Measurement of photon-number statistics of fields composed of photon pairs generated in spontaneous parametric downcoversion pumped by strong ultrashort pulses is described. Final detection quantum efficiencies, noises as well as possible loss of one or both photons from a pair are taken into account. Measured data provided by an intensified single-photon CCD camera are analyzed along the developed model. The joint signal-idler photon-number distribution is obtained using the expectation maximization algorithm. Covariance of the signal and idler photon-numbers equals 80 %. Statistics of the generated photon pairs are identified to be Poissonian in our case. Distribution of the integrated intensities of the signal and idler fields shows strong correlations between the fields. Negative values of this distribution occurring in some regions clearly demonstrate a nonclassical character of the light composed of photon pairs.
We show experimentally how noncollinear geometries in spontaneous parametric downconversion induce ellipticity of the shape of the spatial mode function. The degree of ellipticity depends on the pump beam width, especially for highly focused beams. We also discuss the ellipticity induced by the spectrum of the pump beam.
We present an experimental proposal for the generation of photon triplets based on third-order spontaneous para- metric downconversion in thin optical fibers. Our analysis includes expressions for the quantum state, which de- scribes the photon triplets and for the generation rate in terms of all experimental parameters. We also present, for a specific source design, numerically calculated generation rates.
Spontaneous parametric downconversion is an essential technique in quantum optics experiments. In this paper, various quasi-phase-matching processes in several typical periodically polarized nonlinear materials are analyzed and calculated. Furthermore, a general method for realizing multiple types of quasi-phase-matching in a monolithic material is presented. Finally, a novel design to prepare multiple entangled photon pairs based on the Sagnac interferometer is discussed. This technology can be applied to tiny optical paths in the telecom C band, saving both cost and space.
We study the chronocyclic character, i.e. the joint temporal and spectral properties, of the single-photon constituents of photon pairs generated by spontaneous parametric down conversion. In particular we study how single photon properties, including purity and single-photon chirp, depend on photon pair properties, including the type of signal-idler spectral and correlations and the level of pump chirp.
A class of centrosymmetric molecules support excitons with a well-defined quasi-angular momentum. Cofacial arrangements of these molecules can be engineered so that quantum cutting produces a pair of excitons with angular momenta that are maximally entangled. The Bell state constituents can subsequently travel in opposite directions down molecular chains as ballistic wave packets. This is a direct excitonic analog to the entangled polarization states produced by the spontaneous parametric downconversion of light. As in optical settings, the ability to produce Bell states should enable foundati…
In this paper we study photon pairs generated in a nonlinear cavity, composed of a nonlinear crystal surrounded by mirrors, by the process of spontaneous parametric downconversion. We analyze two different regimes: singly-resonant cavities where the signal and idler modes are resonant, and doubly-resonant cavities where the pump mode is also resonant. We present analytic expressions for the joint spectral amplitude in these two cases, and study the reduction in emission bandwidth as the cavity coefficient finesse is increased. We also study the enhancement of the source brightness resulting fr…
We study the conditional preparation of single photons based on parametric downconversion, where the detection of one photon from a given pair heralds the existence of a single photon in the conjugate mode. We derive conditions on the modal characteristics of the photon pairs, which ensure that the conditionally prepared single photons are quantum-mechanically pure. We propose specific experimental techniques that yield photon pairs ideally suited for single-photon conditional preparation.
