We report an investigation to establish the physical mechanisms responsible for decoherence in the generation of photon pairs from atomic ensembles, via the protocol of Duan et. al for long distance quantum communication [Nature (London) 414, 413 (2001)] and present the experimental techniques necessary to properly control the process. We develop a theory to model in detail the decoherence process in experiments with magneto-optical traps. The inhomogeneous broadening of the ground state by the trap magnetic field is identified as the principal mechanism for decoherence. In conjunction with our theoretical analysis, we report a series of measurements to characterize and control the coherence time in our experimental setup. We use copropagating stimulated Raman spectroscopy to access directly the ground state energy distribution of the ensemble. These spectroscopic measurements allow us to switch off the trap magnetic field in a controlled way, optimizing the repetition rate for single-photon measurements. With the magnetic field off, we then measure nonclassical correlations for pairs of photons generated by the ensemble as a function of the storage time of the single collective atomic excitation. We report coherence times longer than 10 microseconds, corresponding to an increase of two orders of magnitude compared to previous results in cold ensembles. The coherence time is now two orders of magnitude longer than the duration of the excitation pulses. The comparison between these experimental results and the theory shows good agreement. Finally, we employ our theory to devise ways to improve the experiment by optical pumping to specific initial states.
The symmetric collective states of an atomic spin ensemble (i.e., many-body states that are invariant under particle exchange) are not preserved by decoherence that acts identically but individually on members of the ensemble. We develop a class of collective states in an ensemble of N spin-1/2 particles that is invariant under symmetric local decoherence and find that the dimension of the Hilbert space spanned by these collective states scales only as N^2. We then investigate the open system dynamics of experimentally relevant non-classical collective atomic states, including Schroedinger cat…
We analyze seemingly contradictory claims in the literature about the role played by decoherence in ensuring classical behavior for the chaotically tumbling satellite Hyperion. We show that the controversy is resolved once the very different assumptions underlying these claims are recognized. In doing so, we emphasize the distinct notions of the problem of classicality in the ensemble interpretation of quantum mechanics and in decoherence-based approaches that are aimed at addressing the measurement problem.
We revisit the decoherence of the atomic state in the resonant Jaynes-Cummings model with the field initially being in a coherent state. We show that the purity of the atom exhibits oscillating Gaussian dependence on the time with a width independent of the initial atomic state. It is also shown that when the atom and the coherent state match each other in phase, the atomic decoherence is Gaussian time dependence.
Based on the recent experiments on the hybrid quantum system of a superconducting microwave cavity coupling strongly to an inhomogeneous broadening spin ensemble under an external driving field, we use the exact master equation approach to investigate its non-Markovian decoherence dynamics. Here the spin ensemble is made by negatively charged nitrogen-vacancy (NV) defects in diamond. Our exact master equation theory for open systems depicts the experimental decoherence results and reveals the mechanism how the decoherence induced by the inhomogeneous broadening is suppressed in the strong-coup…
We study the multipartite correlations of the multi-atom dark states, which are characterized by the atomic squeezing beyond the pairwise entanglement. It is shown that, in the photon storage process with atomic ensemble via electromagnetically induced transparency (EIT) mechanism, the atomic squeezing and the pairwise entanglement can be created by adiabatically manipulating the Rabi frequency of the classical light field on the atomic ensemble. We also consider the sudden death for the atomic squeezing and the pairwise entanglement under various decoherence channels. An optimal time for gene…
We study the effects of time uncertainty in the interaction of atoms with a standing light wave. We discuss its physical origin and the possibility to observe intrinsic decoherence effects by measuring the atomic momentum distribution.
