A weak continuous quantum measurement of an atomic spin ensemble can be implemented via Faraday rotation of an off-resonance probe beam, and may be used to create and probe nonclassical spin states and dynamics. We show that the probe light shift leads to nonlinearity in the spin dynamics and limits the useful Faraday measurement window. Removing the nonlinearity allows a non-perturbing measurement on the much longer timescale set by decoherence. The nonlinear spin Hamiltonian is of interest for studies of quantum chaos and real-time quantum state estimation.
A new approach to the measurement of gravitational fields with an equilibrium ensemble of ultra-cold alkali atoms confined in a cell of volume $V$ is investigated. The proposed model of the gravitational sensor is based on a variation of the density profile of the ensemble due to changing of the gravitational field. For measurement the atomic density variations of the ensemble the electromagnetically induced transparency method is used.
We report on the storage of orbital angular momentum of light in a cold ensemble of cesium atoms. We employ Bragg diffraction to retrieve the stored optical information impressed into the atomic coherence by the incident light fields. The stored information can be manipulated by an applied magnetic field and we were able to observe collapses and revivals due to the rotation of the stored atomic Zeeman coherence for times longer than 15 $μs$.
Recently, atomic ensemble and single photons were successfully entangled by using collective enhancement [D. N. Matsukevich, \textit{et al.}, Phys. Rev. Lett. \textbf{95}, 040405(2005).], where atomic internal states and photonic polarization states were correlated in nonlocal manner. Here we experimentally clarified that in an ensemble of atoms and a photon system, there also exists an entanglement concerned with spatial degrees of freedom. Generation of higher-dimensional entanglement between remote atomic ensemble and an application to condensed matter physics are also discussed.
We characterize correlations in polarization and time of photon pairs generated from a cold cloud of Rb-87 atoms via a four-wave mixing process in a cascade level scheme. Quantum state tomography reveals entangled polarization states of high purity for each of the decay paths through two different intermediate hyperfine levels. When allowing both decay paths, we observe quantum beats in time-resolved correlation measurements.
We consider a scheme of multiplexed cold atomic ensembles that generate a frequency-entangled biphoton state with controllable entropy of entanglement. The biphoton state consists of a telecommunication photon (signal) immediately followed by an infrared one (idler) via four-wave mixing with two classical pump fields. Multiplexing the atomic ensembles with frequency and phase-shifted signal and idler emissions, we can manipulate and control the spectral property of the biphoton state. Mapping out the entropy of entanglement in the scheme provides the optimal configuration for entanglement reso…
To establish an applicable system for advanced quantum information processing between light and atoms, we have demonstrated the quantum non-demolition (QND) measurement with a collective spin of cold ytterbium atoms (171Yb), and observed 1.8 (-1.5, +2.4) dB spin squeezing. Since a 171Yb atom has only a nuclear spin of 1/2 in the ground state, the system is the simplest spin ensemble and robust against decoherence. We used very short pulses with the width of 100 ns, so the interaction time became much shorter than the decoherence time, which is important for multi-step quantum information proce…
We characterize a source of photon pairs based on cascade decay in a cold Rb-87 ensemble. This source is particularly suited to generate of photons for interaction with Rb-87 based atomic systems. We experimentally investigate the dependence of pair generation rate, single photon heralding efficiency, and bandwidth as a function of the number of atoms, detuning and intensity of the pump beams. The observed power and detuning behaviors can be explained by the steady state solution of an established three-level model of an atom. Measurements presented here provide a useful insight on the optimiz…
We report the generation of a macroscopic singlet state in a cold atomic sample via quantum non-demolition (QND) measurement induced spin squeezing. We observe 3 dB of spin squeezing and detect entanglement of up to $5.5\times10^5 $ atoms with $5σ$ statistical significance using a generalized spin squeezing inequality. The degree of squeezing implies at least 50% of the atoms have formed singlets, while the response to a magnetic field gradient indicates entanglement bonds at all length scales, a characteristic of quantum spin liquids.