We address the intrinsic multimode nature of the quantum state of light obtained by pulsed spontaneous parametric downconversion and develop a theoretical model based only on experimentally accessible quantities. We exploit the pairwise entanglement as a resource for conditional multimode measurements and derive closed formulas for the detection probability and the density matrix of the conditional states. We present a set of experiments performed to validate our model in different conditions that are in excellent agreement with experimental data. Finally, we evaluate nonGaussianity of the con…
For advanced quantum information technology, sources of photon pairs in quantum mechanically factorable states are of great importance for realizing high-fidelity photon-photon quantum gate operations. Here we experimentally demonstrate a technique to produce spectrally factorable photon pairs utilizing multi-order quasi-phase-matching (QPM) conditions in spontaneous parametric downconversion (SPDC). In our scheme, a spatial nonlinearity profile of a nonlinear optical crystal is shaped with current standard poling techniques, and the associated phase-matching function can be approximated to a …
Spontaneous parametric downconversion is the primary source to generate entangled photon pairs in quantum photonics laboratories. Depending on the experimental design, the generated photon pairs can be correlated in the frequency spectrum, polarisation, position-momentum, and spatial modes. Exploring the spatial modes' correlation has hitherto been limited to the polar coordinates' azimuthal angle, and a few attempts to study Walsh modes radial states. Here, we study the full-mode correlation, on a Laguerre-Gauss basis, between photon pairs generated in a type-I crystal. Furthermore, we explor…
We report on the generation of an indistinguishable heralded single-photon state, using highly nondegenerate spontaneous parametric downconversion (SPDC). Spectrally factorable photon pairs can be generated by incorporating a broadband pump pulse and a group-velocity matching (GVM) condition in a periodically-poled potassium titanyl phosphate (PPKTP) crystal. The heralding photon is in the near IR, close to the peak detection efficiency of off-the-shelf Si single-photon detectors; meanwhile, the heralded photon is in the telecom L-band where fiber losses are at a minimum. We observe spectral f…
Parametric downconversion (PDC) in semiconductor Bragg-reflection waveguides (BRW) is routinely exploited for photon-pair generation in the telecommunication range. Contrary to many conventional PDC sources, BRWs offer possibilities to create spectrally broadband but nevertheless indistinguishable photon pairs in orthogonal polarizations that simultaneously incorporate high frequency entanglement. We explore the characteristics of co-propagating twin beams created in a type-II ridge BRW. Our PDC source is bright and efficient, which serves as a benchmark of its performance and justifies its ex…
In this paper we show that by suitably tailoring the dispersion characteristics of a Bragg reflection waveguide (BRW) mode, it is possible to achieve efficient photon pair generation over a large pump bandwidth while maintaining narrow signal bandwidth. The structure proposed consists of a high index core BRW with a periodically poled GaN core and periodically stratified cladding made up of alternate layers of $Al_{0.02}Ga_{0.98}N$ and $Al_{0.45}Ga_{0.55}N$. Such photon-pair generators should find applications in realizing compact and stable sources for quantum information processing.
Parametric downconversion (PDC) is a technique of ubiquitous experimental significance in the production of non-classical, photon-number correlated twin beams. Standard theory of PDC as a two-mode squeezing process predicts and homodyne measurements observe a thermal photon number distribution per beam. Recent experiments have obtained conflicting distributions. In this paper, we explain the observation by an a-priori theoretical model solely based on directly accessible physical quantities. We compare our predictions with experimental data and find excellent agreement.
We show that the states generated by a three-mode spontaneous parametric downconversion (SPDC) interaction Hamiltonian possess tripartite entanglement of a different nature to other paradigmatic three-mode entangled states generated by the combination of two-mode SPDCs interactions. While two-mode SPDC generates gaussian states whose entanglement can be characterized by standard criteria based on two-mode quantum correlations, these criteria fail to capture the entanglement generated by three-mode SPDC. We use criteria built from three-mode correlation functions to show that the class of state…
We demonstrate sub-shot-noise photon-number correlations in a (temporal) multimode mesoscopic ($\sim 10^3$ detected photons) twin-beam produced by ps-pulsed spontaneous non-degenerate parametric downconversion. We have separately detected the signal and idler distributions of photons collected in twin coherence areas and found that the variance of the photon-count difference goes below the shot-noise limit by 3.25 dB. The number of temporal modes contained in the twin-beam, as well as the size of the twin coherence areas, depends on the pump intensity. Our scheme is based on spontaneous downco…
We present a simple treatment for the phenomenon of parametric downconversion considering the coherent scattering of one pump photon into a photon pair by a nonlinear crystal. The energy and momentum entanglement of the quantum state of the generated twin photons are seen as a consequence of the fundamental indistinguishability of the time and the position in which the photon pair is created inside the crystal. We also discuss some consequences of the system entanglement.
