Recently, we have shown that for conditions under which the so-called light-shift imbalance induced blockade (LSIIB) occurs, the collective excitation of an ensemble of a multi-level atom can be treated as a closed two level system. In this paper, we describe how such a system can be used as a quantum bit (qubit) for quantum communication and quantum computing. Specifically, we show how to realize a C-NOT gate using the collective qubit and an easily accessible ring cavity, via an extension of the so-called Pellizzari scheme. We also describe how multiple, small-scale quantum computers realized using these qubits can be linked effectively for implementing a quantum internet. We describe the details of the energy levels and transitions in 87Rb atom that could be used for implementing these schemes.
We consider the dynamics of intracavity electromagnetically induced transparency (EIT) in an ensemble of strongly interacting Rydberg atoms. By combining the advantage of variable cavity lifetimes with intracavity EIT and strongly interacting Rydberg dark-state polaritons, we show that such intracavity EIT system could exhibit very strong photon blockade effect.
Current proposals focusing on neutral atoms for quantum computing are mostly based on using single atoms as quantum bits (qubits), while using cavity induced coupling or dipole-dipole interaction for two-qubit operations. An alternative approach is to use atomic ensembles as qubits. However, when an atomic ensemble is excited, by a laser beam matched to a two-level transition (or a Raman transition) for example, it leads to a cascade of many states as more and more photons are absorbed^1. In order to make use of an ensemble as a qubit, it is necessary to disrupt this cascade, and restrict the …
We propose a scheme for realizing quantum repeaters with Rydberg-blockade coupled atomic ensembles, based on a recently proposed collective encoding strategy. Rydberg-blockade mediated two-qubit gates and efficient cooperative photon emission are employed to create ensemble-photon entanglement. Thanks to deterministic entanglement swapping operations via Rydberg-based two-qubit gates, and to the suppression of multi-excitation errors by the blockade effect, the entanglement distribution rate of the present scheme is higher by orders of magnitude than the rates achieved by other ensemble-based …
The dipole blockade of multiple Rydberg excitations in mesoscopic atomic ensembles allows the implementation of various quantum information tasks using collective states of cold, trapped atoms. Precise coherent manipulations of the collective ground and single Rydberg excitation states of an atomic ensemble requires the knowledge of the number of atoms with small uncertainty. We present an efficient method to acquire such information by interrogating the atomic ensemble with resonant pulses while monitoring the resulting Rydberg excitations. We show that after several such steps accompanied by…
Previously, we had proposed the technique of light shift imbalance induced blockade which leads to a condition where a collection of non-interacting atoms under laser excitation remains combined to a superposition of the ground and the first excited states, thus realizing a collective state quantum bit which in turn can be used to realize a quantum computer. In this paper, we show first that the light shift imbalance by itself is actually not enough to produce such a blockade, and explain the reason why the limitation of our previous analysis had reached this constraint. We then show that by i…
We describe a technique for manipulating quantum information stored in collective states of mesoscopic ensembles. Quantum processing is accomplished by optical excitation into states with strong dipole-dipole interactions. The resulting ``dipole blockade'' can be used to inhibit transitions into all but singly excited collective states. This can be employed for a controlled generation of collective atomic spin states as well as non-classical photonic states and for scalable quantum logic gates. An example involving a cold Rydberg gas is analyzed.
