We propose to entangle macroscopic atomic ensembles in cavity using EPR-correlated beams. We show how the field entanglement can be almost perfectly mapped onto the long-lived atomic spins associated with the ground states of the ensembles, and how it can be retrieved in the fields exiting the cavities after a variable storage time. Such a continuous variable quantum memory is of interest for manipulating entanglement in quantum networks.
Coherent and reversible storage of multi-photon entanglement with a multimode quantum memory is essential for scalable all-optical quantum information processing. Although single photon has been successfully stored in different quantum systems, storage of multi-photon entanglement remains challenging because of the critical requirement for coherent control of photonic entanglement source, multimode quantum memory, and quantum interface between them. Here we demonstrate a coherent and reversible storage of biphoton Bell-type entanglement with a holographic multimode atomic-ensemble-based quantu…
Quantum computation requires efficient long-term storage devices to preserve quantum states. An attractive candidate for such storage devices is qubits connected to a common dissipative environment. The common environment gives rise to persistent entanglements in these qubit systems. Hence these systems act efficiently as a storage device of entanglement. However, the existence of a common environment often requires the physical proximity of the qubits and hence results in direct dipolar coupling between the qubits. In this work, we investigate the total effect of the dipolar coupling on the e…
We introduce a protocol based on optimal control to drive many body quantum systems into long-lived entangled states, protected from decoherence by big energy gaps, without requiring any apriori knowledge of the system. With this approach it is possible to implement scalable entanglement-storage units. We test the protocol in the Lipkin-Meshkov-Glick model, a prototype many-body quantum system that describes different experimental setups, and in the ordered Ising chain, a model representing a possible implementation of a quantum bus.
A novel method of multi-bit quantum optical data storage is presented, where the storage time can be lengthened far beyond the spin phase-decay time in a reversible spin inhomogeneous system excited by consecutive resonant Raman optical data pulses. The ultralong storage time is obtained by an optical population locking mechanism of modified rephasing process. This gives potentials to quantum repeaters utilizing quantum memories for long distance quantum communications, in which ultralong storage time plays a major role.
The deployment of a fully-fledged quantum internet poses the challenge of finding adequate building-blocks for entanglement distribution between remote quantum nodes. An ideal system would combine propagation in optical fibres with quantum memories for light, leveraging on the existing communication network while featuring the scalability required to extend to network sizes. Here we demonstrate a fiber-integrated quantum memory entangled with a photon at telecommunication wavelength. The storage device is based on a fiber-pigtailed laser written waveguide in a rare-earth doped solid and allows…
We replace time-averaged entanglement by ensemble-averaged entanglement and derive a simple expression for the latter. We show how to calculate the ensemble average for a two-spin system and for the Jaynes-Cummings model. In both cases the time-dependent entanglement is known as well so that one can verify that the time average coincides with the ensemble average.
We study how to efficiently manipulate and store quantum information between optical fields and atomic ensembles. We show how various non-dissipative transfer schemes can be used to transfer and store quantum states such as squeezed vacuum states or entangled states into the long-lived ground state spins of atomic ensembles.
The time evolution of the entanglement of a pair of two spin qubits is investigated when the two qubits simultaneously couple to an environment of an anisotropic Heisenberg XXZ spin chain. The entanglement of the two spin qubits can be created and is a periodic function of the time if the magnetic field is greater than a critical value. If the two spin qubits are in the Bell state, the entanglement can be stored with relatively large value even when the magnetic field is large.
We propose a quantum storage scheme independent of the current time-control schemes, and study a "quantum data bus" (transmission line resonator) in a hybrid system consisting of a circuit QED system integrated with a cold molecular ensemble. Here, an effective interaction between charge qubit and molecule is mediated by the off-resonate field in the data bus. Correspondingly, the charge state can be mapped into the collective quasi-spin state of the molecular ensemble via the standard dark state based adiabatic manipulation.
