We study the coherent association of a two-species atomic condensate into a condensate of heteronuclear diatomic molecules, using both a semiclassical treatment and a quantum mechanical approach. The differences and connections between the two approaches are examined. We show that, in this coupled nonlinear atom-molecule system, the population difference between the two atomic species plays a significant role in the ground-state stability properties as well as in coherent population oscillation dynamics.
We study a three-mode Hamiltonian modelling a heteronuclear molecular Bose--Einstein condensate. Two modes are associated with two distinguishable atomic constituents, which can combine to form a molecule represented by the third mode. Beginning with a semi-classical analogue of the model, we conduct an analysis to determine the phase space fixed points of the system. Bifurcations of the fixed points naturally separate the coupling parameter space into different regions. Two distinct scenarios are found, dependent on whether the imbalance between the number operators for the atomic modes is ze…
We report the realization of a heteronuclear two-atom of $^{87}$Rb-$^{85}$Rb in the ground state of an optical tweezer (OT). Starting by trapping two different isotopic single atoms, a $^{87}$Rb and a $^{85}$Rb in two strongly focused and linearly polarized OT with 4 $μ$m apart, we perform simultaneously three dimensional Raman sideband cooling for both atoms and the obtained 3D ground state probabilities of $^{87}$Rb and $^{85}$Rb are 0.91(5) and 0.91(10) respectively. There is no obvious crosstalk observed during the cooling process. We then merge them into one tweezer via a species-dependen…
We present the formation of homonuclear Cs2, K2, and heteronuclear CsK long-range Rydberg molecules in a dual-species magneto-optical trap for 39K and 133Cs by one-photon UV photoassociation. The different ground-state-density dependence of homo- and heteronuclear photoassociation rates and the detection of stable molecular ions resulting from auto-ionization provide an unambiguous assignment. We perform bound-bound millimeter-wave spectroscopy of long-range Rydberg molecules to access molecular states not accessible by one-photon photoassociation. Calculations based on the most recent theoret…
We show that the use of a generalized atom-molecule dark state permits the enhanced coherent creation of triatomic molecules in a repulsive atomic Bose-Einstein condensate, with further enhancement being possible in the case of heteronuclear trimers via the constructive interference between two chemical reaction channels.
Quantum entanglement is crucial for simulating and understanding exotic physics of strongly correlated many-body systems, such as high--temperature superconductors, or fractional quantum Hall states. The entanglement of non-identical particles exhibits richer physics of strong many-body correlations and offers more opportunities for quantum computation, especially with neutral atoms where in contrast to ions the interparticle interaction is widely tunable by Feshbach resonances. Moreover, the inter-species entanglement forms a basis for the properties of various compound systems, ranging from …
We demonstrate a generally applicable technique for mixing two-species quantum degenerate bosonic samples in the presence of an optical lattice, and we employ it to produce low-entropy samples of ultracold 87Rb133Cs Feshbach molecules with a lattice filling fraction exceeding 30%. Starting from two spatially separated Bose-Einstein condensates of Rb and Cs atoms, Rb-Cs atom pairs are efficiently produced by using the superfluid-to-Mott insulator quantum phase transition twice, first for the Cs sample, then for the Rb sample, after nulling the Rb-Cs interaction at a Feshbach resonance's zero cr…
We present a stability analysis of an interacting two-species Bose-Einstein condensate driven by a quantized field in the semi-classical limit. Transitions from Rabi to Josephson dynamics are identified depending on both the inter-atomic interaction to field-condensate coupling ratio and the ratio between the total excitation number and the condensate size. The quantized field is found to produce asymmetric dynamics for symmetric initial conditions for both Rabi and Josephson oscillations.