It is discussed the decoherence problems in ensemble large-scale solid state NMR quantum computer based on the array of P donor atoms having nuclear spin I = 1/2. It is considered here, as main mechanisms of decoherence for low temperature (< 0.1 K), the adiabatic processes of random modulation of qubit resonance frequency determined by secular part of nuclear spin interaction with electron spin of the basic atoms, with impurity paramagnetic atoms and also with nuclear spins of impurity diamagnetic atoms. It was made estimations of allowed concentrations of magnetic impurities and of spin temp…
Large scale quantum information processing requires stable and long-lived quantum memories. Here, using atom-photon entanglement, we propose an experimentally feasible scheme to realize decoherence-free quantum memory with atomic ensembles, and show one of its applications, remote transfer of unknown quantum state, based on laser manipulation of atomic ensembles, photonic state operation through optical elements, and single-photon detection with moderate efficiency. The scheme, with inherent fault-tolerance to the practical noise and imperfections, allows one to retrieve the information in the…
We study the suppression of noise-induced phase decoherence in a single atomic qubit by employing pulse sequences. The atomic qubit is composed of a single neutral atom in a far-detuned optical dipole trap and the phase decoherence may originate from the laser intensity and beam pointing fluctuations as well as magnetic field fluctuations. We show that suitable pulse sequences may prolongate the qubit coherence time substantially as comparing to the conventional spin echo pulse.
We study theoretically the decoherence of a gas of bosonic atoms induced by the interaction with a largely detuned laser beam. It is shown that for a standing laser beam decoherence coincides with the single-particle result. For a running laser beam many-particle effects lead to significant modifications.
We present a quantum interference approach to preserve coherence in the external states of an atom trapped in an optical lattice. We show that this is possible by suitably choosing the initial state of the atom. We demonstrate this in context of decoherence due to spontaneous emission in an one-dimensional optical double-well lattice.
The ultimate stability of atomic clocks is limited by the quantum noise of the atoms. To reduce this noise it has been suggested to use entangled atomic ensembles with reduced atomic noise. Potentially this can push the stability all the way to the limit allowed by the Heisenberg uncertainty relation, which is denoted the Heisenberg limit. In practice, however, entangled states are often more prone to decoherence, which may prevent reaching this performance. Here we present an adaptive measurement protocol that in the presence of a realistic source of decoherence enables us to get near Heisenb…
We studied the dispersive dissipation of denegerate-level atom interacting with a single linearly-polarized mode field. It is found that the degeneracy of the atomic level affects the dissipation bahavior of the system as well as the subsystems. The degeneracy of the atomic level augment the periods of entanglement and increase the degree of the maxima statistical mixture states.
Hybrid quantum systems based on spin ensembles coupled to superconducting microwave cavities are promising candidates for robust experiments in cavity quantum electrodynamics (QED) and for future technologies employing quantum mechanical effects. Currently the main source of decoherence in these systems is inho- mogeneous spin broadening, which limits their performance for the coherent transfer and storage of quantum information. Here we study the dynamics of a superconducting cavity strongly coupled to an ensemble of nitrogen-vacancy centers in diamond. We experimentally observe for the first…
To resist decoherence from destroying the phase factor of qubit state, it is important to use decoherence-free states for processing, transmitting and storing quantum information in quantum computing and quantum communication. We propose a practical scheme using four atoms with decoherence-free states in a single-mode cavity to realize the entanglement and fundamental quantum logic gates. The transmission of quantum information can be made directly from one atom to another, in which the cavity is only virtually excited. The possible application and the experimental requirement of our proposal …
This dissertation studies spin squeezing, entanglement and decoherence in large ensembles of cold, trapped alkali atoms with hyperfine spin f interacting with optical fields. Restricting the state of each atom to a qutrit embedded in the 2f+1 dimensional hyperfine spin enables us to efficiently model the coherent and dissipative dynamics of the ensemble. This formalism also allows us to explore the effects of local control on the internal hyperfine spins of the atoms. State preparation using such control increases the entangling power of the atom-light interface for f>1/2. Subsequent control o…
Heralded entanglement between collective excitations in two atomic ensembles is probabilistically generated, stored, and converted to single photon fields. By way of the concurrence, quantitative characterizations are reported for the scaling behavior of entanglement with excitation probability and for the temporal dynamics of various correlations resulting in the decay of entanglement. A lower bound of the concurrence for the collective atomic state of 0.9\pm 0.3 is inferred. The decay of entanglement as a function of storage time is also observed, and related to the local dynamics.