Scaling law for optimal excitation storage and superradiant release in waveguide QED systems
National Taiwan University（台湾大学）；Institute of Atomic and Molecular Sciences, Academia Sinica（中央研究院原子与分子科学研究所）；Center for Quantum Science and Engineering, National Taiwan University（台湾大学量子科学与工程中心）；Trapped-Ion Quantum Computing Laboratory, Hon Hai Research Institute（鸿海研究院会离子阱量子计算实验室）；Physics Division, National Center for Theoretical Sciences（国家理论科学中心物理组）；Department of Physics, National Central University（中央大学物理系）
We present a proposal for storing and retrieving a continuous-variable quadripartite polarization-entangled cluster state, using macroscopic atomic ensembles in a magnetic field. The Larmor precession of the atomic spins leads to a symmetry between the atomic canonical operators. In this scheme, each of the four spatially separated pulses passes twice through the respective ensemble in order to map the polarization-entangled cluster state onto the long-lived atomic ensembles. The stored state can then be retrieved by another four read-out pulses, each crossing the respective ensemble twice. By…
In this chapter, we will describe the storage and retrieval of quantum light (heralded single photons and entangled photons) in atomic ensembles in a solid state environment. We will consider ensembles of rare-earth ions embedded in dielectric crystals. We will describe the methods used to create quantum light spectrally compatible with the narrow atomic transitions, as well as possible protocols based on dipole rephasing that can be used to reversibly map the quantum light onto collective atomic excitations. We will review the experimental state of the art and describe in more detail quantum …
We propose an experimentally feasible scheme to generate nonmaximal entanglement between two atomic ensembles. The degree of entanglement is readily tunable. The scheme involves laser manipulation of atomic ensembles, adjustable quarter- and half-wave plates, beam splitter, polarizing beam splitters, and single-photon detectors, and well fits the status of the current experimental technology. Finally we use the nonmaximally entangled state of ensembles to demonstrate quantum nonlocality by detecting the Clauser-Horne-Shimony-Holt inequality.
Here we present the quantum storage of three-dimensional orbital-angular-momentum photonic entanglement in a rare-earth-ion-doped crystal. The properties of the entanglement and the storage process are confirmed by the violation of the Bell-type inequality generalized to three dimensions after storage ($S=2.152\pm0.033$). The fidelity of the memory process is $0.993\pm0.002$, as determined through complete quantum process tomography in three dimensions. An assessment of the visibility of the stored weak coherent pulses in higher-dimensional spaces, demonstrates that the memory is highly reliab…
We propose an experimentally feasible scheme to demonstrate quantum nonlocality, using Greenberger-Horne-Zeilinger (GHZ) and $W$ entanglement between atomic ensembles generated by a new developed method based on laser manipulation and{} single-photon detection.
We propose a scheme that employs dissipation to deterministically generate entanglement in an ensemble of strongly interacting Rydberg atoms. With a combination of microwave driving between different Rydberg levels and a resonant laser coupling to a short lived atomic state, the ensemble can be driven towards a dark steady state that entangles all atoms. The long-range resonant dipole-dipole interaction between different Rydberg states extends the entanglement beyond the van der Walls interaction range with perspectives for entangling large and distant ensembles.
We experimentally demonstrate room-temperature storage of quantum entanglement using two nuclear spins weakly coupled to the electronic spin carried by a single nitrogen-vacancy center in diamond. We realize universal quantum gate control over the three-qubit spin system and produce entangled states encoded within the decoherence-free subspace of the two nuclear spins. By injecting arbitrary collective noise, we demonstrate that the decoherence-free entangled state has coherence time longer than that of other entangled states by an order of magnitude in our experiment.