We present a new scheme for cluster states generation based on atomic ensembles and the dipole blockade mechanism. The protocol requires identical single photon sources, one ensemble per physical qubit, and regular photodetectors. The general entangling procedure is presented, as well as a procedure that generates Q-qubit GHZ states with probability p ~ eta^{Q/2}, where eta is the combined detection and source efficiency. This is significantly more efficient than any known robust probabilistic entangling operation. The GHZ states form the basic building block for universal cluster states - a r…
We demonstrate theoretically a scheme for cluster state generation, based on atomic ensembles and the dipole blockade mechanism. In the protocol, atomic ensembles serve as single qubit systems. Therefore, we review single-qubit operations on qubit defined as collective states of atomic ensemble. Our entangling protocol requires nearly identical single-photon sources, one ultra-cold ensemble per physical qubit, and regular photodetectors. The general entangling procedure is presented, as well as a procedure that generates in a single step Q-qubit GHZ states with success probability p_success ~ …
We demonstrate $|W\rangle$ state encoding of multi-atom ensemble qubits. Using optically trapped Rb atoms the $T_2$ coherence time is 2.6(3) ms for $\bar N=7.6$ atoms and scales approximately inversely with the number of atoms. Strong Rydberg blockade between two ensemble qubits is demonstrated with a fidelity of $0.89(1)$ and a fidelity of $\sim \hspace{-.05cm}1.0$ when postselected on control ensemble excitation. These results are a significant step towards deterministic entanglement of atomic ensembles.
We propose an efficient method to filter out single atoms from trapped ensembles with unknown number of atoms. The method employs stimulated adiabatic passage to reversibly transfer a single atom to the Rydberg state which blocks subsequent Rydberg excitation of all the other atoms within the ensemble. This triggers the excitation of Rydberg blockaded atoms to short lived intermediate states and their subsequent decay to untrapped states. Using an auxiliary microwave field to carefully engineer the dissipation, we obtain a nearly deterministic single-atom source. Our method is applicable to sm…
We propose a novel scheme for high fidelity photonic controlled phase gates using Rydberg blockade in an ensemble of atoms in an optical cavity. The gate operation is obtained by first storing a photonic pulse in the ensemble and then scattering a second pulse from the cavity, resulting in a phase change depending on whether the first pulse contained a single photon. We show that the combination of Rydberg blockade and optical cavities effectively enhances the optical non-linearity created by the strong Rydberg interaction and thereby reduces the requirements for photonic quantum gates. The re…
By coupling a probe transition to a Rydberg state using electro-magnetically induced transparency (EIT) we map the strong dipole-dipole interactions onto an optical field. We characterize the resulting cooperative optical non-linearity as a function of probe strength and density. We show that the effect of dipole blockade cannot be described using a mean-field but requires an $N$-atom cooperative model. Good quantitative agreement is obtained for three atoms per blockade with the $n=60$ Rydberg state. We place an upper-limit on the dephasing rate of the blockade spheres of $<110$ kHz.
We show that Jaynes-Cummings dynamics can be observed in mesoscopic atomic ensembles interacting with a classical electromagnetic field in the regime of Rydberg blockade, where the time dynamics of the average number of Rydberg excitations in mesoscopic ensembles displays collapses and revivals typical of this model. As the frequency of Rabi oscillations between collective states of Rydberg blockaded ensembles depends on the number of interacting atoms, for randomly loaded optical dipole traps we predict collapses and revivals of Rabi oscillations. We have studied the effects of finite interac…
We present a simplified version of a repeater protocol in a cold neutral-atom ensemble with Rydberg excitations optimized for two-node entanglement generation and describe a protocol for quantum teleportation. Our proposal draws from previous proposals [Zhao, {\sl et al.}, Phys. Rev. A {\bf 81}, 052329 (2010)] and [Han, {\sl et al.} Phys. Rev. A {\bf 81}, 052311 (2010)] who described efficient and robust protocols for long-distance entanglement with many nodes. Using realistic experimental values we predict an entanglement generation rate of $\sim$25 Hz and teleportation rate of $\sim$ 5 Hz. O…
We present a fast and Quasideterministic protocol for the production of single ions and electrons from a cloud of laser cooled atoms. The approach is based on a two-step process where first a single Rydberg atom is photo-excited from a dipole-blockade configuration and subsequently ionized by an electric field pulse. We theoretically describe these excitation-ionization cycles via dynamical quantum maps and observe a rich behavior of the ionization dynamics as a function of laser Rabi frequency, pulse duration and particle number. Our results show that a fast sequential heralded production of …