Device-independent quantum key distribution (DIQKD) guarantees unconditional security of secret key without making assumptions about the internal workings of the devices used. It does so using the loophole-free violation of a Bell's inequality. The primary challenge in realizing DIQKD in practice is the detection loophole problem that is inherent to photonic tests of Bell's inequalities over lossy channels. We revisit the proposal of Curty and Moroder [Phys. Rev. A 84, 010304(R) (2011)] to use a linear optics-based entanglement-swapping relay (ESR) to counter this problem. We consider realisti…
Optical downconversion is a key resource for generating nonclassical states. Very recently, direct nondegenerate triple-photon spontaneous downconversion (NTPSD) with bright photon triplets and strong third-order correlations has been demonstrated in a superconducting device (2020 Phys. Rev. X 10 011011). Besides, linear and nonlinear tripartite entanglement in this process have also been predicted (2018 Phys. Rev. Lett. 120 043601; 2020 Phys. Rev. Lett. 125 020502). In this paper, we consider the generation of nonclassical optical quantum superpositions and investigate nonlinear quantum steer…
We study the properties of bi-squeezed tripartite Gaussian states created by two spontaneous parametric down-conversion processes that share a common idler. We give a complete description of the quantum correlations across of all partitions, as well as of the genuine multipartite entanglement, obtaining analytical expressions for most of the quantities of interest. We find that the state contains genuine tripartite entanglement, in addition to the bipartite entanglement among the modes that are directly squeezed. We also investigate the effect of homodyne detection of the photons in the common…
The temperature dependence of the refractive indices of potassium titanyl phosphate (KTP) are shown to enable quasi-phasematched type II spontaneous parametric downconversion (SPDC) with low temperature sensitivity. Calculations show the effect to be maximised for emission of photons at around 1165nm, as well as producing potentially useful regions for wavelengths throughout the telecommunications bands. We demonstrate the effect experimentally, observing temperature-insensitive degenerate emission at 1326nm, within the telecommunications O band. This result has practical applications in the d…
We present a theoretical and experimental analysis of the joint effects of the transverse electric field distribution and of the nonlinear crystal characteristics on the properties of photon pairs generated by spontaneous parametric downconversion (SPDC). While it is known that for a sufficiently short crystal the pump electric field distribution fully determines the joint signal-idler properties, for longer crystals the nonlinear crystal properties also play an important role. In this paper we present experimental measurements of the angular spectrum (AS) and of the conditional angular spectr…
We derive frequency correlation and exit probability expressions for photons generated via spontaneous parametric downconversion (SPDC) in nonlinear waveguides that exhibit linear scattering loss. Such loss is included within a general Hamiltonian formalism by connecting waveguide modes to reservoir modes with a phenomenological coupling Hamiltonian, the parameters of which are later related to the usual loss coefficients. In the limit of a low probability of SPDC pair production, the presence of loss requires that we write the usual lossless generated pair state as a reduced density operator,…
We interface a spontaneous parametric down conversion (SPDC) crystal and a cold atomic ensemble and demonstrate a highly efficient quantum memory through polarization-encoded single-photon qubits. Specifically, narrowband heralded single photons from a cavity-enhanced SPDC source is stored using cold atomic ensemble, with ~70% storage-and-retrieval efficiency and ~10$μ$s storage time at 50% efficiency. To prevent the degradation after storage, we also manipulate the single-photon wave profile so that the retrieved non-classical nature of single photon is preserved. On the other hand, the dual-…
Heralded single photon sources are often implemented using spontaneous parametric downconversion, but their quality can be restricted by optical loss, double pair emission and detector dark counts. Here, we show that the performance of such sources can be improved using cascaded downconversion, by providing a second trigger signal to herald the presence of a single photon, thereby reducing the effects of detector dark counts. We find that for a setup with fixed detectors, an improved heralded second-order correlation function $g^{(2)}$ can always be achieved with cascaded downconversion given …
We report spontaneous parametric downconversion having an unusually wide spectral bandwidth. A collinear type-1 phase-matching configuration is employed with degeneracy near the zero group velocity dispersion frequency. With a spectral width of 1080 nm and degenerate wavelength 1885 nm, the source also emits a high flux of photon pairs constrained to a cone of only 2 degree half-angle. A rigorous theoretical approach is developed that confirms the experimental observations. The source properties are consistent with an ultra-short photon-pair correlation time and, for a narrowband pump, extreme…
What are the orbital angular momentum correlations between spatially entangled photon pairs generated in spontaneous parametric down-conversion? We show that the answer to this question can be given in two alternative, although complementary, ways. The answer posed in this letter explains satisfactorily the seemingly contradictory results obtained in different experiments, and theoretical approaches.