We analyze multipartite entanglement between atomic ensembles within quantum matter-light interfaces. In our proposal, a polarized light beam crosses sequentially several polarized atomic ensembles impinging on each of them at a given angle α_i. These angles are crucial parameters for shaping the entanglement since they are directly connected to the appropriate combinations of the collective atomic spins that are squeezed. We exploit such scheme to go beyond the pure state paradigm proposing realistic experimental settings to address multipartite mixed state entanglement in continuous variable…
Electron and nuclear spins have good coherence times and an ensemble of spins is a promising candidate for a quantum memory. By employing holographic techniques via field gradients a single ensemble may be used to store many bits of information. Here we present a coherent memory using a pulsed magnetic field gradient, and demonstrate the storage and retrieval of up to 100 weak 10 GHz coherent excitations in collective states of an electron spin ensemble. We further show that such collective excitations in the electron spin can then be stored in nuclear spin states, which offer coherence times …
I consider several interesting aspects of a new light source, a two-level atom, or N two-level atoms inside an Optical Parametric Oscillator. We find that in the weak driving limit, detection of a transmitted or fluorescent photon generates a highly entangled state of the atom and the cavity. This entanglement can be used with beamsplitters to create more complex quantum states and implement teleportation protocols. Also, one can store a single photon in the atoms, along the lines of recent slow and stopped light proposals and experiments.
We report the storage of microwave pulses at the single-photon level in a spin-ensemble memory consisting of $10^{10}$ NV centers in a diamond crystal coupled to a superconducting LC resonator. The energy of the signal, retrieved $100\, μ\mathrm{s}$ later by spin-echo techniques, reaches $0.3\%$ of the energy absorbed by the spins, and this storage efficiency is quantitatively accounted for by simulations. This figure of merit is sufficient to envision first implementations of a quantum memory for superconducting qubits.
Constructing a quantum memory for a photonic entanglement is vital for realizing quantum communication and network. Besides enabling the realization of high channel capacity communication, entangled photons of high-dimensional space are of great interest because of many extended applications in quantum information and fundamental physics fields. Photons entangled in a two-dimensional space had been stored in different system, but there have been no any report on the storage of a photon pair entangled in a high-dimensional space. Here, we report the first experimental realization of storing an …
Atomic ensembles are effective memory nodes for quantum communication network due to the long coherence time and the collective enhancement effect for the nonlinear interaction between an ensemble and a photon. Here we investigate the possibility of achieving the entanglement distillation for nonlocal atomic ensembles by the input-output process of a single photon as a result of cavity quantum electrodynamics. We give an optimal entanglement concentration protocol (ECP) for two-atomic-ensemble systems in a partially entangled pure state with known parameters and an efficient ECP for the system…
Recently, atomic ensemble and single photons were successfully entangled by using collective enhancement [D. N. Matsukevich, \textit{et al.}, Phys. Rev. Lett. \textbf{95}, 040405(2005).], where atomic internal states and photonic polarization states were correlated in nonlocal manner. Here we experimentally clarified that in an ensemble of atoms and a photon system, there also exists an entanglement concerned with spatial degrees of freedom. Generation of higher-dimensional entanglement between remote atomic ensemble and an application to condensed matter physics are also discussed.
An experimental feasible scheme is proposed to generate Greenberger-Horne-Zeilinger (GHZ) type of maximal entanglement. Distinguishing from the previous schemes, this entanglement can be chosen between either atomic ensembles (stationary qubit) or individual photons (flying qubit), according to the difference applications we desire for it. The physical requirements of the scheme are moderate and well fit the present experimental techinque.
Heralded entanglement between collective excitations in two atomic ensembles is probabilistically generated, stored, and converted to single photon fields. By way of the concurrence, quantitative characterizations are reported for the scaling behavior of entanglement with excitation probability and for the temporal dynamics of various correlations resulting in the decay of entanglement. A lower bound of the concurrence for the collective atomic state of 0.9\pm 0.3 is inferred. The decay of entanglement as a function of storage time is also observed, and related to the local dynamics.
