The interference of two single photons impinging on a beam splitter is measured in a time-resolved manner. Using long photons of different frequencies emitted from an atom-cavity system, a quantum beat with a visibility close to 100% is observed in the correlation between the photodetections at the output ports of the beam splitter. The time dependence of the beat amplitude reflects the coherence properties of the photons. Most remarkably, simultaneous photodetections are never observed, so that a temporal filter allows one to obtain perfect two-photon coalescence even for non-perfect photons.
By using spontaneous Raman processes in the high gain regime, we produce two independent Raman Stokes fields from an atomic ensemble. Temporal beating is observed between the two directly generated Stokes fields in a single realization. The beat frequency is found to be a result of an AC Stark frequency shift effect. However, due to the spontaneous nature of the process, the phases of the two Stokes fields change from one realization to another so that the beat signal disappears after average over many realizations. On the other hand, the beat signal is recovered in a two-photon correlation me…
We present an experiment testing quantum correlations with frequency shifted photons. We test Bell inequality with 2-photon interferometry where we replace the beamsplitters by acousto-optic modulators, which are equivalent to moving beamsplitters. We measure the 2-photon beatings induced by the frequency shifts, and we propose a cryptographic scheme in relation. Finally, setting the experiment in a relativistic configuration, we demonstrate that the quantum correlations are not only independent of the distance but also of the time ordering between the two single-photon measurements.
We characterize correlations in polarization and time of photon pairs generated from a cold cloud of Rb-87 atoms via a four-wave mixing process in a cascade level scheme. Quantum state tomography reveals entangled polarization states of high purity for each of the decay paths through two different intermediate hyperfine levels. When allowing both decay paths, we observe quantum beats in time-resolved correlation measurements.
We consider a recursive device that is based on a Mach-Zehnder interferometer and linear optical elements which allow self-feedback through multiple internal reflection of radiation between two parallel arrays of opposite faced mirrors. By a carefully chosen experimental arrangement and for certain input states it is possible to observe at the open ends of the device time generated coherent superpositions \textit{in perpetuum}.
Precision measurements are important across all fields of science. In particular, optical phase measurements can be used to measure distance, position, displacement, acceleration and optical path length. Quantum entanglement enables higher precision than would otherwise be possible. We demonstrate an optical phase measurement with an entangled four photon interference visibility greater than the threshold to beat the standard quantum limit--the limit attainable without entanglement. These results open the way for new high-precision measurement applications.
Quantum resources outperform classical ones for certain communication and computational tasks. Remarkably, in some cases, the quantum advantage cannot be improved using hypothetical postquantum resources. A class of tasks with this property can be singled out using graph theory. Here we report the experimental observation of an impossible-to-beat quantum advantage on a four-dimensional quantum system defined by the polarization and orbital angular momentum of a single photon. The results show pristine evidence of the quantum advantage and are compatible with the maximum advantage allowed using…
We devise a new technique to enhance transmission of quantum information through linear optical quantum information processors. The idea is based on applying the Quantum Zeno effect to the process of photon absorption. By frequently monitoring the presence of the photon through a QND (quantum non-demolition) measurement the absorption is suppressed. Quantum information is encoded in the polarization degrees of freedom and is therefore not affected by the measurement. Some implementations of the QND measurement are proposed.
We experimentally demonstrate quantum enhanced resolution in confocal fluorescence microscopy exploiting the non-classical photon statistics of single nitrogen-vacancy colour centres in diamond. By developing a general model of super-resolution based on the direct sampling of the kth-order autocorrelation function of the photoluminescence signal, we show the possibility, in some cases, to resolve in principle arbitrarily close emitting centers.
