Giovanna Morigi, Juergen Eschner, Stefano Mancini, David Vitali
备注：
4 pages, 3 figures, revised version (new scheme for generation of subsequent pairs of entangled pulses included). Accepted for publication in Phys. Rev. Lett
The coherent interaction between a laser-driven single trapped atom and an optical high-finesse resonator allows to produce entangled multi-photon light pulses on demand. The mechanism is based on the mechanical effect of light. The degree of entanglement can be controlled through the parameters of the laser excitation. Experimental realization of the scheme is within reach of current technology. A variation of the technique allows for controlled generation of entangled subsequent pulses, with the atomic motion serving as intermediate memory of the quantum state.
Photon pairs, highly entangled in polarization have been generated under femtosecond laser pulse excitation by a type I crystal source, operating in a single arm interferometric scheme. The relevant effects of temporal walk-off existing in these conditions between the ordinary and extraordinary photons were experimentally investigated. By introducing a suitable temporal compensation between the two orthogonal polarization components highly entangled pulsed states were obtained.
We experimentally investigate a double-pass parametric down-conversion scheme for producing pulsed, polarization-entangled photon pairs with high visibility. The amplitudes for creating photon pairs on each pass interfere to compensate for distinguishing characteristics that normally degrade two-photon visibility. The result is a high-flux source of polarization-entangled photon pulses that does not require spectral filtering. We observe quantum interference visibility of over 95% without the use of spectral filters for 200 femtosecond pulses, and up to 98.1% with 5 nm bandwidth filters.
We experimentally demonstrate polarization entanglement for squeezed vacuum pulses containing more than 10^5 photons. We also study photon-number entanglement by calculating the Schmidt number and measuring its operational counterpart. Theoretically, our pulses are the more entangled the brighter they are. This promises important applications in quantum technologies, especially photonic quantum gates and quantum memories.
We propose a scheme to perform basic gates of quantum computing and prepare entangled states in a system with cold trapped ions located in a single mode optical cavity. General quantum computing can be made with both motional state of the trapped ion and cavity state being qubits. We can also generate different kinds of entangled states in such a system without state reduction, and can transfer quantum states from the ion in one trap to the ion in another trap. Experimental requirement for achieving our scheme is discussed.
The generation of ultrafast laser pulses and the reconstruction of their electric fields is essential for many applications in modern optics. Quantum optical fields can also be generated on ultrafast time scales, however, the tools and methods available for strong laser pulses are not appropriate for measuring the properties of weak, possibly entangled pulses. Here, we demonstrate a method to reconstruct the joint-spectral amplitude of a two-photon energy-time entangled state from joint measurements of the frequencies and arrival times of the photons, and the correlations between them. Our rec…
We describe a simple and efficient setup to generate and characterize femtosecond quadrature-entangled pulses. Quantum correlations equivalent to about 2.5 dB squeezing are efficiently and easily reached using the non-degenerate parametric amplification of femtosecond pulses through a single-pass in a thin (0.1 mm) potassium niobate crystal. The entangled pulses are then individually sampled to characterize the non-separability and the entropy of formation of the states. The complete experiment is analysed in the time-domain, from the pulsed source of quadrature entanglement to the time-resolv…
The modification of initially entangled light pulses passing through dispersive and absorbing four-port devices is studied, using recently obtained results on quantum state transformations [Phys. Rev. A 59, 4716 (1999)]. The fidelity and indices of quantum correlations based on the von Neumann entropy are calculated. Their dependence on both the pulse shape and the four-port device parameters is studied. It is shown, that due to dispersion and absorption the quantum correlations are reduced substantially for large initial entanglement.