A theoretical model describing the Raman scattering process in atomic vapors is constructed. The treatment investigates the low-excitation regime suitable for modern experimental applications. Despite the incorporated decoherence effects (possibly mode dependent) it allows for a direct separation of the time evolution from the spatial degrees of freedom. The impact of noise on the temporal properties of the process is examined. The model is applied in two experimentally relevant situations of ultra-cold and room-temperature atoms. The spatial eigenmodes of the Stokes photons and their coupling…
We report characterization of electromagnetically induced transparency (EIT) resonances in the D1 line of Rb-87 under various experimental conditions. The dependence of the EIT linewidth on the power of the pump field was investigated, at various temperatures, for the ground states of the lambda-system associated with different hyperfine levels of the atomic 5S_1/2 state as well as magnetic sublevels of the same hyperfine level. Strictly linear behavior was observed in all cases. A theoretical analysis of our results shows that dephasing in the ground state is the main source of decoherence, w…
In this paper, by exploiting the weak measurement and quantum measurement re- versal (WMQMR) procedure, we propose a scheme to show how one can protect the geometric quantum discord (GQD) of a two-qutrit V-type atomic system each of which interacts with a dissipative reservoir independently. We examine the scheme for the GQD of the initial two-qutrit Werner and Horodecki states for different classes of weak mea- surement strengthes. It is found out that the presented protocol enables us to suppress decoherence due to the amplitude damping (AD) channel and preserve the quantum dis- cord of the …
We consider the STIRAP process in a three-level atom. Viewed as a closed system, no geometric phase is acquired. But in the presence of spontaneous emission and/or collisional relaxation we show numerically that a non-vanishing, purely real, geometric phase is acquired during STIRAP, whose magnitude grows with the decay rates. Rather than viewing this decoherence-induced geometric phase as a nuisance, it can be considered an example of "beneficial decoherence": the environment provides a mechanism for the generation of geometric phases which would otherwise require an extra experimental contro…
In most proposals for the generation of entanglement in large ensembles of atoms via projective measurements, the interaction with the vacuum is responsible for both the generation of the signal that is detected and the spin depolarization or decoherence. In consequence, one has to usually work in a regime where the information aquisition via detection is sufficiently slow (weak measurement regime) such as not to strongly disturb the system. We propose here a four-wave mixing scheme where, owing to the pumping of the atomic system into a dark state, the polarization of the ensemble is not crit…
We study the dynamics of a quantum spin ensemble controlled by trains of ultrashort pulses. To model disturbances of the kicks, we consider that the spins are submitted to different kick trains which follow regular, random, stochastic or chaotic dynamical processes. These are described by dynamical systems on a torus. We study the quantum decoherence and the population relaxation of the spin ensemble induced by these classical dynamical processes disturbing the kick trains. For chaotic kick trains we show that the decoherence and the relaxation processes exhibit a signature of chaos directly r…
It is shown how possible corrections to ordinary quantum mechanics described by the Lindblad equation might be detected by exploiting the great precision of atomic clocks.
We investigate the decoherence of a superposition of symmetric collective internal states of an atomic ensemble due to inhomogeneous coupling to external control fields. For asymptotically large system, we find the characteristic decoherence rate scales as $\sqrt{N}$ with $N$ being the total number of atoms. Our results shed new light on attempts for quantum information processing and storage with atomic ensembles.