Quantum protocols will be more efficient with high-dimensional entangled states. Photons carrying orbital angular momenta can be used to create a high-dimensional entangled state. In this paper we experimentally demonstrate the entanglement of the orbital angular momentum between the Stokes and anti-Stokes photons generated in a hot atomic ensemble using spontaneous four-wave-mixing. This experiment also suggests the existence of the entanglement concerned with spatial degrees of freedom between the hot atomic ensemble and the Stokes photon.
We present a protocol for increasing the entanglement between two atomic ensembles based on applying an approximate atom-light beamsplitter transformation to both ensembles. The effective asymmetric atom-light beamsplitter is created via a double-pass quantum non-demolition interaction between polarized light and a spin polarized atomic ensemble, derived from the linearised dipole interaction. The entanglement concentration protocol itself uses the procrustean method, similar to that first devised for light by Browne et al [2003 Phys Rev A 67 062320] and includes photon counting after the inte…
We propose a scheme for the creation of robust entanglement between a movable mirror and atomic ensemble at the macroscopic level in coupled optomechanical system. In experimentally accessible parameter regimes, we show that critical temperature of the bipartite continuous variable entanglement in our scheme can be raised from previous 24 K [Vitali {\it et al.}, Phys. Rev. Lett. \textbf{98}, 030405 (2007)] and 20 K [Genes {\it et al.}, Phys. Rev. A \textbf{77}, 050307(R) (2008)] to 32 K. We also investigate the entanglement transfer based on this coupled system. The scheme can be used for the …
We study the dynamical stability of the entanglement between the two spin ensembles in the presence of an environment. For a comparative study, we consider the two cases: a single spin ensemble, and two ensembles linearly coupled to a bath, respectively. In both circumstances, we assume the validity of the Markovian approximation for the bath. We examine the robustness of the state by means of the growth of the linear entropy which gives a measure of the purity of the system. We find out macroscopic entangled states of two spin ensembles can stably exist in a common bath. This result may be ve…
Entanglement is the fundamental characteristic of quantum physics. Large experimental efforts are devoted to harness entanglement between various physical systems. In particular, entanglement between light and material systems is interesting due to their prospective roles as "flying" and stationary qubits in future quantum information technologies, such as quantum repeaters and quantum networks. Here we report the first demonstration of entanglement between a photon at telecommunication wavelength and a single collective atomic excitation stored in a crystal. One photon from an energy-time ent…
Quantum information storage (QIS) is a physical process to write quantum states into a quantum memory (QM). We observe that in some general cases the quantum state can be retrieved up to a unitary transformation depicted by the non-Abelian Berry's geometric phase factor (holonomy). The QIS of photon with this geometric character can be implemented with the symmetric collective excitations of a $Λ$-atom ensemble, which is adiabatically controlled by a classical light with a small detuning $δ$. The cyclic change of the controlled Rabi frequency $Ω(t)$ with period $T=\frac{2nπ}δ$ accumulates addi…
We propose a scheme of generating and verifying mesoscopic-level entanglement between two atomic ensembles using non-resonant stimulated Raman scattering. Entanglement can be generated by direct detection or balanced homodyne detection of the Stokes fields from the two cells, after they interfere on a beam splitter. The entanglement of the collective atomic fields can be transferred to the anti-Stokes fields in a readout process. By measuring the operator moments of the anti-Stokes fields, we can verify the presence of entanglement. We model the effects of practical factors such as Stokes fiel…
It is crucial for physical realization of quantum information networks to first establish entanglement among multiple space-separated quantum memories and then at a user-controlled moment to transfer the stored entanglement to quantum channels for distribution and conveyance of information. Here we present an experimental demonstration on generation, storage and transfer of deterministic quantum entanglement among three spatially separated atomic ensembles. The off-line prepared multipartite entanglement of optical modes is mapped into three distant atomic ensembles to establish entanglement o…
Hybrid matter-photon entanglement is the building block for quantum networks. It is very favorable if the entanglement can be prepared with a high probability. In this paper, we report the deterministic creation of entanglement between an atomic ensemble and a single photon by harnessing Rydberg blockade. We design a scheme that creates entanglement between a single photon's temporal modes and the Rydberg levels that host a collective excitation, using a process of cyclical retrieving and patching. The hybrid entanglement is tested via retrieving the atomic excitation as a second photon and pe…
