In the framework of the Lindblad theory for open quantum systems we determine the degree of quantum decoherence and classical correlations of a harmonic oscillator interacting with a thermal bath. The transition from quantum to classical behaviour of the considered system is analyzed and it is shown that the classicality takes place during a finite interval of time. We calculate also the decoherence time and show that it has the same scale as the time after which statistical fluctuations become comparable with quantum fluctuations.
It is shown how possible corrections to ordinary quantum mechanics described by the Lindblad equation might be detected by exploiting the great precision of atomic clocks.
In the framework of the Lindblad theory for open quantum systems, expressions for the density operator, von Neumann entropy and effective temperature of the damped harmonic oscillator are obtained. The entropy for a state characterized by a Wigner distribution function which is Gaussian in form is found to depend only on the variance of the distribution function. We give a series of inequalities, relating uncertainty to von Neumann entropy and linear entropy. We analyze the conditions for purity of states and show that for a special choice of the diffusion coefficients, the correlated coherent…
In this work, we studied the relaxation dynamics of coherences of different order present in a system of two coupled nuclear spins. We used a previously designed model for intrinsic noise present in such systems which considers the Lindblad master equation for Markovian relaxation. We experimentally created zero-, single- and double- quantum coherences in several two-spin systems and performed a complete state tomography and computed state fidelity. We experimentally measured the decay of zero- and double- quantum coherences in these systems. The experimental data fitted well to a model that c…
The quantum dynamics of a damped and forced harmonic oscillator is investigated in terms of a Lindblad master equation. Elementary algebraic techniques are employed allowing for example to analyze the long time behavior, i.e. the quantum limit cycle. The time evolution of various expectation values is obtained in closed form as well as the entropy and the Husimi phase space distribution. We also discuss the related description in terms of a non-Hermitian Hamiltonian.
In the framework of the Lindblad theory for open quantum systems, a master equation for the quantum harmonic oscillator interacting with a dissipative environment, in particular with a thermal bath, is derived for the case when the interaction is based on deformed algebra. The equations of motion for observables strongly depend on the deformation function. The expectation values of the number operator and squared number operator are calculated in the limit of a small deformation parameter for the case of zero temperature of the thermal bath. The steady state solution of the equation for the de…
Zurek, Habib and Paz [W. H. Zurek, S. Habib and J. P. Paz, Phys. Rev. Lett. {\bf 70} (1993)\ 1187] have characterized the set of states of maximal stability defined as the set of states having minimum entropy increase due to interaction with an environment, and shown that coherent states are maximal for the particular environment model examined. To generalize these results, I consider entropy production within the Lindblad theory of open systems, treating environment effects perturbatively. I characterize the maximally predicitive states which emerge from several forms of effective dynamics, i…
A Mean-Field Lindblad Master Equation Framework for Interaction-Driven Decoherence in Solid-State Qubit Ensembles
Department of Chemistry, University of Colorado Boulder（科罗拉多大学博尔德分校化学系）；Ann and H.J. Smead Aerospace Engineering Sciences, University of Colorado Boulder（科罗拉多大学博尔德分校安恩和H.J.斯米德航空航天工程科学）
Decoherence of quantum systems from entanglement with an unmonitored environment is to date the most compelling explanation of the emergence of a classical picture from a quantum world. While it is well understood for a single Lindblad operator, the role in the einselection process of a complex system-environment interaction remains to be clarified. In this paper, we analyze an open quantum dynamics inspired by CQED experiments with two non-commuting Lindblad operators modeling decoherence in the number basis and dissipative decoherence in the coherent state basis. We study and solve exactly t…