We present schemes for geometric phase compensation in adiabatic passage which can be used for the implementation of quantum logic gates with atomic ensembles consisting of an arbitrary number of strongly interacting atoms. Protocols using double sequences of stimulated Raman adiabatic passage (STIRAP) or adiabatic rapid passage (ARP) pulses are analyzed. Switching the sign of the detuning between two STIRAP sequences, or inverting the phase between two ARP pulses, provides state transfer with well defined amplitude and phase independent of atom number in the Rydberg blockade regime. Using the…
Creation of quantum computer is outstanding fundamental and practical problem. The quantum computer could be used for execution of very complicated tasks which are not solvable with the classical computers. The first prototype of solid state quantum computer was created in 2009 with superconducting qubits. However, it suffers from the decoherent processes and it is desirable to find more practical encoding of qubits with long-lived coherence. It could be single impurity or vacancy centers in solids, but their interaction with electromagnetic radiation is rather weak. So, here, ensembles of ato…
In the famous quantum communication scheme developed by Duan {\it et al.}[L.M. Duan, M.D. Lukin, J.I. Cirac, and P. Zoller, Nature (London) {\bf 414} 413 (2001)], the probability of successful generating a symmetric collective atomic state with a single-photon emitted have to be far smaller than 1 to obtain an acceptable entangled state. Because of strong dipole-dipole interaction between two Rydberg atoms, more than one simultaneous excitations in an atomic ensembles are greatly suppressed, which makes it possible to excite a mesoscopic cold atomic ensemble into a singly-excited symmetric col…
Laser excitation pulses that lead to perfect adiabatic state transfer in an ensemble of three-level ladder atoms lead to highly entangled states of many atoms if their highest excited state is subject to Rydberg blockade. Solution of the Schrödinger equation shows that it is increasingly difficult to ensure the adiabatic evolution as the number of atoms increases. A diminishing energy gap, significant variations in collective observables, and increased work fluctuations link the critical slowing down of the adiabatic evolution with a quantum phase transition-like behavior of the system.
We propose a new physical approach for encoding and processing of quantum information in ensembles of multi-level quantum systems, where the different bits are not carried by individual particles but associated with the collective population of different internal levels. One- and two-bit gates are implemented by collective internal state transitions taking place in the presence of an excitation blockade mechanism which restricts the population of each internal state to the values zero and unity. 10-20 bit quantum computers can be built via this scheme in single trapped clouds of ground state a…
Controlling strongly interacting many-body systems enables the creation of tailored quantum matter, with properties transcending those based solely on single particle physics. Atomic ensembles which are optically driven to a Rydberg state provide many examples of this, such as atom-atom entanglement, many-body Rabi oscillations, strong photon-photon interaction and spatial pair correlations. In its most basic form, Rydberg quantum matter consists of an isolated ensemble of strongly interacting atoms spatially confined to the blockade volume - a so-called superatom. Here we demonstrate the cont…
In a previous letter we studied the giant optical nonlinearities of a Rydberg atomic medium within an optical cavity, in the Schwinger-Keldysh formalism. In particular, we calculated the non-linear contributions to the spectrum of the light transmitted through the cavity. In this article we spell out the essential details of this calculation, and we show how it can be extended to higher input photon numbers, and higher order correlation functions. As a relevant example, we calculate and discuss the three-photon correlation function of the transmitted light, and discuss its physical significanc…
Symmetric ensembles of neutral atoms interacting via the Rydberg blockade are well-described by the Jaynes-Cummings Hamiltonian. We use this framework to study the problem of generating arbitrary superpositions of Dicke states of hyperfine qubits in such ensembles. The combination of the symmetric Rydberg blockade and microwaves that drive the qubits with a time-dependent phase is sufficient to make these ensembles completely controllable, in the sense that one can generate an arbitrary unitary transformation on the system. We apply this to the problem of state mapping. With currently feasible…
We observe and measure dispersive optical non-linearities in an ensemble of cold Rydberg atoms placed inside an optical cavity. The experimental results are in agreement with a simple model where the optical non-linearities are due to the progressive appearance of a Rydberg blockaded volume within the medium. The measurements allow a direct estimation of the "blockaded fraction" of atoms within the atomic ensemble.