Optically trapped mixed-species single atom arrays with arbitrary geometries are an attractive and promising platform for various applications, because tunable quantum systems with multiple components provide extra degrees of freedom for experimental control. Here, we report the first demonstration of two-dimensional $6\times4$ dual-species atom assembly with a filling fraction of 0.88 (0.89) for $^{85}$Rb ($^{87}$Rb) atoms. This mixed-species atomic synthetic is achieved via rearranging initially randomly distributed atoms using a sorting algorithm (heuristic heteronuclear algorithm) which is…
We model the formation of stable heteronuclear molecules via pulsed Raman photoassociation of a two-component Bose-Einstein condensate near a strong Feshbach resonance, for both counterintuitive and intuitive pulse sequencing. Compared to lasers alone, weak Raman photoassociation is enhanced by as much as a factor of ten (five) for a counterintuitive (intuitive) pulse sequence, whereas strong Raman photoassociation is barely enhanced at all--regardless of pulse sequence. Stronger intra-atom, molecule, or atom-molecule collisions lead to an expected decrease in conversion efficiency, but strong…
We study two-species Bose-Einstein condensates in quasi two-dimensional optical lattices of varying geometry and potential depth. Based on the numerically exact Bloch and Wannier functions obtained using the plane-wave expansion method, we quantify the drag (entrainment coupling) between the condensate components. This drag originates from the (short range) inter-species interaction and increases with the kinetic energy. As a result of the interplay between interaction and kinetic energy effects, the superfluid-drag coefficient shows a non-monotonic dependence on the lattice depth. To make con…
We theoretically study the loading of a two-species Bose-Einstein condensate to an optical lattice in a tightly-confined one-dimensional trap. Due to quantum fluctuations the relative inter and intra species phase coherence between the atoms and the on-site atom number fluctuations are reduced in the miscible regime. For the immiscible case the fluctuations are enhanced and the atoms form metastable interleaved spatially separated domains where the domain length and its fluctuations are affected by quantum fluctuations.
The stability analysis of a generalized Dicke model, in the semi-classical limit, describing the interaction of a two-species Bose-Einstein condensate driven by a quantized field in the presence of Kerr and spontaneous parametric processes is presented. The transitions from Rabi to Josephson dynamics are identified depending on the relative value of the involved parameters. Symmetry-breaking dynamics are shown for both types of coherent oscillations due to the quantized field and nonlinear optical processes.
Ultracold quantum gases confined in three-dimensional bubble traps are promising tools for exploring many-body effects on curved manifolds. As an alternative to the conventional technique of radio-frequency dressing, we propose to create such shell-shaped Bose-Einstein condensates in microgravity based on dual-species atomic mixtures and we analyze their properties as well as the feasibility to realize symmetrically filled shells. Beyond similarities with the radio-frequency dressing method as in the collective-excitation spectrum, our approach has several natural advantages like the robustnes…
The coupled Gross-Pitaevskii equations for the g.s. of the three-species condensates (3-BEC) have been solved analytically under the Thomas-Fermi approximation. Six types of spatial configurations in miscible phase are found. The whole parameter-space has been divided into zones each supports a specific configuration (miscible or immiscible). The borders of the zones are described by analytical formulae. Due to the division, the variation of the spatial configuration against the parameters can be visualized, and the effects of the parameters can be thereby understood. There are regions in the …
We study the coherent nonlinear tunneling dynamics of a binary mixture of Bose-Einstein condensates in a double-well potential. We demonstrate the existence of a new type of mode associated with the "swapping" of the two species in the two wells of the potential. In contrast to the symmetry breaking macroscopic quantum self-trapping (MQST) solutions, the swapping modes correspond to the tunneling dynamics that preserves the symmetry of the double well potential. As a consequence of two distinct types of broken symmetry MQST phases where the two species localize in the different potential welil…
We report on the first realization of heteronuclear dipolar quantum mixtures of highly magnetic erbium and dysprosium atoms. With a versatile experimental setup, we demonstrate binary Bose-Einstein condensation in five different Er-Dy isotope combinations, as well as one Er-Dy Bose-Fermi mixture. Finally, we present first studies of the interspecies interaction between the two species for one mixture.