Cold atomic ensembles can mediate the generation of entanglement between pairs of photons. Photons with specific directions of propagation are detected, and the entanglement can reside in any of the degrees of freedom that describe the whole quantum state of the photons: polarization, spatial shape or frequency. We show that the direction of propagation of the generated photons determines the spatial quantum state of the photons and therefore, the amount of entanglement generated. When photons generated in different directions are combined, this spatial distinguishing information can degrade t…
We theoretically investigate the spectral entanglement of a multiphoton source generated from the cascade emissions in the cascaded cold atomic ensembles.\ This photon source is highly directional, guaranteed under the four-wave mixing condition, and is also highly frequency-correlated due to finite driving pulse durations and superradiant decay constants.\ We utilize Schmidt decomposition to study the bipartite entanglement of the biphoton states projected from the multiphoton ones.\ This entropy of entanglement can be manipulated by controlling the driving parameters and superradiant decay r…
We present a simplified version of a repeater protocol in a cold neutral-atom ensemble with Rydberg excitations optimized for two-node entanglement generation and describe a protocol for quantum teleportation. Our proposal draws from previous proposals [Zhao, {\sl et al.}, Phys. Rev. A {\bf 81}, 052329 (2010)] and [Han, {\sl et al.} Phys. Rev. A {\bf 81}, 052311 (2010)] who described efficient and robust protocols for long-distance entanglement with many nodes. Using realistic experimental values we predict an entanglement generation rate of $\sim$25 Hz and teleportation rate of $\sim$ 5 Hz. O…
Tapered optical fibers with a nanofiber waist are versatile tools for interfacing light and matter. In this context, laser-cooled atoms trapped in the evanescent field surrounding the optical nanofiber are of particular interest: They exhibit both long ground-state coherence times and efficient coupling to fiber-guided fields. Here, we demonstrate electromagnetically induced transparency, slow light, and the storage of fiber-guided optical pulses in an ensemble of cold atoms trapped in a nanofiber-based optical lattice. We measure a slow-down of light pulses to group velocities of 50 m/s. More…
We report on the delay of optical pulses using electromagnetically induced transparency in an ensemble of cold atoms with an optical depth exceeding 500. To identify the regimes in which four-wave mixing impacts on EIT behaviour, we conduct the experiment in both rubidium 85 and rubidium 87. Comparison with theory shows excellent agreement in both isotopes. In rubidium 87, negligible four-wave mixing was observed and we obtained one pulse-width of delay with 50% efficiency. In rubidium 85, four-wave-mixing contributes to the output. In this regime we achieve a delay-bandwidth product of 3.7 at…
We study the conditions for generating spin squeezing via a quantum non-demolition measurement in an ensemble of cold 87Rb atoms. By considering the interaction of atoms in the 5S_{1/2}(F=1) ground state with probe light tuned near the D2 transition, we show that, for large detunings, this system is equivalent to a spin-1/2 system when suitable Zeeman substates and quantum operators are used to define a pseudo-spin. The degree of squeezing is derived for the rubidium system in the presence of scattering causing decoherence and loss. We describe how the system can decohere and lose atoms, and p…
We investigate the spectral properties of the biphoton state from the cascade emissions of cold atomic ensembles, which composes of a telecommunication photon (signal) followed by an infrared one (idler) via four-wave mixing.\ With adiabatic conditions for Gaussian driving pulses of width $τ$, the spectrum of the biphoton state has the form of a Gaussian that conserves signal and idler photon energies within $\hbar/τ$ modulated by a Lorentzian with a superradiant linewidth.\ Multiplexing the atomic ensembles with frequency-shifted cascade emissions, we may manipulate and shape the spectrum of …
Quantum memory is one of key ingredients consisting of quantum networks, therefore storing light at single photon level is an important step for realizing quantum networks. A photon, encoded in a high-dimensional state, can significantly increase the information capacity that a photon can carry. Furthermore, quantum memories with the ability to store multiple optical modes offer advantages in speed and robustness over single mode memories in quantum communication and computation. So far, there is no any report about the storage and retrieval of multiple mode images at single photon level. Here…
We observe and measure dispersive optical non-linearities in an ensemble of cold Rydberg atoms placed inside an optical cavity. The experimental results are in agreement with a simple model where the optical non-linearities are due to the progressive appearance of a Rydberg blockaded volume within the medium. The measurements allow a direct estimation of the "blockaded fraction" of atoms within the atomic ensemble.
We show that atomic motion leads not only to noticeable quantitative, but in some cases also to qualitative modification of collective effects in dense and cold atomic ensembles even in the case when the characteristic Doppler shifts are tens of times smaller than the natural linewidth. The observed influence is explained as a result of the suppression of the impact of sub-radiant collective states caused by the displacement of the atoms.
We calculate the differential cross section of polarized light scattering from a cold and dense atomic ensemble. The regularities in the transformation of the cross section when increasing the size of the atomic ensemble are analyzed numerically. We show that for typical experimental conditions, an approximate scaling law can be obtained. Very good agreement is found in a comparison with experimental data on the size dependence of a dense and cold cloud of 87$Rb atoms.