We present a protocol for performing entanglement connection between pairs of atomic ensembles in the single excitation regime. Two pairs are prepared in an asynchronous fashion and then connected via a Bell measurement. The resulting state of the two remaining ensembles is mapped to photonic modes and a reduced density matrix is then reconstructed. Our observations confirm for the first time the creation of coherence between atomic systems that never interacted, a first step towards entanglement connection, a critical requirement for quantum networking and long distance quantum communications…
In this paper we provide an operational method to detect multipartite entanglement in ensemble-based quantum computing. This method is based on the concept of entanglement witness. We decompose the entanglement witness for each class of multipartite entanglement into nonlocal operations in addition to local measurements. Individual single qubit measurements are performed simultaneously, hence complete detection of entanglement is performed in a single run experiment. This approach is particularly important for experiments where it is operationally difficult to prepare several copies of an unkn…
The Einstein-Podolsky-Rosen (EPR) entanglement is of special importance not only for fundamental research in quantum mechanics, but also for quantum information processing. Establishing EPR entanglement between two memory systems, such as atomic ensembles, nitrogen-vacancy centers, and rare-earth-ion-doped solids is promising for realizing spatial-multimode based quantum communication, quantum computation, and quantum imaging. To date, there have been few reports on realizing EPR entanglement between physical systems in true position and momentum. Here we describe successfully establishing suc…
Quantum repeaters hold the promise to prevent the photon losses in communication channels. Most recently, the serious efforts have been applied to achieve scalable distribution of entanglement over long distances. However, the probabilistic nature of entanglement generation and realistic quantum memory storage times make the implementation of quantum repeaters an outstanding experimental challenge. We propose a quantum repeater protocol based on the deterministic storage of a single photon in atomic ensembles confined in distant high-finesse cavities and show that this system is capable of dis…
We present an experimentally feasible protocol for the complete storage and retrieval of arbitrary light states in an atomic quantum memory using the well-established Faraday interaction between light and matter. Our protocol relies on multiple passages of a single light pulse through the atomic ensemble without the impractical requirement of kilometer long delay lines between the passages. Furthermore, we introduce a time dependent interaction strength which enables storage and retrieval of states with arbitrary pulse shapes. The fidelity approaches unity exponentially without squeezed or ent…
We consider a scheme of multiplexed cold atomic ensembles that generate a frequency-entangled biphoton state with controllable entropy of entanglement. The biphoton state consists of a telecommunication photon (signal) immediately followed by an infrared one (idler) via four-wave mixing with two classical pump fields. Multiplexing the atomic ensembles with frequency and phase-shifted signal and idler emissions, we can manipulate and control the spectral property of the biphoton state. Mapping out the entropy of entanglement in the scheme provides the optimal configuration for entanglement reso…
Here we demonstrate generating and storing entanglement in a solid state spin-wave quantum memory with on-demand read out using the process of rephased amplified spontaneous emission (RASE). Amplified spontaneous emission (ASE), resulting from an inverted ensemble of Pr$^{3+}$ ions doped into a Y$_2$SiO$_5$ crystal, generates entanglement between collective states of the praseodymium ensemble and the output light. The ensemble is then rephased using a four-level photon echo technique. Entanglement between the ASE and its echo is confirmed and the inseparability violation preserved when the RAS…
The entanglement of multi-atom quantum states is considered. In order to cancel noise due to inhomogeneous light atom coupling, the concept of matched multi-atom observables is proposed. As a means to eliminate an important form of decoherence this idea should be of broad relevance for quantum information processing with atomic ensembles. The general approach is illustrated on the example of rotation angle measurement, and it is shown that the multi-atom states that were thought to be only weakly entangled can exhibit near-maximum entanglement.