Multiparameter estimation theory offers a general framework to explore imaging techniques beyond the Rayleigh limit. While optimal measurements of single parameters characterizing a composite light source are now well understood, simultaneous determination of multiple parameters poses a much greater challenge that in general requires implementation of collective measurements. Here we show, theoretically and experimentally, that Hong-Ou-Mandel interference followed by spatially resolved detection of photons provides precise information on both the separation and the centroid for a pair of point…
We propose a two-photon beating experiment based upon biphotons generated from a resonant pumping two-level system operating in a backward geometry. On the one hand, the linear optical-response leads biphotons produced from two sidebands in the Mollow triplet to propagate with tunable refractive indices, while the central-component propagates with unity refractive index. The relative phase difference due to different refractive indices is analogous to the pathway-length difference between long-long and short-short in the original Franson interferometer. By subtracting the linear Rayleigh scatt…
Quantum metrology promises high-precision measurements beyond the capability of any classical techniques, and has the potential to be integral to investigative techniques. However, all sensors must tolerate imperfections if they are to be practical. Here we show that photons with perfectly overlapped modes, which are therefore fully indistinguishable, are not required for quantum-enhanced measurement, and that partially-distinguishable photons do not have to be engineered to mitigate the adverse effects of distinguishability. We quantify the effect of distinguishability on quantum metrology ex…
We propose and demonstrate experimentally a projection scheme to measure the quantum phase with a precision beating the standard quantum limit. The initial input state is a twin Fock state $|N,N>$ proposed by Holland and Burnett [Phys. Rev. Lett. {\bf 71}, 1355 (1993)] but the phase information is extracted by a quantum state projection measurement. The phase precision is about $1.4/N$ for large photon number $N$, which approaches the Heisenberg limit of 1/N. Experimentally, we employ a four-photon state from type-II parametric down-conversion and achieve a phase uncertainty of $0.291\pm 0.001…
Spatial quantum enhancement effects are studied under a unified framework. It is shown that the multiphoton absorption rate of photons with a quantum-enhanced lithographic resolution is reduced, not enhanced, contrary to popular belief. The use of adiabatic soliton expansion is proposed to beat the standard quantum limit on the optical beam displacement accuracy, as well as to engineer an arbitrary multiphoton interference pattern for quantum lithography. The proposed scheme provides a conceptually simple method that works for an arbitrary number of photons.
The interferometer is one of the most important devices for revealing the nature of light and for precision optical metrology. Though lots of experiments were performed for probing photons behaviors in various configurations, a complete study of photons behavior in a birefringent interferometer has not ever been performed. Based on an environmental turbulence immune Mach-Zehnder interferometer, tunable photonic beatings by rotating a birefringent crystal versus the temperature of the crystal for both single-photon and two-photon are observed. Furthermore, the two-photon interference fringes be…
Quantum number-path entanglement is a resource for super-sensitive quantum metrology and in particular provides for sub-shotnoise or even Heisenberg-limited sensitivity. However, such number-path entanglement has thought to have been resource intensive to create in the first place --- typically requiring either very strong nonlinearities, or nondeterministic preparation schemes with feed-forward, which are difficult to implement. Very recently, arising from the study of quantum random walks with multi-photon walkers, as well as the study of the computational complexity of passive linear optica…
Surpassing the repeaterless bound is a crucial task on the way towards realizing long-distance quantum key distribution. In this paper, we focus on the protocol proposed by Azuma et al. in [Nature Communications 6, 10171 (2015)], which can beat this bound with idealized devices. We investigate the robustness of this protocol against imperfections in realistic setups, particularly the multiple-photon pair components emitted by practical entanglement sources. In doing so, we derive necessary conditions on the photon-number statistics of the sources in order to beat the repeaterless bound. We sho…
Dense coding is arguably the protocol that launched the field of quantum communication. Today, however, more than a decade after its initial experimental realization, the channel capacity remains fundamentally limited as conceived for photons using linear elements. Bob can only send to Alice three of four potential messages owing to the impossibility of carrying out the deterministic discrimination of all four Bell states with linear optics, reducing the attainable channel capacity from 2 to log_2 3 \approx 1.585 bits. However, entanglement in an extra degree of freedom enables the complete an…
In 2011, Nair published a no-go theorem for quantum radar target detection [Phys. Rev. A {\bf 84}, 032312 (2011)]. He showed, under fairly general assumptions, that a coherent-state radar's error probability was within a factor of two of the best possible quantum performance for the pure-loss (no background radiation) channel whose roundtrip radar-to-target-to-radar transmissivity $κ$ satisfies $κ\ll 1$. We introduce first-photon radars (FPRs) to circumvent and beat Nair's performance limit. FPRs transmit a periodic sequence of pulses, each containing $N_S$ photons on average, and perform idea…