The measurement of joint signal-idler photon-number distribution of a field obtained from spontaneous parametric downconversion using an intensified CCD camera is presented. It is shown that a classicality criterion is violated directly by the measured data. Characteristic dimensions of the area of correlation are determined in the same experimental setup.
We study the joint spectral properties of photon pairs generated by spontaneous parametric down-conversion in a one-dimensional nonlinear photonic crystal in a collinear, degenerate, type-II geometry. We show that the photonic crystal properties may be exploited to compensate for material dispersion and obtain photon pairs that are nearly factorable, in principle, for arbitrary materials and spectral regions, limited by the ability to fabricate the nonlinear crystal with the required periodic variation in the refractive indices for the ordinary and extraordinary waves.
This paper presents the general Schmidt decomposition of two-photon fields generated in spontaneous parametric down-conversion (SPDC). It discusses in particular the separation of the radial and azimuthal degrees of freedom, the role of projection in modal analysis, and the benefits of collinear phase mismatch. The paper is written in a review style and presents a wealth of numerical results. It aims at emphasising the physics beyond the mathematics, through discussions and graphical representations of key results.
We discuss a novel method of efficiently producing multi-photon states using repeated spontaneous parametric downconversion. Specifically, by attempting downconversion several times, we can pseudo-deterministically add photons to a mode, producing various several-photon states. We discuss both expected performance and experimental limitations.
Alternative theories to quantum mechanics motivate important fundamental tests of our understanding and descriptions of the smallest physical systems. Here, using spontaneous parametric downconversion as a heralded single-photon source, we place experimental limits on a class of alternative theories, consisting of classical field theories which result in power-dependent normalized correlation functions. In addition, we compare our results with standard quantum mechanical interpretations of our spontaneous parametric downconversion source over an order of magnitude in intensity. Our data match …
We show the equivalence between two different communication schemes that employ a couple of modes of the electromagnetic field. One scheme uses unconventional heterodyne detection, with correlated signal and image-band modes in a twin-beam state from parametric downconversion. The other scheme is realized through a complex-number coding over quadrature-squeezed states of two uncorrelated modes, each detected by ordinary homodyning. This equivalence concerns all the stages of the communication channel: the encoded state, the optimal amplifier for the channel, the master equation modeling the lo…
We present a study of the effects of dispersion on the properties of photon pairs generated by type-II, collinear spontaneous parametric downconversion. Specifically, we take into consideration the effects of a chirped pump, as well as of dispersive propagation of the photon pairs. We present expressions for the joint amplitude both in the spectral and temporal domains, as well as for the chronocyclic Wigner function of heralded single photons, which fully characterizes the single photon spectral (temporal) properties. On the one hand, we show that unwanted effects of pump chirp in terms of th…
Spontaneous parametric downconversion (SPDC) has been a key enabling technology in exploring quantum phenomena and their applications for decades. For instance, traditional SPDC, which splits a high energy pump photon into two lower energy photons, is a common way to produce entangled photon pairs. Since the early realizations of SPDC, researchers have thought to generalize it to higher order, e.g., to produce entangled photon triplets. However, directly generating photon triplets through a single SPDC process has remained elusive. Here, using a flux-pumped superconducting parametric cavity, w…
Correlations in twin beams composed of many photon pairs are studied using an intensified CCD camera. Joint signal-idler photon-number distribution and quantum phase-space quasi-distributions determined from experimental data have nonclassical features.
We present a novel yet simple approach to produced multiple entangled photon pairs through spontaneous parametric downconversion. We have developed Gaussian masks to subdivide the pump beam before passing it through a nonlinear medium. In this way, we are able to observe simultaneous separate down-converted emission cones with spatial overlap. The technique we employ can be used to greatly increase the dimensionality of entangled photonic systems generated from spontaneous parametric down conversion, affording greater scalability to optical quantum computing than previously explored.