We report the generation of polarization-entangled photons by femtosecond-pulse-pumped spontaneous parametric down-conversion in a cascade of two type-I crystals. Highly entangled pulsed states were obtained by introducing a temporal delay between the two orthogonal polarization components of the pump field. They exhibited high-visibility quantum interference and a large concurrence value, without the need of post-selection using narrow-bandwidth-spectral filters. The results are well explained by the theory which incorporates the space-time dependence of interfering two-photon amplitudes if d…
The Stokes and anti-Stokes components of the spectrum of resonance fluorescence of a single trapped atom, which originate from the mechanical coupling between the scattered photons and the quantized motion of the atomic center of mass, exhibit quantum correlations which are of two-mode-squeezing type. We study and demonstrate the build-up of such correlations in a specific setup, which is experimentally accessible, and where the atom acts as efficient and continuous source of EPR-entangled, two-mode squeezed light.
The controlled interaction between a single, trapped, laser-driven atom and the mode of a high-finesse optical cavity allows for the generation of temporally separated, entangled light pulses. Entanglement between the photon-number fluctuations of the pulses is created and mediated via the atomic center-of-mass motion, which is interfaced with light through the mechanical effect of atom-photon interaction. By means of a quantum noise analysis we determine the correlation matrix which characterizes the entanglement, as a function of the system parameters. The scheme is feasible in experimentall…
We show that a single, trapped, laser-driven atom in a high-finesse optical cavity allows for the quantum-coherent generation of entangled light pulses on demand. Schemes for generating simultaneous and temporally separated pulse pairs are proposed. The mechanical effect of the laser excitation on the quantum motion of the cold trapped atom mediates the entangling interaction between two cavity modes and between the two subsequent pulses, respectively. The entanglement is of EPR-type, and its degree can be controlled through external parameters. At the end of the generation process the atom is…
The entanglement of different classes of initially entangled qubit pair is investigated in the presence of short laser pulses of rectangular and exponential shapes with either one or both qubits are excited. For the rectangular pulse, the detuning parameter protects the entanglement from degradation and controls its upper and lower bounds. We show that the upper bounds of entanglement decrease if both particles are excited, but the lower bounds are much better if only one particle is excited. The phenomena of entanglement degradation, sudden- death and -birth are shown for small initial time. …
We present a theoretical treatment of electromagnetically induced transparency and light storage using standing wave coupling fields in a medium comprised of stationary atoms, such as an ultra cold atomic gas or a solid state medium. We show that it is possible to create stationary pulses of light which have a qualitatively different behavior than in the case of a thermal gas medium, offering greater potential for quantum information processing applications.
We present a detailed analysis of the multimode quantum state embedded in an optical frequency comb generated by a Synchronously Pumped Optical Parametric Oscillator (SPOPO). The full covariance matrix of the state is obtained with homodyne detection where the local oscillator is spectrally controlled with pulse shaping techniques. The resulting matrix reveals genuine multipartite entanglement. Additionally, the beam is comprised of several independent eigenmodes that correspond to specific pulse shapes. The experimental data is confirmed with numerical simulations. Finally, the potential to c…
Within the matrix product state framework, we study the non-Markovian feedback dynamics of a two-level system interacting with the electromagnetic field inside a semi-infinite waveguide where the excitation of an atom-photon bound state is possible. Taking the steady-state excitation of the emitter as a figure of merit, we compare the trapped excitation for an initially excited quantum emitter and an emitter prepared via quantized pulses containing up to four photons. In the latter case, we find that for large feedback delay times, multi-photon pulses can yield a significantly higher steady-st…
We theoretically investigate the spectral entanglement of a multiphoton source generated from the cascade emissions in the cascaded cold atomic ensembles.\ This photon source is highly directional, guaranteed under the four-wave mixing condition, and is also highly frequency-correlated due to finite driving pulse durations and superradiant decay constants.\ We utilize Schmidt decomposition to study the bipartite entanglement of the biphoton states projected from the multiphoton ones.\ This entropy of entanglement can be manipulated by controlling the driving parameters and superradiant decay r…
The quantum state of the photon pair generated from type-II spontaneous parametric down-conversion pumped by a ultrafast laser pulse exhibits strong decoherence in its polarization entanglement, an effect which can be attributed to the clock effect of the pump pulse or, equivalently, to distinguishing spectral information in the two-photon state. Here, we propose novel temporal and spectral engineering techniques to eliminate these detrimental decoherence effects. The temporal engineering of the two-photon wavefunction results in a universal Bell-state synthesizer that is independent of the ch…
We theoretically investigate the quantum interference of entangled two-photon states generated in a nonlinear crystal pumped by femtosecond optical pulses. Interference patterns generated by the polarization analog of the Hong-Ou-Mandel interferometer are studied. Attention is devoted to the effects of the pump-pulse profile (pulse duration and chirp) and the second-order dispersion in both the nonlinear crystal and the interferometer's optical elements. Dispersion causes the interference pattern to have an asymmetric shape. Dispersion cancellation occurs in some cases.