Coupling photons to Rydberg excitations in a cold atomic gas yields unprecedentedly large optical nonlinearities at the level of individual light quanta, where the formation of nearby dark-state polaritons is blocked by the strong interactions between Rydberg atoms. This blockade mechanism, however, realizes an inherently dissipative nonlinearity, which limits the performance of practical applications. In this work, we propose a new approach to strong photon interactions via a largely coherent mechanism at drastically suppressed photon losses. Rather than a polariton blockade, it is based on a…
We propose to use a collective excitation blockade mechanism to identify errors that occur due to disturbances of single atoms in ensemble quantum registers where qubits are stored in the collective population of different internal atomic states. A simple error correction procedure and a simple decoherence-free encoding of ensemble qubits in the hyperfine states of alkali atoms are presented.
We discuss the application of dipole blockade techniques for the preparation of single atom and single photon sources. A deterministic protocol is given for loading a single atom in an optical trap as well as ejecting a controlled number of atoms in a desired direction. A single photon source with an optically controlled beam-like emission pattern is described.
A scheme is proposed to prepare squeezed states and Schrödinger cat-like states of the collective spin degrees of freedom associated with a pair of ground states in an atomic ensemble. The scheme uses an effective Jaynes-Cummings interaction which can be provided by excitation of the atoms to Rydberg states and an effective J_x interaction implemented by a resonant Raman coupling between the atomic ground states. Both dynamical evolution with a constant Hamiltonian and with adiabatic variation of the two interaction terms are studied. We show that by the application of further resonant laser f…
We have numerically simulated quantum tomography of single-qubit and two-qubit quantum gates with qubits represented by mesoscopic ensembles containing random numbers of atoms. Such ensembles of strongly interacting atoms in the regime of Rydberg blockade are known as Rydberg superatoms. The Stimulated Raman Adiabatic Passage (STIRAP) in the regime of Rydberg blockade is used for deterministic Rydberg excitation in the ensemble, required for storage of quantum information in the collective state of the atomic ensemble and implementation of two-qubit gates. The optimized shapes of the STIRAP pu…
We use coherent excitation of 3-16 atom ensembles to demonstrate collective Rabi flopping mediated by Rydberg blockade. Using calibrated atom number measurements, we quantitatively confirm the expected $\sqrt{N}$ Rabi frequency enhancement to within 4%. The resulting atom number distributions are consistent with essentially perfect blockade. We then use collective Rabi $π$ pulses to produce ${\cal N}=1,2$ atom number Fock states with fidelities of 62% and 48% respectively. The ${\cal N}=2$ Fock state shows the collective Rabi frequency enhancement without corruption from atom number fluctuatio…
The dipole blockade effect at laser excitation of mesoscopic ensembles of Rydberg atoms lies in the fact that the excitation of one atom to a Rydberg state blocks the excitation of other atoms due to the shift in the collective energy levels of interacting Rydberg atoms. It is used to obtain the entangled qubit states based on single neutral atoms in optical traps. In this paper, we present our experimental results on the observation of the dipole blockade for mesoscopic ensembles of 1-5 atoms when they are detected by the selective field ionization method. We investigated the spectra of the t…
Strongly Rydberg-blockaded two-level atoms form a Rydberg superatom, which is excited only to a collective symmetrical Dicke state. However, emerging often in the alkali-earth atoms, the spontaneous decay from the Rydberg state to an additional pooling state renders the ensemble no longer a closed superatom. Herein we present a computationally-efficient model to characterize the interaction between a fully Rydberg-blockaded ensemble of $N$ $Λ$-type three-level atoms and a strong probe light field in a coherent state. The model enables us to achieve a decomposition of the coupled dynamics in th…
We study the interaction of two photons in a Rydberg atomic ensemble under the condition of electromagnetically induced transparency, combining a semi-classical approach for pulse propagation and a complete quantum treatment for quantum state evolution. We find that the blockade regime is not suitable for implementing photon-photon cross-phase modulation due to pulse absorption and dispersion. However, approximately ideal cross-phase modulation can be realized based on relatively weak interactions, with counter-propagating and transversely separated pulses.