We study the process of seeded, or stimulated, third-order parametric down-conversion, as an extension of our previous work on spontaneous parametric downconversion (TOSPDC). We present general expressions for the spectra and throughputs expected for the cases where the seed field or fields overlap either only one or two of the TOSPDC modes, and also allow for both pump and seed to be either monochromatic or pulsed. We present a numerical study for a particular source design, showing that doubly-overlapped seeding can lead to a considerably greater generated flux as compared with singly-overla…
We report a simple scheme for direct generation of frequency-bin entangled photon pairs via spontaneous parametric downconversion. Our fabricated nonlinear optical crystal with two different poling periods can simultaneously satisfy two different, spectrally symmetric nondegenerate quasi-phase-matching conditions, enabling the direct generation of entanglement in two discrete frequency-bin modes. Our produced photon pairs exhibited Hong-Ou-Mandel interference with high-visibility beating oscillations, a signature of two-mode frequency-bin entanglement. Moreover, we demonstrate deterministic en…
Spontaneous parametric down-conversion (SPDC) is widely used in quantum applications based on photonic entanglement. The efficiency of photon pair generation is often characterized by means of a $sinc(LΔk/2)$-function, where $L$ is the length of the nonlinear medium and $Δk$ the phase mismatch between the pump and down-converted fields. In theoretical investigations, the \textit{sinc} behavior of the phase mismatch has often been approximated by a Gaussian function $\exp{(-αx^2)}$ in order to derive analytical expressions for the SPDC process. Different values have been chosen in the literatur…
We study the Bloch-Messiah reduction of parametric downconversion of light in the pulsed regime with a nondegenerate phase matching providing generation of twin beams. We find that in this case every squeezing eigenvalue has multiplicity at least two. We discuss the problem of ambiguity in the definition of the squeezing eigenmodes in this case and develop two approaches to unique determination of the latter. First, we show that the modal functions of the squeezing eigenmodes can be tailored from the Schmidt modes of the signal and idler beams. Alternatively, they can be found as a solution of…
Optical parametric downconversion has proven to be a valuable source of nonclassical light. The process is inherently able to produce twin beam correlations along with individual intensity squeezing of either parametric beam, when pumped far above threshold. Here, we present for the first time the direct observation of intensity squeezing of -1.2 dB of each of the individual parametric beams in parametric downconversion by use of a high quality whispering gallery mode disk resonator. In addition we observed twin beam quantum correlations of -2.7 dB with this cavity. Such resonators feature str…
Coherence-domain imaging systems can be operated in a single-photon counting mode, offering low detector noise; this in turn leads to increased sensitivity for weak light sources and weakly reflecting samples. We have demonstrated that excellent axial resolution can be obtained in a photon-counting coherence domain imaging (CDI) system that uses light generated via spontaneous parametric down-conversion (SPDC) in a chirped periodically poled stoichiometric lithium tantalate (chirped-PPSLT) structure, in conjunction with a niobium nitride superconducting single-photon detector (SSPD). The bandw…
An important step for photonic quantum technologies is the demonstration of a quantum advantage through boson sampling. In order to prevent classical simulability of boson sampling, the photons need to be almost perfectly identical and almost without losses. These two requirements are connected through spectral filtering, improving one leads to a decrease of the other. A proven method of generating single photons is spontaneous parametric downconversion (SPDC). We show that an optimal trade-off between indistinguishability and losses can always be found for SPDC. We conclude that a 50-photon s…
Hyperentangled photonic states - exhibiting nonclassical correlations in several degrees of freedom - offer improved performance of quantum optical communication and computation schemes. Experimentally, a hyperentanglement of transverse-wavevector and spectral modes can be obtained in a straightforward way with multimode parametric single-photon sources. Nevertheless, experimental characterization of such states remains challenging. Not only single-photon detection with high spatial resolution - a single-photon camera - is required, but also a suitable mode-converter to observe the spectral/te…
We study the processes of spontaneous four wave mixing and of third-order spontaneous parametric downconversion in optical fibers, as the basis for the implementation of photon-pair and photon-triplet sources. We present a comparative analysis of the two processes including expressions for the respective quantum states and plots of the joint spectral intensity, a discussion of phasematching characteristics, and expressions for the conversion efficiency. We have also included a comparative study based on numerical results for the conversion efficiency for the two sources, as a function of sever…
Heralding of single photon at 1550 nm from pump pulsed non degenerate spontaneous parametric downconversion is demonstrated. P(1) and P(2) of our source are 0.1871 and 2.4 x 10 ^-3 respectively. Triggering of our source is 2.16 x 10^5 trigger.s^-1. This source may be used in QKD system.