Quantum metrology promises greater sensitivity for optical phase measurements than could ever be achieved classically. Here we present a theory of the phase sensitivity for the general case where the detection probability is given by an $N$ photon interference fringe. We find that the phase sensitivity has a complex dependence on both the intrinsic efficiency of detection $η$ and the interference fringe visibility $V$. Most importantly, the phase that gives maximum phase sensitivity is in general not the same as the phase at which the slope of the interference fringe is a maximum, as has previ…
Detailed derivation of the master equation and the corresponding time evolution of the cavity radiation of a coherent beat laser when the atoms are initially prepared in a partial coherent superposition is presented. It turns out that the quantum features and intensity of the cavity radiation are considerably modified by the phase fluctuation arising due to the practical incapability of preparing atoms in the intended coherent superposition. New terms having an opposite sign with the contribution of the driving radiation emerged in the master equation. This can be taken as an indication for a …
Boson sampling is considered as a strong candidate to demonstrate the quantum computational supremacy over classical computers. However, previous proof-of-principle experiments suffered from small photon number and low sampling rates owing to the inefficiencies of the single-photon sources and multi-port optical interferometers. Here, we develop two central components for high-performance boson sampling: robust multi-photon interferometers with 0.99 transmission rate, and actively demultiplexed single-photon sources from a quantum-dot-micropillar with simultaneously high efficiency, purity and…
We demonstrate the tunable quantum beat of single photons through the co-development of core nonlinear nanophotonic technologies for frequency-domain manipulation of quantum states in a common physical platform. Spontaneous four-wave mixing in a nonlinear resonator is used to produce non-degenerate, quantum-correlated photon pairs. One photon from each pair is then frequency shifted, without degradation of photon statistics, using four-wave mixing Bragg scattering in a second nonlinear resonator. Fine tuning of the applied frequency shift enables tunable quantum interference of the two photons…
Classical, interferometric, optical lithography is diffraction limited to writing features of a size lambda/2 or greater, where lambda is the optical wavelength. Using nonclassical photon number states, entangled N at a time, we show that it is possible to write features of minimum size lambda/(2N) in an N-photon absorbing substrate. This result surpasses the usual classical diffraction limit by a factor of N. Since the number of features that can be etched on a two-dimensional surface scales inversely as the square of the feature size, this allows one to write a factor of N^2 more elements on…
We demonstrate a method for characterizing the coherence function of coherent states based on two-photon interference. Two states from frequency mismatched faint laser sources are fed into a Hong-Ou-Mandel interferometer and the interference pattern is fitted with the presented theoretical model for the quantum beat. The fitting parameters are compared to the classical optical beat when bright versions of the sources are used. The results show the equivalence between both techniques.
In practical quantum key distribution, weak coherent state is often used and the channel transmittance can be very small therefore the protocol could be totally insecure under the photon-number-splitting attack. We propose an efficient method to verify the upper bound of the fraction of counts caused by multi-photon pluses transmitted from Alice to Bob, given whatever type of Eve's action. The protocol simply uses two coherent states for the signal pulses and vacuum for decoy pulse. Our verified upper bound is sufficiently tight for QKD with very lossy channel, in both asymptotic case and non-…
We probe a ground-state superposition that produces a quantum beat in the intensity correlation of a two-mode cavity QED system. We mix drive with scattered light from an atomic beam traversing the cavity, and effectively measure the interference between the drive and the light from the atom. When a photon escapes the cavity, and upon detection, it triggers our feedback which modulates the drive at the same beat frequency but opposite phase for a given time window. This results in a partial interruption of the beat oscillation in the correlation function, that then returns to oscillate.
Hong-Ou-Mandel interference, the fact that identical photons that arrive simultaneously on different input ports of a beam splitter bunch into a common output port, can be used to measure optical delays between different paths. It is generally assumed that great precision in the measurement requires that photons contain many frequencies, i.e., a large bandwidth. Here we challenge this well-known assumption and show that the use of two well-separated frequencies embedded in a quantum entangled state (discrete color entanglement) suffices to achieve great precision. We determine optimum working …
We study the sensitivity and resolution of phase measurement in a Mach-Zehnder interferometer with two-mode squeezed vacuum (<n> photons on average). We show that super-resolution and sub-Heisenberg sensitivity is obtained with parity detection. In particular, in our setup, dependence of the signal on the phase evolves <n> times faster than in traditional schemes, and uncertainty in the phase estimation is better than 1/<n>.
