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arXiv 0704.1887cond-mat.supr-con
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YBa_2Cu_3O_6+x中60 K平台的起源

Origin of the 60K plateau in YBa_2Cu_3O_6+x

V. M. Matic, N. Dj. Lazarov

摘要:

基于临界链长的概念,提出了YBa_2Cu_3O_(6 +x)高Tc铜酸盐的电荷转移机制模型,用以解释Tc(x)依赖性的60 K和90 K平台。用二维非对称次近邻Ising(ASYNNNI)模型描述CuO链形成的统计特性时,发现在低于OII相顶部的任何恒定温度下,都存在一个唯一确定的临界链长lcr(T)值,该值在OII相区域内产生恒定的掺杂p(x)=const(与Tc(x)的60 K平台相关),而90 K平台与在OI相区域中在最佳掺杂水平p=0.16上单调增加的p(x)一致。短链(l<lcr(T))与较长链(l>lcr(T))中的第一个lcr(T)-2空穴一起被认为不能从CuO 2平面吸引电子。结果表明,长链中剩余的l-lcr(T)+1空穴中只有一部分(41%)能俘获电子.结果表明,YBa_2Cu_3O_(6 +x)中Tc(x)的ASYNNNI模型与双平台行为密切相关。

英文摘要:

A model for charge transfer mechanism in YBa2Cu3O6+x high-Tc cuprate based on critical chain length concept is proposed to account for 60K and 90K plateaus in Tc(x) dependence. It has been shown, when the statistics of CuO chain formation was described in terms of two dimensional asymmetric next-to-nearest neighbor Ising (ASYNNNI) model, that at any constant temperature below the top of OII phase there exists a uniquely defined value of critical chain length lcr(T) that yields a constant doping p(x)=const over the regime of OII phase (related to 60K plateau of Tc(x)), while 90K plateau coincides with the monotonously increasing p(x) over optimal doping level p=0.16 in the regime of OI phase. Short length chains (l<lcr(T)), together with the first lcr(T)-2 holes in longer chains (l>lcr(T)), are taken as not capable of attracting electrons from CuO2 planes.. It is shown that only a part (41%) of the remaining l-lcr(T)+1 holes in the long chains can capture electrons. The results obtained indicate that the ASYNNNI model and two-plateaus-like behavior of Tc(x) in YBa2Cu3O6+x are closely connected.

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