We calculate the dispersive properties of the reflected field from a cavity coupled to a single dipole. We show that when a field is resonant with the dipole it experiences a 90 degree phase shift relative to reflection from a bare cavity if the Purcell factor exceeds the bare cavity reflectivity. We then show that optically Stark shifting the dipole with a second field can be used to achieve giant Kerr non-linearites. It is shown that currently achievable cavity lifetimes and cavity quality factors can allow a single emitter in the cavity to impose a nonlinear $π$ phase shift at the single photon level.
We observe and measure dispersive optical non-linearities in an ensemble of cold Rydberg atoms placed inside an optical cavity. The experimental results are in agreement with a simple model where the optical non-linearities are due to the progressive appearance of a Rydberg blockaded volume within the medium. The measurements allow a direct estimation of the "blockaded fraction" of atoms within the atomic ensemble.
We develop a fully quantum treatment of electromagnetically induced transparency (EIT) in a vapor of three-level $Λ$-type atoms. Both the probe and coupling lasers with arbitrary intensities are quantized, and treated on the same footing. In addition to reproducing known results on ultraslow pulse propagation at the lowest order in the ratio of their Rabi frequencies, our treatment uncovers that the atomic medium with EIT exhibits giant Kerr as well as higher order non-linearities. Enhancement of many orders of magnitude is predicted for higher-order refractive-index coefficients.
We show, that photon non-linearities in electromagnetically induced transparency can be at least one order of magnitude larger than predicted in all previous approaches. As an application we demonstrate that, in this regime they give rise to very strong photon - photon interactions which are strong enough to make an experimental realization of a photonic Mott insulator state feasible in arrays of coupled ultra high-Q micro-cavities.
We investigate experimentally the absorptive and dispersive properties of triple-resonant optical parametric amplifier OPA for the degenerate subharmonic field. In the experiment, the subharmonic field is utilized as the probe field and the harmonic wave as the pump field. We demonstrate that EIT-like effect can be simulated in the triple-resonant OPA when the cavity line-width for the harmonic wave is narrower than that for the subharmonic field. However, this phenomenon can not be observed in a double-resonant OPA. The narrow transparency window appears in the reflected field. Especially, in…
We demonstrate electromagnetically induced transparency (EIT) in a sample of rubidium atoms, trapped in an optical dipole trap. Mixing a small amount of $σ^-$-polarized light to the weak $σ^+$-polarized probe pulses, we are able to measure the absorptive and dispersive properties of the atomic medium at the same time. Features as small as 4 kHz have been detected on an absorption line with 20 MHz line width.
Interest in lossless nonlinearities has focussed on the the dispersive properties of $Λ$ systems under conditions of electromagnetically induced transparency (EIT). We generalize the lambda system by introducing further degenerate states to realize a `Chain $ Λ$' atom where multiple coupling of the probe field significantly enhances the intensity dependent dispersion without compromising the EIT condition.
We study the propagation of a weak probe field through an optomechanical system in which $N$ nearly degenerate mechanical membranes are inside a Febry-Perot cavity, and couple dispersively to an intracavity field. We derive a general analytical expression for the output probe field. We show that the in-phase quadrature of the output probe field can exhibit multiple electromagnetically induced transparency with at most $N$ narrow transparency windows. We find that the superluminal light can be achieved with at most $N$ different negative group velocities at the transparency windows. Moreover, b…
Superconducting cavities with high quality factors play an essential role in circuit quantum electrodynamics and quantum computing. In measurements of the the intrinsic loss rates of high frequency modes, it can be challenging to design an appropriate coupling to the measurement circuit in such a way that the resulting signal is sufficiently strong but also that this coupling does not lead to unwanted loading circuit, obscuring the intrinsic internal loss rates. Here, we propose and demonstrate a spectroscopic probe of high-Q resonators based on the phenomena of electromagnetically-induced tra…
We study optical bistable behavior of a Rydberg electromagnetically-induced transparency (EIT) atomic medium in a unidirectional optical ring-cavity. Due to strong van del Waal (vdW) interactions between the atoms, both optical nonlinear dispersion and nonlinear absorption coefficients are enhanced substantially. Under the condition of two-photon on resonance, we show that probe one-photon detuning can change the phase of the third order nonlinearity coefficient, which tunes the character of the optical bistability within different ratios of dispersive and absorptive types. This enables the si…
We propose a technique for quantum nondemolition (QND) measurement and heralded preparation of Fock states by dynamics of electromagnetically induced transparency (EIT). An atomic ensemble trapped in an optical cavity is driven by two external continuous-wave classical fields to form EIT in steady state. As soon as a weak coherent field is injected into the cavity, the EIT system departs from steady state, falls into transient state dynamics by the dispersive coupling between cavity injected photons and atoms. Because the imaginary part of time-dependent linear susceptibility Im[X(t)] of the a…