We observe narrowband pairs of time-correlated photons of wavelengths 776\,nm and 795\,nm from non-degenerate four-wave mixing in a laser-cooled atomic ensemble of $^{87}${Rb} using a cascade decay scheme. Coupling the photon pairs into single mode fibers, we observe an instantaneous rate of 7700 pairs per second with silicon avalanche photodetectors, and an optical bandwidth below 30\,MHz. Detection events exhibit a strong correlation in time ($g^{(2)}(τ=0)\approx5800$), and a high coupling efficiency indicated by a pair-to-single ratio of 23%. The violation of the Cauchy-Schwarz inequality b…
The reversible transfer of the quantum information between a photon, an information carrier, and a quantum memory with high fidelity and reliability is the prerequisite for realizing a long-distance quantum communication and a quantum network. Encoding photons into higher-dimensional states could significantly increase their information-carrying capability and network capacity. Moreover, the large-alphabet quantum key distribution affords a more secure flux of information. Quantum memories have been realized in different physical systems, such as atomic ensembles and solid systems etc., but to…
We demonstrate a cooperative optical non-linearity caused by dipolar interactions between Rydberg atoms in an ultra-cold atomic ensemble. By coupling a probe transition to the Rydberg state we map the strong dipole-dipole interactions between Rydberg pairs onto the optical field. We characterize the non-linearity as a function of electric field and density, and demonstrate the enhancement of the optical non-linearity due to cooperativity.
An important step towards the successful development of network that allows the distribution of quantum information is the storage of light in a matter at the single-photon level. Encoding photons in high-dimensional photonic states can significantly increase their information-carrying capacity. So far, there is no any report on the storage of an image at true single photon level, realizing a quantum memory that can record the shape of a single photon is a challenging work. In this work, we report on the first experimental realization of storing a true single photon carrying an orbital angular…
We propose the use of Rydberg interactions and ensembles of cold atoms in mixed state for the implementation of a protocol for deterministic quantum computation with one quantum bit (DQC1) that can be readily operated in high dimensional Hilbert spaces. We propose an experimental test for the scalability of the protocol and to study the physics of discord. Furthermore we develop a scheme to add control to non-trivial unitaries that will enable the study of many-body physics with ensembles in mixed states.
Quantum memory for flying optical qubits is a key enabler for a wide range of applications in quantum information science and technology. A critical figure of merit is the overall storage-and-retrieval efficiency. So far, despite the recent achievements of efficient memories for light pulses, the storage of qubits has suffered from limited efficiency. Here we report on a quantum memory for polarization qubits that combines an average conditional fidelity above 99% and an efficiency equal to (68$\pm$ 2)%, thereby demonstrating a reversible qubit mapping where more information is retrieved than …
Interfacing superconducting qubits with optical photons requires noise-free microwave-to-optical transducers, a technology currently not realized at the single-photon level. We propose to use four-wave-mixing in an ensemble of cold ytterbium (Yb) atoms prepared in the metastable 'clock' state. The parametric process uses two high-lying Rydberg states for bidirectional conversion between a 10 GHz microwave photon and an optical photon in the telecommunication E-band. To avoid noise photons due to spontaneous emission, we consider continuous operation far detuned from the intermediate states. We…
We present a detailed, realistic proposal and analysis of the implementation of a cold atom deflector using time-dependent far off-resonance optical guides. An analytical model and numerical simulations are used to illustrate its characteristics when applied to both non-degenerate atomic ensembles and to Bose-Einstein condensates. Using for all relevant parameters values that are achieved with present technology, we show that it is possible to deflect almost entirely an ensemble of $^{87}$Rb atoms falling in the gravity field. We discuss the limits of this proposal, and illustrate its robustne…
We demonstrate a dual-axis accelerometer and gyroscope atom interferometer, which forms the building blocks of a six-axis inertial measurement unit. By recapturing the atoms after the interferometer sequence, we maintain a large atom number at high data-rates of 50 to 100 measurements per second. Two cold ensembles are formed in trap zones located a few centimeters apart, and are launched toward one-another. During their ballistic trajectory, they are interrogated with a stimulated Raman sequence, detected, and recaptured in the opposing trap zone. We achieve sensitivities at $\mathrm{μ\mathit…
Highly stable laser sources based on narrow atomic transitions provide a promising platform for direct generation of stable and accurate optical frequencies. Here we investigate a simple system operating in the high-temperature regime of cold atoms. The interaction between a thermal ensemble of $^{88}$Sr at mK temperatures and a medium-finesse cavity produces strong collective coupling and facilitates high atomic coherence which causes lasing on the dipole forbidden $^1$S$_0 \leftrightarrow ^3$P$_1$ transition. We experimentally and theoretically characterize the lasing threshold and evolution…