In the framework of the Lindblad theory for open quantum systems, we derive closed analytical expressions of the Heisenberg and Schrödinger generalized uncertainty functions for a particle moving in a harmonic oscillator potential. The particle is initially in an arbitrary correlated coherent state, and interacts with an environment at finite temperature. We describe how the quantum and thermal fluctuations contribute to the uncertainties in the canonical variables of the system and analyze the relative importance of these fluctuations in the evolution of the system. We show that upon contact …
Within the framework of the Lindblad master equation, we propose a general methodology to describe the effects of the environment on a system in dilute gas phase. The phenomenological parameters characterizing the transitions between rovibrational states of the system induced by collisions can be extracted from experimental transition kinetic constants, relying on Energy Gap fitting laws. As the availability of this kind of experimental data can be limited, the present work relied on experimental line broadening coefficients, however still using Energy Gap fitting laws. The 3 $μ$m infrared spe…
A single quantum dissipative oscillator described by the Lindblad equation serves as a model for a nanosystem. This model is solved exactly by using the ambiguity function. The solution shows the features of decoherence (spatial extent of quantum behavior), correlation (spatial scale over which the system localizes to its physical dimensions), and mixing (mixed- state spatial correlation). A new relation between these length scales is obtained here. By varying the parameters contained in the Lindblad equation, it is shown that decoherence and correlation can be controlled. We indicate possible…
Control of quantum dissipative systems can be challenging because control variables are typically part of the system Hamiltonian, which can only generate motion along unitary orbits of the system. To transit between orbits, one must harness the dissipation super-operator. To separate the inter-orbit dynamics from the Hamiltonian dynamics for a generic two-dimensional system, we project the Lindblad master equation onto the set of spectra of the density matrix, and we interpret the location along the orbit to be a new control variable. The resulting differential equation allows us to analyze th…
The Lindblad equation governs general markovian evolution of the density operator in an open quantum system. An expression for the rate of change of the Wigner function as a sum of integrals is one of the forms of the Weyl representation for this equation. The semiclassical description of the Wigner function in terms of chords, each with its classically defined amplitude and phase, is thus inserted in the integrals, which leads to an explicit differential equation for the Wigner function. All the Lindblad operators are assumed to be represented by smooth phase space functions corresponding to …
By using the complete solution of the Milburn equation (beyond the Lindblad form that it is generally used) that describes intrinsic decoherence, we study the decaying dynamics of a displaced harmonic oscillator. We calculate the expectation values of position quadrature, and the number operator in initial coherent and squeezed states.
A pair of coupled quantum dissipative oscillators, serving as a model for a nanosystem, is here described by the Lindblad equation. Its dynamic evolution is shown to exhibit the features of decoherence (spatial extent of quantum behavior), correlation (spatial scale over which the system localizes to its physical dimensions), and entanglement (a special quantum feature making its appearance first in such bipartite systems) as a function of the coupling constants of the Lindblad equation. One interesting feature emerging out of this calculation is that the entanglement may exhibit revivals in t…
We investigate how to model Markovian evolution of coupled harmonic oscillators, each of them interacting with a local environment. When the coupling between the oscillators is weak, dissipation may be modeled using local Lindblad terms for each of the oscillators in the master equation, as is commonly done. When the coupling between oscillators is strong, this model may become invalid. We derive a master equation for two coupled harmonic oscillators which are subject to individual heat baths modeled by a collection of harmonic oscillators, and show that this master equation in general contain…
We investigate departures from the Hamiltonian dynamics such as the quantum decoherence in a supersymmetric quantum system due to its interaction with the environment. The effective description is given by the Franke-Gorini-Kossakowski-Lindblad-Sudarshan (FGKLS) equation. The prescription for supersymmetrization of this equation is elaborated and pairs of related isospectral quantum systems are built. We present some instructive examples of such a construction.