Einstein-Podolsky-Rosen (EPR) entanglement introduced in 1935 deals with two particles that are entangled in their positions and momenta. Here we report the first experimental demonstration of EPR position-momentum entanglement of narrowband photon pairs generated from cold atoms. By using two-photon quantum ghost imaging and ghost interference, we demonstrate explicitly that the narrowband photon pairs violate the separability criterion, confirming EPR entanglement. We further demonstrate continuous variable EPR steering for positions and momenta of the two photons. Our new source of EPR-enta…
Quantum metrology with entangled states in realistic noisy environments always suffers from decoherence. Therefore, the measurement precision is greatly reduced. Here we applied the dynamical decoupling method to protect the $N$-qubit quantum metrology protocol and successfully revived the scaling of the measurement precision as ${N^{-k}}$ with $k\in \left[{5/6,11/12}\right]$. The degree of the precision revival, as determined by the noise spectrum distribution, indicates that the performance of the protected protocol can be further improved by controlling the noise spectrum. Such a protected …
Time-bin entangled single-photons are highly demanded for long distance quantum communication. We propose a heralded source of tunable narrowband single photons entangled in well-separated multiple temporal modes (time bins) with controllable amplitudes. The detection of a single Stokes photon generated in a cold atomic ensemble via Raman scattering of a weak write pulse heralds the preparation of one spin excitation stored within the atomic medium. A train of read laser pulses deterministically converts the atomic excitation into a single anti-Stokes photon delocalized in multi-time-bins. The…
A quantum gravity-gradiometer consists of two spatially separated ensembles of atoms interrogated by pulses of a common laser beam. Laser pulses cause the probability amplitudes of atomic ground-state hyperfine levels to interfere, producing two motion-sensitive phase shifts which allow the measurement of the average acceleration of each ensemble, and, via simple differencing, of the acceleration gradient. Here I propose entangling the quantum states of the two ensembles prior to the pulse sequence, and show that entanglement encodes their relative acceleration in a single interference phase w…
We investigate theoretically the slow group velocity of a pulse probe laser propagating through a cold sample and interacting with atoms in a three-level $Λ$ configuration having losses towards external states. The EIT phenomenon produces very small group velocities for the probe pulse in presence of a strong coupling field even in presence of the population losses, as in an open three-level system. The group velocity and the transmission of the pulses are examined numerically as functions of several parameters, the adiabatic transfer, the loss rate, the modification of the atomic velocity pro…
We study the formation of an entangled state in a one-dimensional chain of three nuclear spins system which interact weakly through the Ising type of interaction and taking into account first and second neighbor interactions. We can get this entangled state using two pulses ($π/2$ and $π$ pulses), and we study the efficiency of getting this entangled state as a function of the ratio of the second neighbor interaction coupling constant to the first neighbor interaction coupling constant ($J'/J$). We found that for $J'/J\ge 0.04$, the entangled state is well defined.