We discuss methods for coherently controlling mesoscopic atomic ensembles where the number of atoms varies randomly from one experimental run to the next. The proposed schemes are based on adiabatic passage and Rydberg blockade and can be used for implementation of a scalable quantum register formed by an array of randomly loaded optical dipole traps.
Neutral atom array serves as an ideal platform to study the quantum logic gates, where intense efforts have been devoted to improve the two-qubit gate fidelity. We report our recent findings in constructing a different type of two-qubit controlled-PHASE quantum gate protocol with neutral atoms enabled by Rydberg blockade, which aims at both robustness and high-fidelity. It relies upon modulated driving pulse with specially tailored smooth waveform to gain appropriate phase accumulations for quantum gates. The major features include finishing gate operation within a single pulse, not necessaril…
Interaction between Rydberg atoms can significantly modify Rydberg excitation dynamics. Under a resonant driving field the Rydberg-Rydberg interaction in high-lying states can induce shifts in the atomic resonance such that a secondary Rydberg excitation becomes unlikely leading to the Rydberg blockade effect. In a related effect, off-resonant coupling of light to Rydberg states of atoms contributes to the Rydberg anti-blockade effect where the Rydberg interaction creates a resonant condition that promotes a secondary excitation in a Rydberg atomic gas. Here, we study the light-matter interact…
We present a scheme for scalable quantum information processing (QIP) with atomic ensembles and flying photons. Using the Rydberg blockade, we encode the qubits in the collective atomic states, which could be manipulated fast and easily due to the enhanced interaction, in comparison to the single-atom case. We demonstrate that our proposed gating could be applied to generation of two-dimensional cluster states for measurement-based quantum computation. Moreover, the atomic ensembles also function as quantum repeaters useful for long distance quantum state transfer. We show the possibility of o…
We demonstrate that an ultracold many-body bosonic ensemble confined in an one-dimensional (1D) double well potential exhibits a population imbalance between the two wells at large timescales, when the depth of the wells are modulated by a time-dependent driving force. The specific form of the driving force is shown to break spatial parity and time-reversal symmetries, which leads to such an asymptotic population imbalance (API). The value of the API can be flexibly controlled by changing the phase of the driving force and the total number of particles. While the API is highly sensitive to the…
We present a theory of electromagnetically induced transparency in a cold ensemble of strongly interacting Rydberg atoms. Long-range interactions between the atoms constrain the medium to behave as a collection of superatoms, each comprising a blockade volume that can accommodate at most one Rydberg excitation. The propagation of a probe field is affected by its two-photon correlations within the blockade distance, which are strongly damped due to low saturation threshold of the superatoms. Our model is computationally very efficient and is in quantitative agreement with the results of recent …
The transparence of a laser-driven optical resonator containing an ensemble of cold atoms can have two distinct, robust states. Atoms in their initially prepared pure state blockade the transmission by detuning the cavity mode from the laser drive. The interacting system can, however, transition into an uncoupled state via a non-linear channel opening up in a critical run-away process toward a transparent bright phase. The experiment enables a time-resolved observation of the dynamical transmission blockade breakdown phase transition as well as quantification of enhanced fluctuations in the cr…
We study the atom-photon quantum interface with intracavity Rydberg-blocked atomic ensemble where the ground-Rydberg transition is realized by two-photon transition. Via theoretical analysis, we report our recent findings of the Jaynes-Cummings model on optical domain and robust atom-photon quantum gate enabled by this platform. The requirement on the implementation is mild which includes an optical cavity of moderately high finesse, typical alkali atoms such as Rb or Cs and the condition that cold atomic ensemble is well within the Rydberg blockade radius. The analysis focuses on the atomic e…