We experimentally demonstrate a method to control the relative amount of quantum and classical energy correlations between two photons from a pair emitted by spontaneous parametric downconversion. Decoherence in the energy basis is achieved by applying random spectral phases on the photons. As a consequence a diverging temporal second order correlation function is observed and is explained by a mixture between an energy entangled pure state and a fully classically correlated mixte state.
We propose and implement a novel method to produce a spatial anti-bunched field with free propagating twin beams from spontaneous parametric down-conversion. The method consists in changing the spatial propagation by manipulating the transverse degrees of freedom through reflections of one of the twin beams. Our method use reflective elements eliminating losses from absorption by the objects inserted in the beams.
The measurement of photon-number statistics of fields composed of photon pairs, generated in spontaneous parametric down-conversion and detected by an intensified CCD camera is described. Final quantum detection efficiencies, electronic noises, finite numbers of detector pixels, transverse intensity spatial profiles of the detected beams as well as losses of single photons from a pair are taken into account in a developed general theory of photon-number detection. The measured data provided by an iCCD camera with single-photon detection sensitivity are analyzed along the developed theory. Join…
A non-classical light source emitting pairs of identical photons represents a versatile resource of interdisciplinary importance with applications in quantum optics and quantum biology. Emerging research fields, which benefit from such type of quantum light source, include quantum-optical spectroscopy or experiments on photoreceptor cells sensitive to photon statistics. To date, photon twins have mostly been generated using parametric downconversion sources, relying on Poissonian number distributions, or atoms, exhibiting low emission rates. Here, we propose and experimentally demonstrate the …
We present a tunable, frequency-stabilized, narrow-bandwidth source of frequency-degenerate, entangled photon pairs. The source is based on spontaneous parametric downconversion (SPDC) in periodically-poled KTiOPO4 (PPKTP). Its wavelength can be stabilized to 850 or 854 nm, thus allowing to address two D-P transitions in 40Ca+ ions. Its output bandwidth of 22 MHz coincides with the absorption bandwidth of the calcium ions. Its spectral power density is 1.0 generated pairs/(s MHz mW).
We present a scheme, based only on linear optics and standard photon detection, that allows to generate heralded multiphoton entangled states of arbitrary photon number from spontaneous parametric downconversion (PDC) in the weak interaction regime. The scheme also works in the strong interaction regime, i.e., for the production of large photon numbers, when photon-number resolving detectors with nearly perfect quantum efficiency are used. In addition, the same setup can be used for quantum metrology as multiphoton interferometer with sensitivity at the Heisenberg limit.
Robust and reliable method for reconstructing quasi-distributions of integrated intensities of twin beams generated in spontaneous parametric down-conversion and entangled in photon numbers is suggested. It utilizes the first and second photocount moments and minimizes the declination from experimental photocount histograms. Qualitatively different forms of quasi-distributions for quantum and classical states are suggested in the method. The transition from quantum to classical states caused by an increased detection noise is discussed. Momentum criterion for non-classicality of twin beams is …
Using a spontaneous parametric-downconversion source of photon pairs, we are working towards the creation of arbitrary 2-qubit quantum states with high fidelity. Currently, all physically allowable combinations of polarization entanglement and mixture can be produced, including maximally-entangled mixed states. The states are experimentally measured and refined via computer-automated quantum-state tomography, and this system has also been used to perform single-qubit and ancilla-assisted quantum process tomography.
This work analyses the temporal coherence and correlation of twin beams generated in a quasi-phase matched nonlinear crystal in a counterpropagating configuration, ranging from the low-gain regime, where counterpropagating photon pairs are generated spontaneously, to the regime of stimulated pair production, close to the MOPO (Mirrorless Optical Parametric Oscillator) threshold. Here we show a critical divergence of the correlation time and slowing down of quantum fluctuations originating from the feedback mechanism responsible of the MOPO threshold.