We study photon-photon correlations and entanglement generation in a one-dimensional waveguide coupled to two qubits with an arbitrary spatial separation. We develop a novel Green function method to study vacuum-mediated qubit-qubit interactions, including both spontaneous and coherent couplings. As a result of these interactions, quantum beats appear in the second-order correlation function. We go beyond the Markovian regime and observe that such quantum beats persist much longer than the qubit life time. Using these non-Markovian processes, a high degree of long-distance entanglement can be …
Conditional measurements on the undriven mode of a two-mode cavity QED system prepare a coherent superposition of ground states which generate quantum beats. The continuous system drive induces decoherence through the phase interruptions from Rayleigh scattering, which manifests as a decrease of the beat amplitude and an increase of the frequency of oscillation. We report recent experiments that implement a simple feedback mechanism to protect the quantum beat. We continuously drive the system until a photon is detected, heralding the presence of a coherent superposition. We then turn off the …
Precise characterization of a hyperfine interaction is a prerequisite for high fidelity manipulations of electron and nuclear spins belonging to a hybrid qubit register in diamond. Here, we demonstrate a novel scheme for determining a hyperfine interaction, using single-quantum and zero-quantum Ramsey fringes, by applying it to the system of a Nitrogen Vacancy (NV) center and a $^{13}$C nuclear spin in the 1$^{\mathrm{st}}$ shell. The zero-quantum Ramsey fringe, analogous to the quantum beat in a $Λ$-type level structure, particularly enhances the measurement precision for non-secular hyperfin…
We report ground-state quantum beats in spontaneous emission from a continuously driven atomic ensemble. Beats are visible only in an intensity autocorrelation and evidence spontaneously generated coherence in radiative decay. Our measurement realizes a quantum eraser where a first photon detection prepares a superposition and a second erases the "which-path" information in the intermediate state.
We implement a simple feedback mechanism on a two-mode cavity QED system to preserve the Zeeman coherence of a ground state superposition that generates quantum beats on the second-order correlation function. Our investigation includes theoretical and experimental studies that show how to prevent a shift away from the Larmor frequency and associated decoherence caused by Rayleigh scattering. The protocol consists of turning off the drive of the system after the detection of a first photon and letting it evolve in the dark. Turning the drive back on after a pre-set time reveals a phase accumula…
The spatiotemporal dynamics of photon emission into a non-local farfield channel and two local nearfield channels from a pair of coupled two level systems is analysed using a model for emission based on Wigner-Weisskopf theory. The local quantum beats can be observed in the two nearfield channels. However, the presence of the farfield causes decoherence in the quantum beats even if only photon emissions into the near field channels are considered.
Spin interferometry of the 4th order for independent polarized as well as unpolarized photons arriving simultaneously at a beam splitter and exhibiting spin correlation while leaving it, is formulated and discussed in the quantum approach. Beam splitter is recognized as a source of genuine singlet photon states. Also, typical nonclassical beating between photons taking part in the interference of the 4th order is given a polarization dependent explanation.
We investigate quantum beats in the arrival-time distribution of single photons from a single trapped $^{40}$Ca$^+$ ion, revealing their fundamentally different physical origins in two distinct experimental situations: In a $Λ$-type level scheme the interference of two 854-nm absorption amplitudes suppresses and enhances the emission process of Raman-scattered 393-nm photons; in a V-type level scheme the interference of two 393-nm emission amplitudes causes a rotation of their dipole emission pattern resulting in a temporal modulation of the detected photons. For both cases we demonstrate cohe…
The spontaneous creation and persistence of ground-state coherence in an ensemble of intracavity Rb atoms has been observed as a quantum beat. Our system realizes a quantum eraser, where the detection of a first photon prepares a superposition of ground-state Zeeman sublevels, while detection of a second erases the stored information. Beats appear in the time-delayed photon-photon coincidence rate (intensity correlation function). We study the beats theoretically and experimentally as a function of system parameters, and find them remarkably robust against perturbations such as spontaneous emi…
We report on an experiment demonstrating entanglement swapping of time-frequency entangled photons. We perform a frequency-resolved Bell-state measurement on the idler photons from two independent entangled photon pairs, which projects the signal photons onto a two-color Bell state. We verify entanglement in this heralded state using two-photon interference and observing quantum beating without the use of filters, indicating the presence of two-color entanglement. Our method could lend itself to use as a highly-tunable source of frequency-bin entangled single photons.