We use the Bloch-Redfield-Wangsness theory to calculate the effects of acoustic phonons in coherent control experiments, where quantum-dot excitons are driven by shaped laser pulses. This theory yields a generalized Lindblad equation for the density operator of the dot, with time-dependent damping and decoherence due to phonon transitions between the instantaneous dressed states. It captures similar physics to the form recently applied to Rabi oscillation experiments [A. J. Ramsay et al., Phys. Rev. Lett. 104, 017402 (2010)], but guarantees positivity of the density operator. At sufficiently l…
We prove that a harmonic oscillator driven by Lindblad dynamics where the typical drive and loss channels are two-photon processes instead of single-photon ones, converges to a protected subspace spanned by two coherent states of opposite amplitude. We then characterize the slow dynamics induced by a perturbative single-photon loss on this protected subspace, by performing adiabatic elimination in the Lindbladian dynamics.
The quantum dynamics of a damped and forced harmonic oscillator described by a Lindblad master equation is analyzed. The master equation is converted into a matrix-vector representation and the resulting non-Hermitian Schrödinger equation is solved by Lie-algebraic techniques allowing the construction of the general solution for the density operator.
We consider the simple hypothesis of letting quantum systems have an inherent random nature. Using well-known stochastic methods we thus derive a stochastic evolution operator which let us define a stochastic density operator whose expectation value under certain conditions satisfies a Lindblad equation. As natural consequences of the former assumption decoherence and spontaneous emission processes are obtained under the same conceptual scheme. A temptative solution for the preferred basis problem is suggested. All this is illustrated with a comprehensive study of a two-level quantum system ev…
We propose a novel symmetrization procedure to beat decoherence for oscillator-assisted quantum gate operations. The enacted symmetry is related to the global geometric features of qubits transformation based on ancillary oscillator modes, e.g. phonons in an ion-trap system. It is shown that the devised multi-circuit symmetrized evolution endows the system with a two-fold resilience against decoherence: insensitivity to thermal fluctuations and quantum dissipation.
Quantum dissipation is studied within two model oscillators, the Caldirola-Kanai (CK) oscillator as an open system with one degree of freedom and the Bateman-Feshbach-Tikochinsky (BFT) oscillator as a closed system with two degrees of freedom. Though these oscillators describe the same classical damped motion, the CK oscillator retains the quantum coherence, whereas the damped subsystem of the BFT oscillator exhibits both quantum decoherence and classical correlation. Furthermore the amplified subsystem of the BFT oscillator shows the same degree of quantum decohernce and classical correlation…
In the framework of the Lindblad theory for open quantum systems, we determine the degree of quantum decoherence of a harmonic oscillator interacting with a thermal bath. It is found that the system manifests a quantum decoherence which is more and more significant in time. We calculate also the decoherence time scale and analyze the transition from quantum to classical behaviour of the considered system.
These lecture notes address an audience of physicists or mathematicians who have been exposed to a first course in quantum mechanics. We start with a brief discussion of the general "system-bath" paradigm of quantum dissipative systems, analyze in some detail the simplest example of "pure dephasing" of a two-level system, and review the basic concept of the density matrix. We then treat the general dissipative time-evolution, introducing completely positive maps, their relation to entanglement theory, and their Kraus decomposition. Restricting ourselves to Markovian evolution, we discuss the L…
We investigate the decoherence of histories of local densities for linear oscillators models. It is shown that histories of local number, momentum and energy density are approximately decoherent, when coarse-grained over sufficiently large volumes. Decoherence arises directly from the proximity of these variables to exactly conserved quantities (which are exactly decoherent), and not from environmentally-induced decoherence. We discuss the approach to local equilibrium and the subsequent emergence of hydrodynamic equations for the local densities.
With time-dependent Lindblad operators, an open system may have a time-dependent decoherence-free subspace (t-DFS). In this paper, we define the t-DFS and present a necessary and sufficient condition for the t-DFS. Two examples are presented to illustrate the t-DFS, showing that this t-DFS is not trivial, when the dimension of the t-DFS varies.
In the framework of the Lindblad theory for open quantum systems, we determine the degree of quantum decoherence of a harmonic oscillator interacting with a thermal bath. It is found that the system manifests a quantum decoherence which is more and more significant in time. We also calculate the decoherence time and show that it has the same scale as the time after which thermal fluctuations become comparable with quantum fluctuations.