It is commonly known that the dephasing in open quantum systems is due to the establishment of bipartite correlations with ambient environments, which are typically difficult to be fully characterized. Recently, a new approach of average over disordered Hamiltonian ensemble is developed and shown to be capable of describing the nonclassicality of incoherent dynamics based on inferring the nonclassical nature of the correlations. Here we further extend the approach of Hamiltonian ensemble in the canonical form to the realm of structural disorder. Under the variable separation of the probability…
We solve the time-dependent Schrodinger equation for the combination of a spin system interacting with a spin bath environment. In particular, we focus on the time development of the reduced density matrix of the spin system. Under normal circumstances we show that the environment drives the reduced density matrix to a fully decoherent state, and furthermore the diagonal elements of the reduced density matrix approach those expected for the system in the canonical ensemble. We show one exception to the normal case is if the spin system cannot exchange energy with the spin bath. Our demonstrati…
Violations of a Bell inequality are reported for an experiment where one of two entangled qubits is stored in a collective atomic memory for a user-defined time delay. The atomic qubit is found to preserve the violation of a Bell inequality for storage times up to 21 microseconds, 700 times longer than the duration of the excitation pulse that creates the entanglement. To address the question of the security of entanglement-based cryptography implemented with this system, an investigation of the Bell violation as a function of the cross-correlation between the generated nonclassical fields is …
We present a fully analytical solution of the dynamics of two strongly-driven atoms resonantly coupled to a dissipative cavity field mode. We show that an initial atom-atom entanglement cannot be increased. In fact, the atomic Hilbert space divides into two subspaces, one of which is decoherence free so that the initial atomic entanglement remains available for applications, even in presence of a low enough atomic decay rate. In the other subspace a measure of entanglement, decoherence, and also purity, are described by a similar functional behavior that can be monitored by joint atomic measur…
We analyze the time evolution of an initial spatial coherence for a two level atom whose internal degrees of freedom interact with a single mode of a cavity field. When the qubit-field subsystem is taken as an environment, the translational dynamics experiences a decoherence process which may be encoded in a decoherence factor D. We find that the field statistics affects D through the alternative paths the system-environment may follow along their entanglement, while eventual field phase properties give rise to an imaginary part of D which is related to the atomic translation. From the decoher…
We derive a model to describe decoherence of atomic clouds in atom-chip traps taking the excited states of the trapping potential into account. We use this model to investigate decoherence for a single trapping well and for a pair of trapping wells that form the two arms of an atom interferometer. Including the discrete spectrum of the trapping potential gives rise to a decoherence mechanism with a decoherence rate $Γ$ that scales like $Γ\sim 1/r_0^4$ with the distance $r_0$ from the trap minimum to the wire.
Optical lattice clocks can now resolve the height difference below 1 mm within an atomic ensemble by means of gravitational redshift with integration over sufficient amount of time. Further improvement in the stability enables the clocks to resolve the height difference of subsystems within an atomic ensemble that is conventionally interrogated as a single coherent spin state in a single Ramsey sequence, resulting in the dephasing of the coherent spin state. This effect is observable with a clock of a stability of $\lesssim 10^{-21}$ by introducing a single-layer-resolved imaging system for a …
We derive scaling laws for the spin decoherence of neutral atoms trapped near conducting and superconducting plane surfaces. A new result for thin films sheds light on the measurement of Y.J. Lin, I. Teper, C. Chin, and V. Vuletić [Phys. Rev. Lett. \textbf{92}, 050404 (2004)]. Our calculation is based on a quantum-theoretical treatment of electromagnetic radiation near metallic bodies [P.K. Rekdal, S. Scheel, P.L. Knight, and E.A. Hinds, Phys. Rev. A \textbf{70}, 013811 (2004)]. We show that there is a critical atom-surface distance that maximizes the spin relaxation rate and we show how this …
We consider an ensemble of atoms with $Λ$-type level structure trapped in a single-mode cavity, and propose a geometric scheme of coherent manipulation of quantum states on the subspace of zero-energy states within the quantum Zeno subspace of the system. We find that the particular subspace inherits the decoherence-free nature of the quantum Zeno subspace and features a symmetry-protected degeneracy, fulfilling all the conditions for a universal scheme of arbitrary unitary operations on it.
We solve the dynamics of an open quantum system where N strongly driven two-level atoms are equally coupled on resonance to a dissipative cavity mode. Analytical results are derived on decoherence, entanglement, purity, atomic correlations and cavity field mean photon number. We predict decoherence-free subspaces for the whole system and the N-qubit subsystem, the monitoring of quantum coherence and purity decay by atomic populations measurements, the conditional generation of atomic multi-partite entangled states and of cavity cat-like states. We show that the dynamics of atoms prepared in st…
We provide an intuitive interpretation of the optical Stern-Gerlach effect (OSGE) in the dressed-state point of view. We also analyze the effect of atomic damping in an experiment on the OSGE. We show that the atomic damping also causes the wave packet splitting, in a non-mechanical fashion, as opposed to the coherent process that is mechanical.