A novel method for preparation of a single photon in temporally-delocalized entangled modes is proposed and analyzed. We show that two single-photon pulses propagating in a driven nonabsorbing medium with different group velocities are temporally split under parametric interaction into well-separated pulses. In consequence, the single-photon "time-bin-entangled" states are generated with a programmable entanglement easily controlled by driving field intensity. The experimental study of nonclassical features and nonlocality of generated states by means of balanced homodyne tomography is discuss…
When a single emitter is excited by two phase-coherent pulses with a time delay, each of the pulses can lead to the emission of a photon pair, thus creating a ``time-bin entangled'' state. Double pair emission can be avoided by initially preparing the emitter in a metastable state. We show how photons from separate emissions can be made indistinguishable, permitting their use for multi-photon interference. Possible realizations are discussed. The method might also allow the direct creation of n-photon entangled states (n>2).
We suggest an operating scheme for the deliberate generation of spin-entangled electron pairs in a normal-metal mesoscopic structure with fork geometry. Voltage pulses with associated Faraday flux equal to one flux unit $Φ_0=hc/e$ drive individual singlet-pairs of electrons towards the beam splitter. The spin-entangled pair is created through a post-selection in the two branches of the fork. We analyze the appearance of entanglement in a Bell inequality test formulated in terms of the number of transmitted electrons with a given spin polarization.
We investigate how entanglement can enhance two-photon absorption in a three-level system. First, we employ the Schmidt decomposition to determine the entanglement properties of the optimal two-photon state to drive such a transition, and the maximum enhancement which can be achieved in comparison to the optimal classical pulse. We then adapt the optimization problem to realistic experimental constraints, where photon pairs from a down-conversion source are manipulated by local operations such as spatial light modulators. We derive optimal pulse shaping functions to enhance the absorption effi…
A pair of optical pulses traveling through two dispersive media will become broadened and, as a result, the degree of coincidence between the optical pulses will be reduced. For a pair of entangled photons, however, nonlocal dispersion cancellation in which the dispersion experienced by one photon cancels the dispersion experienced by the other photon is possible. In this paper, we report an experimental demonstration of nonlocal dispersion cancellation using entangled photons. The degree of two-photon coincidence is shown to increase beyond the limit attainable without entanglement. Our resul…
High-precision time transfer is of fundamental interest in physics and metrology. Quantum time transfer technologies that use frequency-entangled pulses and their coincidence detection have been proposed, offering potential enhancements in precision and better guarantees of security. In this paper, we describe a fiber-optic two-way quantum time transfer experiment. Using quantum nonlocal dispersion cancellation, time transfer over a 20-km fiber link achieves a time deviation of 922 fs over 5 s and 45 fs over 40960 s. The time transfer accuracy as a function of fiber lengths from 15 m to 20 km …
The Einstein Podolsky Rosen (EPR) entangled quantum state is of special importance not only for fundamental research in quantum mechanics, but also for information processing in the field of quantum information. Previous EPR entangled state demonstrations were constructed with photons of equal phase wave fronts. More complex scenarios with structured wave fronts have not been investigated. Here, we report the first experimental demonstration of EPR entanglement for photon pairs carrying orbital angular momentum (OAM) information, resulting in an OAM embedded EPR entangled state. We measured th…
We create pairs of non-degenerate time-bin entangled photons at telecom wavelengths with ultra-short pump pulses. Entanglement is shown by performing Bell kind tests of the Franson type with visibilities of up to 91%. As time-bin entanglement can easily be protected from decoherence as encountered in optical fibers, this experiment opens the road for complex quantum communication protocols over long distances. We also investigate the creation of more than one photon pair in a laser pulse and present a simple tool to quantify the probability of such events to happen.