We study electromagnetically induced transparency (EIT) of a weakly interacting cold Rydberg gas. We show that the onset of interactions is manifest as a depopulation of the Rydberg state and numerically model this effect by adding a density-dependent non-linear term to the optical Bloch equations. In the limit of a weak probe where the depopulation effect is negligible, we observe no evidence of interaction induced decoherence and obtain a narrow Rydberg dark resonance with a linewidth of <600 kHz, limited by the Rabi frequency of the coupling beam
We present a toolbox for cold atom manipulation with time-dependent magnetic fields generated by an atom chip. Wire layouts, detailed experimental procedures and results are presented for the following experiments: Use of a magnetic conveyor belt for positioning of cold atoms and Bose-Einstein condensates with a resolution of two nanometers; splitting of thermal clouds and BECs in adjustable magnetic double well potentials; controlled splitting of a cold reservoir. The devices that enable these manipulations can be combined with each other. We demonstrate this by combining reservoir splitter a…
A simplified theory for the wavepackets of the photons emitted during the read process of a quantum memory formed by cold atoms is provided. We arrive at analytical expressions for the single- and double-photon emissions, evidencing superradiant features in both cases. In the two-photon case, both photons are emitted in the same spatiotemporal mode, characterizing a superradiant emission of a Fock state of light with two excitations. Experiments confirm the theoretical predictions with a satisfactory agreement.
We observe an optical filtering effect in four-wave mixing (FWM) process based on a cold atomic gas. The side peaks appear at the edges of pulse of generated optical field, and they propagate through the atomic media without absorption. The theoretical analysis shows that these side peaks corresponded to the high frequency part of pulse of generated signal, which means the atoms cannot response to the rapid change of the electromagnetic field in time. On the contrary, the low frequency components of generated signal are absorbed during the transmission through the atoms. In addition, we experi…
We use optical tweezers based on time-multiplexed acousto-optic deflectors to trap ultra-cold cesium atoms in one-dimensional arrays of atomic ensembles. For temperatures between 2.5 $μ$K and 50 nK we study the maximal time between optical tweezer pulses that retains the number of atoms in a single trap. This time provides an estimate on the maximal number of sites in an array of time-multiplexed optical tweezers. We demonstrate evaporative cooling of atoms in arrays of up to 25 optical tweezer traps and the preparation of atoms in a box potential. Additionally, we demonstrate three different …
Planar squeezed states, i.e. quantum states which are squeezed in two orthogonal spin components, have recently attracted attention due to their applications in atomic interferometry and quantum information [Q. Y. He et al, New J. Phys. 14, 093012 (2012)]. While canonical variables such as quadratures of the radiation field can be squeezed in at most one component, simultaneous squeezing in two orthogonal spin components can be achieved due to the angular momentum commutation relations. We present a novel scheme for planar squeezing via quantum non-demolition (QND) measurements in spin-1 syste…
Interfacing fundamentally different quantum systems is key to build future hybrid quantum networks. Such heterogeneous networks offer superior capabilities compared to their homogeneous counterparts as they merge individual advantages of disparate quantum nodes in a single network architecture. However, only very few investigations on optical hybrid-interconnections have been carried out due to the high fundamental and technological challenges, which involve e.g. wavelength and bandwidth matching of the interfacing photons. Here we report the first optical quantum interconnection between two d…
We discuss the evolution of the quantum state of an ensemble of atoms that are coupled via a single propagating optical mode. We theoretically show that the quantum state of N atoms, which are initially prepared in the timed Dicke state, evolves through all the N - 1 states that are subradiant with respect to the propagating mode. We predict this process to occur for any atom number and any atom-light coupling strength. These findings are supported by measurements performed with cold cesium atoms coupled to the evanescent field of an optical nanofiber. We experimentally observe the evolution o…
We experimentally and theoretically investigate collective radiative effects in an ensemble of cold atoms coupled to a single-mode optical nanofiber. Our analysis unveils the microscopic dynamics of the system, showing that collective interactions between the atoms and a single guided photon gradually build-up along the atomic array in the direction of propagation of light. These results are supported by time-resolved measurements of the light transmitted and reflected by the ensemble after excitation via nanofiber-guided laser pulses, whose rise and fall times are shorter than the atomic life…
The spatial modes of light, carrying a quantized amount of orbital angular momentum (OAM), is one of the excellent candidates that provides access to high-dimensional quantum states, which essentially makes it promising towards building high-dimensional quantum networks. In this paper, we report the storage and retrieval of photonic qubits encoded with OAM state in the cold atomic ensemble, achieving an average conditional fidelity above 98% and retrieval efficiency around 65%. The photonic OAM qubits are encoded with weak coherent states at the single-photon level and the memory is based on e…