Applying the Milburn equation to describe intrinsic decoherence, we study the interaction of three-coupled quantum harmonic oscillators or quantized fields. We give an explicit solution for the complete equation, i.e., beyond the usual second order approximation used to arrive to the Lindblad form. Then we calculate the expectation value of the number operator of each oscillator or mode for one of the modes given in an initial coherent
The dynamics of a quantum anharmonic oscillator whose position is monitored by a Bose-Einstein condensate (BEC) trapped in a symmetric double well potential is studied. The (non-exponential) decoherence induced on the oscillator by the measuring device is analysed. A detailed quasiclassical and quantum analysis is presented. In the first case, for an arbitrary initial coherent state, two different decoherence regimes are observed: An initial Gaussian decay followed by a power law decay for longer times. The characteristic time scales of both regimes are reported. Analytical approximated expres…
We study three methods of obtaining an approximation of unitary evolution of a quantum system under decoherence. We use three methods of optimizing the control pulses: genetic optimization, approximate evolution method and approximate gradient method. To model the noise in the system we use the Lindblad equaiton. We obtain results showing that genetic optimization may give a better approximation of a unitary evolution in the case of high noise.
The equilibrium properties of an open harmonic oscillator are considered in three steps: First the creation and destruction operators are generalized for open dynamics and the creation operator is used to construct coherent states. The second step consists of the introduction of the Heisenberg representation where the dynamical decoherence can be identified without making reference to the state of the system. Finally it is pointed out that the quantum fluctuations generate non-continuous limit for infinitesimal system-environment interactions and at the border of the under- and over-damped osc…
In the framework of the Lindblad theory for open quantum systems the damping of the harmonic oscillator is studied. A generalization of the fundamental constraints on quantum mechanical diffusion coefficients which appear in the master equation for the damped quantum oscillator is presented; the Schrödinger and Heisenberg representations of the Lindblad equation are given explicitly. On the basis of these representations it is shown that various master equations for the damped quantum oscillator used in the literature are particular cases of the Lindblad equation and that the majority of these…
Using the numerical path integral method we investigate the decoherence and relaxation of qubits coupled to an Ohmic bath directly and via an intermediate harmonic oscillator (IHO). Here, we suppose the oscillation frequencies of the bath modes are higher than the IHO's. When we choose suitable parameters the qubits in the two models may have almost same decoherence and relaxation times. However, the decoherence and relaxation times of the qubit in the qubit-IHO-bath model can be modulated through changing the coupling coefficients of the qubit-IHO and IHO-bath and the oscillation frequency of…
Using the numerical path integral method we investigate the decoherence and relaxation of qubits in spin-boson (SB) and spin-intermediate harmonic oscillator (IHO)-bath (SIB) models. The cases that the environment baths with low and medium frequencies are investigated. It is shown that the qubits in SB and SIB models have the same decoherence and relaxation as the baths with low frequencies. However, the qubits in the two models have different decoherence and relaxation as the baths with medium frequencies. The decoherence and relaxation of the qubit in SIB model can be modulated through chang…
We study the intrinsic decoherence of coupled harmonic oscillators. The Milburn master equation is solved exactly, and the dynamics of virtual ground state excitations are investigated. The interaction of quantum correlations and virtual excitation was then studied. The following is a summary of our major findings. (i) The damped oscillatory profile of all three quantities is the same. (ii) Ultra-strong coupling combined with huge anisotropy values results in the reemergence of entanglement and steering. (iii) To sustain entanglement and steering, virtual excitations are required. (iv) The qua…
In the framework of the Lindblad theory for open quantum systems we determine the degree of quantum decoherence and classical correlations of a harmonic oscillator interacting with a thermal bath. The transition from quantum to classical behaviour of the considered system is analyzed and it is shown that the classicality takes place during a finite interval of time. We calculate also the decoherence time and show that it has the same scale as the time after which thermal fluctuations become comparable with quantum fluctuations.