We consider a class of states in an ensemble of two-level atoms: a superposition of two distinct atomic coherent states, which can be regarded as atomic analogues of the states usually called Schrodinger cat states in quantum optics. According to the relation of the constituents we define polar and nonpolar cat states. The properties of these are investigated by the aid of the spherical Wigner function. We show that nonpolar cat states generally exhibit squeezing, the measure of which depends on the separation of the components of the cat, and also on the number of the constituent atoms. By so…
Two-photon processes that involve different sub-levels of the ground state of an atom, are highly sensitive to depopulation and decoherence within the ground state. For example, the spectral width of electromagnetically induced transparency resonances in $Λ-$type system, are strongly affected by the ground state depopulation and decoherence rates. We present a direct measurement of decay rates between hyperfine and Zeeman sub-levels in the ground state of $^{87}$Rb vapor. Similar to the relaxation-in-the-dark technique, pumping lasers are used to pre-align the atomic vapor in a well defined qu…
We present a method for performing quantum state reconstruction on qubits and qubit registers in the presence of decoherence and inhomogeneous broadening. The method assumes only rudimentary single qubit rotations as well as knowledge of decoherence and loss mechanisms. We show that full state reconstruction is possible even in the case where single qubit rotations may only be performed imperfectly. Furthermore we show that for ensemble quantum computing proposals, quantum state reconstruction is possible even if the ensemble experiences inhomogeneous broadening and if only imperfect qubit man…
We present a first-principles derivation of spatial atomic-sublevel decoherence near dielectric and metallic surfaces. The theory is based on the electromagnetic-field quantization in absorbing dielectric media. We derive an expression for the time-variation of the off-diagonal matrix element of the atomic density matrix for arbitrarily shaped substrates. For planar multilayered substrates we find that for small lateral separations of the atom's possible positions the spatial coherence decreases quadratically with the separation and inversely to the squared atom-surface distance.
Pair collisions in atomic gases lead to decoherence and decay. Assuming that all the atoms in the gas are equally likely to collide one is led to consider Lindbladian of mean field type where the evolution in the limit of many atoms reduces to a single qudit Lindbladian with quadratic non-linearity. We describe three smoking guns for non-linear evolutions: Power law decay and dephasing rates; Dephasing rates that take a continuous range of values depending on the initial data and finally, anomalous flow of the Bloch ball towards a hemisphere.
As an ensemble scheme of solid-state NMR quantum computers the extension of Kane's many-qubits silicon scheme based on the array of 31 P donor atoms are spaced lengthwise of the strip gates is considered. The possible planar topology of such ensemble quantum computer is suggested. The estimation of the output NMR signal was performed and it was shown that for the number N>=10^5 of ensemble elements involving L~10^3 qubits each, the standard NMR methods are usable. As main mechanisms of decoherence for low temperature (<0.1K), the adiabatic processes of random modulation of qubit resonance freq…
We develop a theory to analyze the decoherence effect in a charged qubit array system with photon echo signals in the multiwave mixing configuration. We present how the decoherence suppression effect by the {\it bang-bang} control with the $π$ pulses can be demonstrated in laboratory by using a bulk ensemble of exciton qubits and optical pulses whose pulse area is even smaller than $π$. Analysis is made on the time-integated multiwave mixing signals diffracted into certain phase matching directions from a bulk ensemble. Depending on the pulse interval conditions, the cross over from the decohe…
We consider four two-level atoms interacting with independent non-Markovian reservoirs with detuning. We mainly investigate the effects of the detuning and the length of the reservoir correlation time on the decoherence dynamics of the multipartite entanglement. We find that the time evolution of the entanglement of atomic and reservoir subsystems is determined by a parameter, which is a function of the detuning and the reservoir correlation time. We also find that the decay and revival of the entanglement of the atomic and reservoir subsystems are closely related to the sign of the decay rate…
We study dynamics of nonclassical correlations by exactly solving a model consisting of two atomic qubits with spontaneous emission. We find that the nonclassical correlations defined by different measures give different qualitative characterizations of those correlations. The relative behaviors of those correlation measures are presented explicitly for various quantum states in the two-qubit atomic system. In particular, we find that the robustness of quantum correlations can be greatly enhanced by performing appropriate local unitary operations on the initial state of the system.