We demonstrate a coherent and dynamic beam splitter based on light storage in cold atoms. An input weak laser pulse is first stored in a cold atom ensemble via electromagnetically-induced transparency (EIT). A set of counter-propagating control fields, applied at a later time, retrieves the stored pulse into two output spatial modes. The high visibility interference between the two output pulses clearly demonstrates that the beam splitting process is coherent. Furthermore, by manipulating the control lasers, it is possible to dynamically control the storage time, the power splitting ratio, the…
Quantum memories are an integral component of quantum repeaters - devices that will allow the extension of quantum key distribution to communication ranges beyond that permissible by passive transmission. A quantum memory for this application needs to be highly efficient and have coherence times approaching a millisecond. Here we report on work towards this goal, with the development of a $^{87}$Rb magneto-optical trap with a peak optical depth of 1000 for the D2 $F=2 \rightarrow F'=3$ transition using spatial and temporal dark spots. With this purpose-built cold atomic ensemble to implement t…
Effective and unrestricted engineering of atom-photon interactions requires precise spatially-resolved control of light beams. The significant potential of such manipulations lies in a set of disciplines ranging from solid state to atomic physics. Here we use a Zeeman-like ac-Stark shift of a shaped laser beam to perform rotations of spins with spatial resolution in a large ensemble of cold rubidium atoms. We show that inhomogeneities of light intensity are the main source of dephasing and thus decoherence, yet with proper beam shaping this deleterious effect is strongly mitigated allowing rot…
The strong demand for quantum memory, a key building block of quantum network, has inspired new methodologies and led to experimental progress for quantum storage. The use of quantum memory for spatial multimode or image storage could dramatically increase the channel bit-rate. Furthermore, quantum memory that can store multiple optical modes would lead to higher efficiencies in quantum communication and computation. Here, by using resonant tripod electromagnetically induced transparency in a cold atomic ensemble, we experimentally demonstrate multiple probes storage in frequency domain, where…
On the basis of our general theoretical results developed previously in JETP 112, 246 (2011), we calculate the spatial distribution of atoms excited in a dense and cold atomic cloud by weak monochromatic light. We also study the atomic distribution over different Zeeman sublevels of the excited state in different parts of the cloud. The dependence of this distribution of atomic excitation on the density of the atomic ensemble and the frequency of external emission is investigated. We show that in the boundary regions of the cloud the orientation and alignment of atomic angular momentum takes p…
We study the emergence of collective scattering in the presence of dipole-dipole interactions when we illuminate a cold cloud of rubidium atoms with a near-resonant and weak intensity laser. The size of the atomic sample is comparable to the wavelength of light. When we gradually increase the atom number from 1 to 450, we observe a broadening of the line, a small red shift and, consistently with these, a strong suppression of the scattered light with respect to the noninteracting atom case. Numerical simulations, which include the internal atomic level structure, agree with the data.
The combination of electromagnetically induced transparency (EIT) with the nonlinear interaction between Rydberg atoms provides an effective interaction between photons. In this paper, we investigate the storage of optical pulses as collective Rydberg atomic excitations in a cold atomic ensemble. By measuring the dynamics of the stored Rydberg polaritons, we experimentally demonstrate that storing a probe pulse as Rydberg polaritons strongly enhances the Rydberg mediated interaction compared to the slow propagation case. We show that the process is characterized by two time scales. At short st…
The coupling of weak light fields to Rydberg states of atoms under conditions of electromagnetically induced transparency (EIT) leads to the formation of Rydberg polaritons which are quasi-particles with tunable effective mass and long-range interactions. Confined to one spatial dimension their low energy physics is that of a moving-frame Luttinger liquid which due to the long-range character of the repulsive interaction can form a Wigner crystal. We calculate the Luttinger $K$ parameter using density-matrix renormalization group (DMRG) simulations and find that under typical slow-light condit…
We experimentally characterize the optical nonlinear response of a cold atomic medium placed inside an optical cavity, and excited to Rydberg states. The excitation to S and D Rydberg levels is carried out via a two-photon transition in an EIT (electromagnetically induced transparency) configuration, with a weak (red) probe beam on the lower transition, and a strong (blue) coupling beam on the upper transition. The observed optical nonlinearities induced by S states for the probe beam can be explained using a semi-classical model with van der Waals' interactions. For the D states, it appears n…