We unravel the spontaneous generation of vortex-bright-soliton structures in binary Bose-Einstein condensates with a small mass imbalance between the species confined in a two-dimensional harmonic trap where one of the two species has been segmented into two parts by a potential barrier. To trigger the dynamics the potential barrier is suddenly removed and subsequently the segments perform a counterflow dynamics. We consider a relative phase difference of $π$ between the segments, while a singly quantized vortex may be imprinted at the center of the other species. The number of vortex structur…
We examine the quantum tunneling process in Bose condensates of two interacting species trapped in a double well configuration. We discover the condition under which particles of different species can tunnel as pairs through the potential barrier between two wells in opposition directions. This novel form of tunneling is due to the interspecies interaction that eliminates the self- trapping effect. The correlated motion of tunneling atoms leads to the generation of quantum entanglement between two macroscopically coherent systems.
A mixture of two kinds of identical bosons held in a harmonic potential and interacting by harmonic particle-particle interactions is discussed. This is an exactly-solvable model of a mixture of two trapped Bose-Einstein condensates which allows us to examine analytically various properties. Generalizing the treatment in [Cohen and Lee, J. Math. Phys. {\bf 26}, 3105 (1985)], closed form expressions for the ground-state energy, wave-function, and lowest-order densities are obtained and analyzed for attractive and repulsive intra-species and inter-species particle-particle interactions. A partic…
We study circularly-symmetric phase separation of vortex lattices in a rapidly rotating harmonically-trapped quasi--two-dimensional binary Bose-Einstein condensate (BEC) by introducing a weak quartic trap in one of the components. The increase of the rotational frequency in such a system is also found to generate a phase separation of the vortex lattices of an overlapping non-rotating BEC. The phase-separated vortex lattices have different structures for a binary BEC with inter-species repulsion and inter-species attraction. In the former case of a fully repulsive binary BEC the phase separati…
We propose a possible scheme for generating spin-J geometric phases using a coupled two-mode Bose-Einstein condensate (BEC). First we show how to observe the standard Berry phase using Raman coupling between two hyperfine states of the BEC. We find that the presence of intrinsic interatomic collisions creates degeneracy in energy that allows implementation of the non-Abelian geometric phases as well. The evolutions produced can be used to produce interference between different atomic species with high numbers of atoms or to fine control the difference in atoms between the two species. Finally,…
We study numerically the outcome of the phase separation instability of a dual-species Bose-Einstein condensate in an optical lattice. When only one excitation mode is unstable a bound pair of a bright and dark soliton-like structures periodically appears and disappears, whereas for more than one unstable mode a persistent soliton-antisoliton pair develops. The oscillating soliton represents a regime where the two-species condensate neither remains phase-separated nor is dynamically stable.
We study dynamical and energetic instabilities in the transport properties of Bloch waves for atomic multi-component Bose-Einstein condensates in optical lattices in the tight-binding limit. We obtain stability criteria analytically, as a function of superfluid velocities and interaction parameters, in several cases for two-component and spinor condensates. In the two-species case we find that the presence of the other condensate component can stabilize the superfluid flow of an otherwise unstable condensate and that the free space dynamical miscibility condition of the two species can be reve…
Motivated by experiments on heteronuclear Feshbach resonances in Bose mixtures, we investigate s-wave pairing of two species of bosons in an optical lattice. The zero temperature phase diagram supports a rich array of superfluid and Mott phases and a network of quantum critical points. This topology reveals an underlying structure that is succinctly captured by a two-component Landau theory. Within the second Mott lobe we establish a quantum phase transition described by the paradigmatic longitudinal and transverse field Ising model. This is confirmed by exact diagonalization of the 1D bosonic…
Binary discrete nonlinear Schrödinger equation is used to describe dynamics of two-species Bose-Einstein condensate loaded into an optical lattice. Linear inter-species coupling leads to Rabi transitions between the species. In the regime of strong nonlinearity, a wavepacket corresponding to condensate separates into localized and ballistic fractions. Localized fraction is predominantly formed by immiscible solitons consisted of only one species. Initial states without spatial separation of occupied sites expose formation of immiscible solitons after a strongly chaotic transient. We calculate …