In this paper we present a comprehensive analysis of the coherence phenomenon of two coupled dissipative oscillators. The action of a classical driving field on one of the oscillators is also analyzed. Master equations are derived for both regimes of weakly and strongly interacting oscillators from which interesting results arise concerning the coherence properties of the joint and the reduced system states. The strong coupling regime is required to achieve a large frequency shift of the oscillator normal modes, making it possible to explore the whole profile of the spectral density of the res…
A longstanding challenge in the foundations of quantum mechanics is the verification of alternative collapse theories despite their mathematical similarity to decoherence. To this end, we suggest a novel method based on dynamical decoupling. Experimental observation of nonzero saturation of the decoupling error in the limit of fast decoupling operations can provide evidence for alternative quantum theories. As part of the analysis we prove that unbounded Hamiltonians can always be decoupled, and provide novel dilations of Lindbladians.
The description of the dynamics of closed quantum systems, governed by the Schroedinger equation at first sight seems incompatible with the Lindblad equation describing open ones. By analyzing closed dynamics of a spin-1/2 chain we reconstruct exponential decays characteristic for the latter model. We identify all necessary ingredients to efficiently model this behavior, such as an infinitely large environment and the coupling to the system weak in comparison to the internal couplings in the bath.
We derive and analyze the Born-Markov master equation for a quantum harmonic oscillator interacting with a bath of independent two-level systems. This hitherto virtually unexplored model plays a fundamental role as one of the four "canonical" system-environment models for decoherence and dissipation. To investigate the influence of further couplings of the environmental spins to a dissipative bath, we also derive the master equation for a harmonic oscillator interacting with a single spin coupled to a bosonic bath. Our models are experimentally motivated by quantum-electromechanical systems an…
A Lindblad master equation for a harmonic oscillator, which describes the dynamics of an open system, is formally solved. The solution yields the spectral resolution of the Liouvillian, that is, all eigenvalues and eigenprojections are obtained. This spectral resolution is discussed in depth in the context of the biorthogonal system and the rigged Hilbert space, and the contribution of each eigenprojection to expectation values of physical quantities is revealed. We also construct the ladder operators of the Liouvillian, which clarify the structure of the spectral resolution.
We introduce the quantitative measures characterizing the rates of decoherence and thermalization of quantum systems. We study the time evolution of these measures in the case of a quantum harmonic oscillator whose relaxation is described in the framework of the standard master equation, for various initial states (coherent, `cat', squeezed and number). We establish the conditions under which the true decoherence measure can be approximated by the linear entropy $1-{Tr}\hatρ^2$. We show that at low temperatures and for highly excited initial states the decoherence process consists of three dis…
Time-dependent density-matrix propagation is used to demonstrate, in a schematic model of an open quantum system, that the complex potential approach and the Lindblad dissipative dynamics are \emph{not} equivalent. While the former preserves coherence, it is destroyed in the Lindblad dissipative dynamics. Quantum decoherence is the key aspect that makes the difference between the two approaches, indicating that the complex potential model is inadequate for a consistent description of open quantum-system dynamics. It is suggested that quantum decoherence should always be explicitly included whe…
Master equations govern the time evolution of a quantum system interacting with an environment, and may be written in a variety of forms. Time-independent or memoryless master equations, in particular, can be cast in the well-known Lindblad form. Any time-local master equation, Markovian or non-Markovian, may in fact also be written in a Lindblad-like form. A diagonalisation procedure results in a unique, and in this sense canonical, representation of the equation, which may be used to fully characterize the non-Markovianity of the time evolution. Recently, several different measures of non-Ma…
We study the spontaneous decoherence of the coupled harmonic oscillators confined in a ring container, where the nearest-neighbor harmonic potentials are taken into consideration. Without any external symmetry breaking field or surrounding environment, the quantum superposition state prepared in the relative degrees of freedom gradually loses its quantum coherence spontaneously. This spontaneous decoherence is interpreted by the hidden couplings between the center-of-mass and relative degrees of freedoms, which actually originates from the symmetries of the ring geometry and corresponding nont…