We demonstrate a coherent and dynamic beam splitter based on light storage in cold atoms. An input weak laser pulse is first stored in a cold atom ensemble via electromagnetically-induced transparency (EIT). A set of counter-propagating control fields, applied at a later time, retrieves the stored pulse into two output spatial modes. The high visibility interference between the two output pulses clearly demonstrates that the beam splitting process is coherent. Furthermore, by manipulating the control lasers, it is possible to dynamically control the storage time, the power splitting ratio, the…
Controls of waveforms (pulse durations) of single photons are important tasks for effectively interconnecting disparate atomic memories in hybrid quantum networks. So far, the waveform control of single photon that is entangled with an atomic memory remains unexplored. Here, we demonstrated control of waveform length of the photon that is entangled with an atomic spin-wave memory by varying light-atom interaction time in cold atoms. The Bell parameter S as a function of the duration of photon pulse is measured, which shows that violations of Bell equality can be achieved for the photon pulse i…
Entangled photon pairs are key to many novel applications in quantum technologies. Semiconductor quantum dots can be used as sources of on-demand, highly entangled photons. The fidelity to a fixed maximally entangled state is limited by the excitonic fine-structure splitting. This work demonstrates that, even if this splitting is absent, the degree of entanglement cannot reach unity when the excitation pulse in a two-photon resonance scheme has a finite duration. The degradation of the entanglement has its origin in a dynamically induced splitting of the exciton states caused by the laser puls…
Entangled states are crucial for modern quantum enabled technology which makes their creation key for future developments. In this paper, a robust quantum control methodology is presented to create entangled states of two typical classes, the W and the Greenberger-Horne-Zeilinger (GHZ). It was developed from the analysis of a chain of alkali atoms $^{87}Rb $ interaction with laser pulses, which lead to the two-photon transitions from the ground to the Rydberg states with a predetermined magnetic quantum number. The methodology is based on the mechanism of two-photon adiabatic passage using ove…
We demonstrate a scheme to spectrally manipulate a collinear, continuous stream of time and energy entangled photons to generate beamlike, bandwidth-limited fuxes of polarization-entangled photons with nearly-degenerate wavelengths. Utilizing an ultrashort-pulse shaper to control the spectral phase and polarization of the photon pairs, we tailor the shape of the Hong-Ou-Mandel interference pattern, demonstrating the rules that govern the dependence of this interference pattern on the spectral phases of the photons. We then use the pulse shaper to generate all four polarization Bell states. The…
We present a proposal for storing and retrieving a continuous-variable quadripartite polarization-entangled cluster state, using macroscopic atomic ensembles in a magnetic field. The Larmor precession of the atomic spins leads to a symmetry between the atomic canonical operators. In this scheme, each of the four spatially separated pulses passes twice through the respective ensemble in order to map the polarization-entangled cluster state onto the long-lived atomic ensembles. The stored state can then be retrieved by another four read-out pulses, each crossing the respective ensemble twice. By…
In this work we analyse the structure of highly-entangled multimode squeezed states, such as those generated by broadband pulses undergoing type-II parametric down-conversion (PDC). Such down-conversion has previously been touted as a natural and efficient means of cluster-state generation, and therefore a viable future pathway to quantum computation. We first detail how broadband PDC processes lead directly to a series of orthogonal supermodes that are linear combinations of the original frequency modes. We then calculate the total squeezing of the multimode entangled states when they are ass…
We present a source of polarization entangled photon pairs based on spontaneous parametric downconversion engineered for frequency uncorrelated telecom photon generation. Our source provides photon pairs that display, simultaneously, the key properties for high-performance quantum information and fundamental quantum science tasks. Specifically, the source provides for high heralding efficiency, high quantum state purity and high entangled state fidelity at the same time. Among different tests we apply to our source we observe almost perfect non-classical interference between photons from indep…
Effectiveness of using laser field to produce entanglement between two dipole-interacting identical two-level atoms is considered in detail. The entanglement is achieved by driving the system with a carefully designed laser pulse transferring the system's population to one of the maximally entangled Dicke states in a way analogous to population inversion by a resonant $π$-pulse in a two-level atom. It is shown that for the optimally chosen pulse frequency, power and duration, the fidelity of generating a maximally entangled state approaches unity as the distance between the atoms goes to zero.