We experimentally demonstrate the generation of heralded bi-chromatic single photons from an atomic collective spin excitation (CSE). The photon arrival times display collective quantum beats, a novel interference effect resulting from the relative motion of atoms in the CSE. A combination of velocity-selective excitation with strong laser dressing and the addition of a magnetic field allows for exquisite control of this collective beat phenomenon. The present experiment uses a diamond scheme with near-IR photons that can be extended to include telecommunications-wavelengths or modified to all…
We provide a compact full description of multiboson correlation measurements of arbitrary order N in passive linear interferometers with arbitrary input single-photon pure states. This allows us to physically analyze the novel problem of multiboson correlation sampling at the output of random linear interferometers. Our results also describe general multiboson correlation landscapes for an arbitrary number of input single photons and arbitrary interferometers. In particular, we use two different schemes to demonstrate, respectively, arbitrary-order quantum beat interference and 100% visibility…
We calculate the one- and two-photon scattering matrices of a pair of collocated non-identical two-level atoms coupled to a waveguide. We show that by proper choice of a two-photon input, the background fluorescence by the atoms may be completely quenched, as a result of quantum interference, and that when the atoms' detuning is smaller than their linewidths, extremely narrow fluorescence features emerge. Furthermore, the system emits a two-photon bound state which can display spatial oscillations/quantum beats, and can be tuned from bunched to anti-bunched statistics as the total photon energ…
We present two-photon interference experiments with polarization-entangled photon pairs in a polarization-based Franson-type interferometer. Although the two photons do not meet at a common beamsplitter, a phase-insensitive Hong-Ou-Mandel type two-photon interference peak and dip fringes are observed, resulting from the two-photon interference effect between two indistinguishable two-photon probability amplitudes leading to a coincidence detection. A spatial quantum beating fringe is also measured for nondegenerate photon pairs in the same interferometer, although the two-photon states have no…
There has been much recent interest in quantum metrology for applications to sub-Raleigh ranging and remote sensing such as in quantum radar. For quantum radar, atmospheric absorption and diffraction rapidly degrades any actively transmitted quantum states of light, such as N00N states, so that for this high-loss regime the optimal strategy is to transmit coherent states of light, which suffer no worse loss than the linear Beer's law for classical radar attenuation, and which provide sensitivity at the shot-noise limit in the returned power. We show that coherent radar radiation sources, coupl…
It is shown how to implement quantum feedback and probabilistic error correction in an open quantum system consisting of a single atom, with ground- and excited-state Zeeman structure, in a driven two-mode optical cavity. The ground state superposition is manipulated and controlled through conditional measurements and external fields, which shield the coherence and correct quantum errors. Modeling of an experimentally realistic situation demonstrates the robustness of the proposal for realization in the laboratory.
Chirped-pulse interferometry (CPI) captures the metrological advantages of quantum Hong-Ou-Mandel (HOM) interferometry in a completely classical system. Modified HOM interferometers are the basis for a number of seminal quantum-interference effects. Here, the corresponding modifications to CPI allow for the first observation of classical analogues to the HOM peak and quantum beating. They also allow a new classical technique for generating phase super-resolution exhibiting a coherence length dramatically longer than that of the laser light, analogous to increased two-photon coherence lengths i…
The interference of two independent single-photon pulses impinging on a beam splitter is analysed in a generalised time-resolved manner. Different aspects of the phenomenon are elaborated using different representations of the single-photon wave packets, like the decomposition into single-frequency field modes or spatio-temporal modes matching the photonic wave packets. Both representations lead to equivalent results, and a photon-by-photon analysis reveals that the quantum-mechanical two-photon interference can be interpreted as a classical one-photon interference once a first photon is detec…
Scattershot photon sources are known to have useful properties for optical quantum computing and boson sampling purposes, in particular for scaling to large numbers of photons. This paper investigates the application of these scattershot sources towards the metrological task of estimating an unknown phase shift. In this regard, we introduce three different scalable multimode interferometers, and quantify their quantum Fisher information performance using scattershot sources with arbitrary system sizes. We show that two of the interferometers need the probing photons to be in certain input conf…
We investigate the quantum discord dynamics and inversion operator of a two-level atom initially in thermal equilibrium mixed state interacting with a cavity field prepared in a n-photon Fock state. We considered the Jaynes-Cummings model which is an exactly quantum mechanical model of interaction between two different quantum systems, an optical cavity in single mode n-photon Fock state and a two-level atom. The influence of interaction time and measurement basis used for calculating the conditional entropy is discussed on the evolution of the quantum discord and on its minimum. The evolution…