Decoherence of a center spin or qubit in a spin bath is essentially determined by the many-body bath evolution. The bath dynamics can start either from a pure state or, more generally, from a statistical ensemble. In the preceding article [W. Yang and R. B. Liu, Phys. Rev. B \textbf{78}, 085315 (2008)], we have developed the cluster-correlation expansion (CCE) theory for the so-called single-sample bath dynamics initiated from a factorizable pure state. Here we present the ensemble CCE theory, which is based on similar ideas of the single-sample CCE: The bath evolution is factorized into the p…
We propose a protocol to achieve high fidelity quantum state teleportation of a macroscopic atomic ensemble using a pair of quantum-correlated atomic ensembles. We show how to prepare this pair of ensembles using quasiperfect quantum state transfer processes between light and atoms. Our protocol relies on optical joint measurements of the atomic ensemble states and magnetic feedback reconstruction.
We study the decoherence of atomic interferometers due to the scattering of stochastic gravitational waves. We evaluate the `direct' gravitational effect registered by the phase of the matter waves as well as the `indirect' effect registered by the light waves used as beam-splitters and mirrors for the matter waves. Considering as an example the space project HYPER, we show that both effects are negligible for the presently studied interferometers.
We present a combined theoretical and experimental study of solid-state spin decoherence in an electronic spin bath, focusing specifically on ensembles of nitrogen vacancy (NV) color centers in diamond and the associated substitutional nitrogen spin bath. We perform measurements of NV spin free induction decay times $T_2^*$ and spin-echo coherence times $T_2$ in 25 diamond samples with nitrogen concentrations [N] ranging from 0.01 to 300\,ppm. We introduce a microscopic model and perform numerical simulations to quantitatively explain the degradation of both $T_2^*$ and $T_2$ over four orders …
Atomic clocks are typically operated by locking a local oscillator (LO) to a single atomic ensemble. In this article we propose a scheme where the LO is locked to several atomic ensembles instead of one. This results in an exponential improvement compared to the conventional method and provides a stability of the clock scaling as $(αN)^{-m/2}$ with $N$ being the number of atoms in each of the $m$ ensembles and $α$ is a constant depending on the protocol being used to lock the LO
Random matrix theory is used to represent generic loss of coherence of a fixed central system coupled to a quantum-chaotic environment, represented by a random matrix ensemble, via random interactions. We study the average density matrix arising from the ensemble induced, in contrast to previous studies where the average values of purity, concurrence, and entropy were considered; we further discuss when one or the other approach is relevant. The two approaches agree in the limit of large environments. Analytic results for the average density matrix and its purity are presented in linear respon…
To establish an applicable system for advanced quantum information processing between light and atoms, we have demonstrated the quantum non-demolition (QND) measurement with a collective spin of cold ytterbium atoms (171Yb), and observed 1.8 (-1.5, +2.4) dB spin squeezing. Since a 171Yb atom has only a nuclear spin of 1/2 in the ground state, the system is the simplest spin ensemble and robust against decoherence. We used very short pulses with the width of 100 ns, so the interaction time became much shorter than the decoherence time, which is important for multi-step quantum information proce…
We employ a continuous dynamical decoupling scheme to suppress the decoherence induced by elastic collisions of cold atoms. Using a continuous echo pulse we achieve a thirty-fold increase in the coherence time of Rb87 atoms trapped in a dipole trap. Coherence times of more than 100ms are demonstrated for an ensemble with an optical depth of 120.
The Lindblad approach to continuous quantum measurements is applied to a system composed of a two-level atom interacting with a stationary quantized electromagnetic field through a dispersive coupling fulfilling quantum nondemolition criteria. Two schemes of measurements are examined. The first one consists in measuring the atomic electric dipole, which indirectly allows one to infer the photon distribution inside the cavity. The second one schematizes a measurement of photon momentum, which permits to describe the atomic level distribution. Decoherence of the corresponding reduced density mat…
A new heuristic model of interaction of an atomic system with a gravitational wave is proposed. In it, the gravitational wave alters the local electromagnetic field of the atomic nucleus, as perceived by the electron, which changes the energy of the system. The spectral decomposition of the wave function is calculated, from which the energy of the system can be obtained. The results suggest a shift in the energy difference of the atomic energy levels, which will induce a small detuning to any given resonant transition. The detuning increases with the quantum numbers of the levels, making the e…