We investigate system-environment correlations based on the exact dynamics of a qubit and its environment in the framework of pure decoherence (phase damping). We focus on the relation of decoherence and the build-up of system-reservoir entanglement for an arbitrary (possibly mixed) initial qubit state. In the commonly employed regime where the qubit dynamics can be described by a Markov master equation of Lindblad type, we find that for almost all qubit initial states inside the Bloch sphere, decoherence is complete while the total state is still separable - no entanglement is involved. In ge…
We consider an open quantum system described by a Lindblad-type master equation with two times-scales. The fast time-scale is strongly dissipative and drives the system towards a low-dimensional decoherence-free space. To perform the adiabatic elimination of this fast relaxation, we propose a geometric asymptotic expansion based on the small positive parameter describing the time-scale separation. This expansion exploits geometric singular perturbation theory and center-manifold techniques. We conjecture that, at any order, it provides an effective slow Lindblad master equation and a completel…
In this paper we analyze the double Caldeira-Leggett model: the path integral approach to two interacting dissipative harmonic oscillators. Assuming a general form of the interaction between the oscillators, we consider two different situations: i) when each oscillator is coupled to its own reservoir, and ii) when both oscillators are coupled to a common reservoir. After deriving and solving the master equation for each case, we analyze the decoherence process of particular entanglements in the positional space of both oscillators. To analyze the decoherence mechanism we have derived a general…
An important issue in developing quantum technology is that quantum states are so sensitive to noise. We propose a protocol that introduces reverse dynamics, in order to precisely control quantum systems against noise described by the Lindblad master equation. The reverse dynamics can be obtained by constructing the Petz recovery map in continuous time. By providing the exact form of the Hamiltonian and jump operators for the reverse dynamics, we explore the potential of utilizing the near-optimal recovery of the Petz map in controlling noisy quantum dynamics. While time-dependent dissipation …
In the framework of Lindblad theory for open quantum systems, we calculate the entropy of a damped quantum harmonic oscillator which is initially in a quasi-free state. The maximally predictable states are identified as those states producing the minimum entropy increase after a long enough time. In general, the states with a squeezing parameter depending on the environment's diffusion coefficients and friction constant are singled out, but if the friction constant is much smaller than the oscillator's frequency, coherent states (or thermalized coherent states) are obtained as the preferred cl…
The time development of the reduced density matrix for a quantum oscillator damped by coupling it to an ohmic environment is calculated via an identity of the Debye-Waller form. Results obtained some years ago by Hakim and the author in the free particle limit [1] are thus recovered. The evolution of a free particle in a prepared initial state is examined, and a previously published exchange [2,3] is illuminated with figures showing no decoherence without dissipation. [1] V. Hakim and V. Ambegaokar, Phys. Rev. A 32, 423 (1985). [2] G.W. Ford and R.F. O'Connell, Phys. Rev. A 70, 026102 (2004). …
We study standard quantum teleportation of one-qubit state for the situation in which the channel is subject to decoherence, and where the evolution of the channel state is ruled by a master equation in the Lindblad form. A detailed calculation reveals that the quality of teleportation is determined by both the entanglement and the purity of the channel state, and only the optimal matching of them ensures the highest fidelity of standard quantum teleportation. Also our results demonstrated that the decoherence induces distortion of the Bloch sphere for the output state with different rates in …
The Lindblad master equation for an open quantum system with a Hamiltonian containing an arbitrary potential is written as an equation for the Wigner distribution function in the phase space representation. The time derivative of this function is given by a sum of three parts: the classical one, the quantum corrections and the contribution due to the opening of the system. In the particular case of a harmonic oscillator, quantum corrections do not exist.