Hybrid matter-photon entanglement is the building block for quantum networks. It is very favorable if the entanglement can be prepared with a high probability. In this paper, we report the deterministic creation of entanglement between an atomic ensemble and a single photon by harnessing Rydberg blockade. We design a scheme that creates entanglement between a single photon's temporal modes and the Rydberg levels that host a collective excitation, using a process of cyclical retrieving and patching. The hybrid entanglement is tested via retrieving the atomic excitation as a second photon and pe…
The coherent control of mesoscopic ensembles of atoms and Rydberg atom blockade are the basis for proposed quantum devices such as integrable gates and single photon sources. So far, experimental progress has been limited to complex experimental setups that use ultracold atoms. Here, we show that coherence times of ~100ns are achievable with coherent Rydberg atom spectroscopy in um sized thermal vapor cells. We investigated states with principle quantum numbers between 30 and 50. Our results demonstrate that microcells with a size on the order of the blockade radius, ~2um, at temperatures of 1…
We propose an efficient quantum repeater architecture with mesoscopic atomic ensembles, where the Rydberg blockade is employed for deterministic local entanglement generation, entanglement swapping and entanglement purification. Compared with conventional atomic-ensemble-based quantum repeater, the entanglement distribution rate is improved by up to two orders of magnitude with the help of the deterministic Rydberg gate. This new quantum repeater scheme is robust and fast, and thus opens up a new way for practical long-distance quantum communication.
We propose a scheme for preparing an ensemble of atoms in a maximally entangled W state by exploiting the Rydberg blockade effect. The success of our protocol is indicated by the detection of an ion, which thus serves as a herald for successful entangled state preparation. The fidelity of the preparation scheme is independent of the number of atoms in the ensemble. Therefore, a small cloud of atoms in a dipole trap randomly loaded from a background gas can be reliably prepared in a maximally entangled state despite of atom number fluctuations.
We demonstrate deterministic generation of two distinct collective excitations in one atomic ensemble, and we realize the Hong-Ou-Mandel interference between them. Using Rydberg blockade we create single collective excitations in two different Zeeman levels, and we use stimulated Raman transitions to perform a beam-splitter operation between the excited atomic modes. By converting the atomic excitations into photons, the two-excitation interference is measured by photon coincidence detection with a visibility of 0.89(6). The Hong-Ou-Mandel interference witnesses an entangled NOON state of the …
We propose to use adiabatic rapid passage with a chirped laser pulse in the strong dipole blockade regime to deterministically excite only one Rydberg atom from randomly loaded optical dipole traps or optical lattices. The chirped laser excitation is shown to be insensitive to the random number \textit{N} of the atoms in the traps. Our method overcomes the problem of the $\sqrt {N} $ dependence of the collective Rabi frequency, which was the main obstacle for deterministic single-atom excitation in the ensembles with unknown \textit{N}, and can be applied for single-atom loading of dipole trap…
We study the quantum statistical properties of the collective excitations of an atomic ensemble inside a high-finesse cavity. In the large-detuning regime, it is found that the virtual photon exchange can induce a long-range interaction between atoms, which results in correlated excitations. In particular, the atomic blockade phenomenon occurs when the induced long-range interaction effectively suppresses the double atomic excitation, when the average photon number takes certain values, which makes the two nearest energy levels degenerate. We also show that quantum phase transitions occur in t…
Entanglement between a single photon and a matter qubit is an indispensable resource for quantum repeater and quantum networks. With atomic ensembles, the entanglement creation probability is typically very low to inhibit high-order events. In this paper, we propose and experimentally realize a scheme which creates atom-photon entanglement with an intrinsic efficiency of 50%. We make use of Rydberg blockade to generate two collective excitations, lying in separate internal states. By introducing the momentum degree of freedom for the excitations, and interfering them via Raman coupling, we ent…
