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arXiv quant-ph/0406138quant-ph
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单分子纯电子零声子线发射的超长相干时间

Ultralong coherence times in the purely electronic zero-phonon line emission of single molecules

Alper Kiraz, Moritz Ehrl, Christoph Bräuchle, Andreas Zumbusch

摘要:

本文报道了在1.4K下观察到的单聚萘二酰亚胺分子纯电子零声子线发射的超长相干时间。振动激发和光谱分辨检测与扫描法布里-珀罗光谱分析仪被用来测量65 MHz的线宽。这在变换极限的1.6倍内。这表明单分子辐射可能适用于线性光学量子计算。此外,它示出,高分辨率光谱与光谱分析仪允许快速光谱动力学的调查在一个单一的分子的发射。

英文摘要:

We report the observation of ultralong coherence times in the purely electronic zero-phonon line emission of single terrylenediimide molecules at 1.4 K. Vibronic excitation and spectrally resolved detection with a scanning Fabry-Perot spectrum analyzer were used to measure a linewidth of 65 MHz. This is within a factor of 1.6 of the transform limit. It therefore indicates that single molecule emission may be suited for applications in linear optics quantum computation. Additionally it is shown that high resolution spectra taken with the spectrum analyzer allow for the investigation of fast spectral dynamics in the emission of a single molecule.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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