We study dispersive optical nonlinearities of short pulses propagating in high number density, warm atomic vapors where the laser resonantly excites atoms to Rydberg $P$-states via a single-photon transition. Three different regimes of the light-atom interaction, dominated by either Doppler broadening, Rydberg atom interactions, or decay due to thermal collisions between groundstate and Rydberg atoms, are described. We show that using fast Rabi flopping and strong Rydberg atom interactions, both in the order of gigahertz, can overcome the Doppler effect as well as collisional decay, leading to…
We demonstrate the non-dispersive deflection of an optical beam in a Stern-Gerlach magnetic field. An optical pulse is initially stored as a spin-wave coherence in thermal rubidium vapour. An inhomogeneous magnetic field imprints a phase gradient onto the spin wave, which upon reacceleration of the optical pulse leads to an angular deflection of the retrieved beam. We show that the obtained beam deflection is non-dispersive, i.e. its magnitude is independent of the incident optical frequency. Compared to a Stern-Gerlach experiment carried out with propagating light under the conditions of elec…
A three-level atomic medium can be made transparent to a resonant probe field in the presence of a strong control field acting on an adjacent atomic transition to a long-lived state, which can be represented by a highly excited Rydberg state. The long-range interactions between the Rydberg state atoms then translate into strong, non-local, dispersive or absorptive interactions between the probe photons, which can be used to achieve deterministic quantum logic gates and single photon sources. Here we show that long-range dipole-dipole exchange interaction with one or more spins -- two-level sys…
The implementation of electromagnetically induced transparency (EIT) in a cold Rydberg gas provides an attractive route towards strong photon--photon interactions and fully deterministic all-optical quantum information processing. In this brief review we discuss the underlying principles of how large single photon non-linearities are achieved in this system and describe experimental progress to date.
Hollow-core photonic-crystal waveguides filled with cold atoms can support giant optical nonlinearities through nondispersive propagation of light tightly confined in the transverse direction. Here we explore electromagnetically induced transparency is such structures, considering a pair of counter-propagating weak quantum fields in the medium of coherently driven atoms in the ladder configuration. Strong dipole--dipole interactions between optically excited, polarized Rydberg states of the atoms translate into a large dispersive interaction between the two fields. This can be used to attain a…
Faraday rotation of a laser field induced by a single atom is demonstrated by tightly focussing a linearly polarized laser beam onto a laser-cooled ion held in a harmonic Paul trap. The polarization rotation signal is further used to measure the phase-shift associated with electromagnetically-induced-transparency and to demonstrate read-out of the internal state on the qubit transition with a detection fidelity of 98 $\pm$ 1%. These results have direct implications for single atom magnetometery and dispersive read-out of atomic superpositions.
In this paper we study cavity optomechanical systems in which the position of a mechanical oscillator modulates both the resonance frequency (dispersive coupling) and the linewidth (dissipative coupling) of a cavity mode. Using a quantum noise approach we calculate the optical damping and the optically-induced frequency shift. We find that dissipatively coupled systems feature two parameter regions providing amplification and two parameter regions providing cooling. To investigate the strong-coupling regime, we solve the linearized equations of motion exactly and calculate the mechanical and o…
We show that an ensemble of organic dye molecules with permanent electric dipole moments embedded in a microcavity can lead to strong optical nonlinearities at the single photon level. The strong long-range electrostatic interaction between chromophores due to their permanent dipoles introduces the desired nonlinearity of the light-matter coupling in the microcavity. We obtain the absorption spectra of a weak probe field under the influence of strong exciton-photon coupling with the cavity field. Using realistic parameters, we demonstrate that a single cavity photon can significantly modify th…
We experimentally demonstrate the elementary case of electromagnetically induced transparency (EIT) with a single atom inside an optical cavity probed by a weak field. We observe the modification of the dispersive and absorptive properties of the atom by changing the frequency of a control light field. Moreover, a strong cooling effect has been observed at two-photon resonance, increasing the storage time of our atoms twenty-fold to about 16 seconds. Our result points towards all-optical switching with single photons.
The interaction of a five-level atomic system involving electromagnetically induced transparency with four light fields is investigated. Two different light-atom configurations are considered, and their efficiency in generating large nonlinear cross-phase shifts compared. The dispersive properties of those schemes are analyzed in detail, and the conditions leading to group velocity matching for two of the light fields identified. An analytical treatment based on amplitude equations is used in order to obtain approximate solutions for the susceptibilities, ehich are shown to fit well with the n…
The intention of this work is twofold, first to present a most simple system capable of simulating the intrinsic bosonic Josephson effect with photons, and second to study various outcomes deriving from inherent or external decoherence. A qubit induces an effective coupling between two externally pumped cavity modes. Without cavity losses and in the dispersive regime, intrinsic Josephson oscillations of photons between the two modes occurs. In this case, contrary to regular Markovian decoherence, the qubit purity shows a Gaussian decay and recurrence of its coherence. Due to intrinsic non-line…
