two-dimensional graphene and a one dimensional (1D) InAs nanowire (NW) heterostructure exhibiting distinct results from 2D-2D heterostructures. For monolayer graphene (MLG)-NW heterostructures, we observe an unconventional drag resistance peak near the Dirac point due to the correlated inter-layer charge puddles. The drag signal decreas…
Coulomb drag is a process whereby the repulsive interactions between electrons in spatially separated conductors enable a current flowing in one of the conductors to induce a voltage drop in the other. If the second conductor is part of a closed circuit, a net current will flow in that circuit. The drag current is typically much smaller than the drive current owing to the heavy screening of the Coulomb interaction. There are, however, rare situations in which strong electronic correlations exist between the two conductors. For example, bilayer two-dimensional electron systems can support an ex…
Using the semiclassical quantum Boltzmann equation (QBE), we numerically calculate the DC transport properties of bilayer graphene near charge neutrality. We find, in contrast to prior discussions, that phonon scattering is crucial even at temperatures below 40K. Nonetheless, electron-electron scattering still dominates over phonon collisions allowing a hydrodynamic approach. We introduce a simple two-fluid hydrodynamic model of electrons and holes interacting via Coulomb drag and compare our results to the full QBE calculation. We show that the two-fluid model produces quantitatively accurate…