We analyze a scheme for preparation of magnetically ordered states of two-component bosonic atoms in optical lattices. We compute the dynamics during adiabatic and optimized time-dependent ramps to produce ground states of effective spin Hamiltonians, and determine the robustness to decoherence for realistic experimental system sizes and timescales. Ramping parameters near a phase transition point in both effective spin-1/2 and spin-1 models produces entangled spin-symmetric states that have potential future applications in quantum enhanced measurement. The preparation of these states and thei…
We demonstrate an optical-fiber based source of polarization entangled photon-pairs with improved quality and efficiency, which has been integrated with off-the-shelf telecom components and is, therefore, well suited for quantum communication applications in the 1550 nm telecom band. Polarization entanglement is produced by simultaneously pumping a loop of standard dispersion-shifted fiber with two orthogonally-polarized pump pulses, one propagating in the clockwise and the other in the counter-clockwise direction. We characterize this source by investigating two-photon interference between th…
The paper investigates cold molecules formation in the photoassociation of two cold atoms by a strong laser pulse applied at short interatomic distances, which lead to a molecular dynamics taking place in the light-induced (adiabatic) potentials. A two electronic states model in the cesium dimer is used to analyse the effects of this strong coupling regime and to show specific results: i) acceleration of the ground state population to the inner zone due to a non-impulsive regime of coupling at short and intermediate interatomic distances; ii) formation of cold molecules in strongly bound level…
Quantum memory is an essential building block for quantum communication and scalable linear quantum computation. Storing two color entangled photons, with one photon being at telecom-wavelength while the other photon being compatible of quantum memory, has great advantages toward the realization of the fiber based long-distance quantum communication with the aid of quantum repeaters. Here, we report an experimental realization of storing a photon entangled with a telecom photon in polarization as an atomic spin wave in a cold atomic ensemble, thus establishing the entanglement between the tele…
We have studied stationary and quasi-stationary signal light pulses in cold lambda-type atomic media driven by counterpropagating control laser fields at the condition of electromagnetically induced transparency. By deriving a dispersion relation we present spectral and temporal properties of the signal light pulse and a significant influence of atomic decoherence on the coupled stationary light pulses for spatial splitting. Finally we discuss quasi-stationary light pulse evolution characterized by frozen spatial spreading for a robust coherent control of slow light pulses.
A pulsed laser scenario, designed to prepare an appropriately chosen self-assembled quantum dot with 100% population in a biexciton state, is proposed. The ensuing radiative emission would provide a near perfect (99.5%) high rate, on-demand, source of entangled photons.
Tapered optical fibers with a nanofiber waist are versatile tools for interfacing light and matter. In this context, laser-cooled atoms trapped in the evanescent field surrounding the optical nanofiber are of particular interest: They exhibit both long ground-state coherence times and efficient coupling to fiber-guided fields. Here, we demonstrate electromagnetically induced transparency, slow light, and the storage of fiber-guided optical pulses in an ensemble of cold atoms trapped in a nanofiber-based optical lattice. We measure a slow-down of light pulses to group velocities of 50 m/s. More…
We report on the delay of optical pulses using electromagnetically induced transparency in an ensemble of cold atoms with an optical depth exceeding 500. To identify the regimes in which four-wave mixing impacts on EIT behaviour, we conduct the experiment in both rubidium 85 and rubidium 87. Comparison with theory shows excellent agreement in both isotopes. In rubidium 87, negligible four-wave mixing was observed and we obtained one pulse-width of delay with 50% efficiency. In rubidium 85, four-wave-mixing contributes to the output. In this regime we achieve a delay-bandwidth product of 3.7 at…
We propose and demonstrate an atomic qubit based on a cold $^{85}$Rb-$^{87}$Rb isotopic mixture, entangled with a frequency-encoded optical qubit. The interface of an atomic qubit with a single spatial light mode, and the ability to independently address the two atomic qubit states, should provide the basic element of an interferometrically robust quantum network.
We present a very simple model for realizing directed transport with cold atoms in a pair of periodically flashed optical lattices. The origin of this ratchet effect is explained and its robustness demonstrated under imperfections typical of cold atom experiments. We conclude that our model offers a clear-cut way to implement directed transport in an atom optical experiment.