We study the modification of a traditional electromagnetically induced transparency (EIT) stored light technique that includes both EIT and four-wave mixing (FWM) in an ensemble of hot Rb atoms. The standard treatment of light storage involves the coherent and reversible mapping of one photonic mode onto a collective spin coherence. It has been shown that unwanted, competing processes such as four-wave mixing are enhanced by EIT and can significantly modify the signal optical pulse propagation. We present theoretical and experimental evidence to indicate that while a Stokes field is indeed det…
Coherent control of collective spontaneous emission in an extended atomic ensemble resonantly interacting with single-photon wave packets is analyzed. A scheme for coherent manipulation of collective atomic states is developed such that superradiant states of the atomic system can be converted into subradiant ones and vice versa. Possible applications of such a scheme for optical quantum state storage and single-photon wave packet shaping are discussed. It is shown that also in the absence of inhomogeneous broadening of the resonant line, single-photon wave packets with arbitrary pulse shape m…
We describe an experimental scheme of preparing multipartite W class of maximally entangled states between many atomic ensembles. The scheme is based on laser manipulation of atomic ensembles and single-photon detection, and well fits the status of the current experimental technology. In addition, we show one of the applications of the kind of W class states, teleporting an entangled state of atomic ensembles with unknown coefficients to more than one distant parties, either one of which equally likely receives the transmitted state.
We study the entanglement of the superconducting charge qubit with the quantized electromagnetic field in a microwave cavity. It can be controlled dynamically by a classical external field threading the SQUID within the charge qubit. Utilizing the controllable quantum entanglement, we can demonstrate the dynamic process of the quantum storage of information carried by charge qubit. On the other hand, based on this engineered quantum entanglement, we can also demonstrate a progressive decoherence of charge qubit with quantum jump due to the coupling with the cavity field in quasi-classical stat…
We present an analysis of transfer of quantum information between the collective spin degrees of freedom of a large ensemble of two-level systems and a single central qubit. The coupling between the central qubit and the individual ensemble members may be varied and thus provides access to more than a single storage mode. Means to store and manipulate several independent qubits are derived for the case where the variation in coupling strengths does not allow addressing of orthogonal modes of the ensemble. While our procedures and analysis may apply to a number of different physical systems, fo…
Cold atomic ensembles can mediate the generation of entanglement between pairs of photons. Photons with specific directions of propagation are detected, and the entanglement can reside in any of the degrees of freedom that describe the whole quantum state of the photons: polarization, spatial shape or frequency. We show that the direction of propagation of the generated photons determines the spatial quantum state of the photons and therefore, the amount of entanglement generated. When photons generated in different directions are combined, this spatial distinguishing information can degrade t…
Quantum repeaters based on atomic ensemble quantum memories are promising candidates for achieving scalable distribution of entanglement over long distances. Recently, important experimental progress has been made towards their implementation. However, the entanglement rates and scalability of current approaches are limited by relatively low retrieval and single-photon detector efficiencies. We propose a scheme, which makes use of fluorescent detection of stored excitations to significantly increase the efficiency of connection and hence the rate. Practical performance and possible experimenta…
We describe a general technique that allows for an ideal transfer of quantum correlations between light fields and metastable states of matter. The technique is based on trapping quantum states of photons in coherently driven atomic media, in which the group velocity is adiabatically reduced to zero. We discuss possible applications such as quantum state memories, generation of squeezed atomic states, preparation of entangled atomic ensembles and quantum information processing.
Bernstein and Varizani have given the first quantum algorithm to solve parity problem in which a strong violation of the classical imformation theoritic bound comes about. In this paper, we refine this algorithm with fewer resource and implement a two qubits algorithm in a single query on an ensemble quantum computer for the first time.
We report the storage and retrieval of a small microwave field from a superconducting resonator into collective excitations of a spin ensemble. The spins are nitrogen-vacancy centers in a diamond crystal. The storage time of the order of 30 ns is limited by inhomogeneous broadening of the spin ensemble.
