A pulse shaping algorithm for a matter wave with the purpose of controlling a binary reaction has been designed. The scheme is illustrated for an Eley-Rideal reaction where an impinging matter-wave atom recombines with an adsorbed atom on a metal surface. The wave function of the impinging atom is shaped such that the desorbing molecule leaves the surface in a specific vibrational state.
Quantum computing exploits the quantum-mechanical nature of matter to exist in multiple possible states simultaneously. This new approach promises to revolutionize the present form of computing. As an approach to quantum computing, we discuss ultrafast laser pulse shaping, in particular, the acousto-optic modulator based Fourier-Transform pulse-shaper, which has the ability to modulate tunable high power ultrafast laser pulses. We show that optical pulse shaping is an attractive route to quantum computing since shaped pulses can be transmitted over optical hardware and the same infrastructure …
We describe a technique for generating pulses of light with controllable photon numbers, propagation direction, timing, and pulse shapes. The technique is based on preparation of an atomic ensemble in a state with a desired number of atomic spin excitations, which is later converted into a photon pulse. Spatio-temporal control over the pulses is obtained by exploiting long-lived coherent memory for photon states and electromagnetically induced transparency (EIT) in an optically dense atomic medium. Using photon counting experiments we observe generation and shaping of few-photon sub-Poissonian…
In this paper we discuss possibilities to manipulate a matter-wave with time-dependent potentials. Assuming a specific setup on an atom chip, we explore how one can focus, accelerate, reflect, and stop an atomic wave packet, with, for example, electric fields from an array of electrodes. We also utilize this method to initiate coherent splitting. Special emphasis is put on the robustness of the control schemes. We begin with the wave packet of a single atom, and extend this to a BEC, in the Gross-Pitaevskii picture. In analogy to laser pulse shaping with its wide variety of applications, we ex…
We introduce a protocol capable of generating a general measurement operator for a mechanical resonator. The technique requires a qubit-resonator interaction and uses a coherent pulse to drive qubit transitions. This is followed by projective measurement of the qubit's energy, constraining the resonator in a state that depends on the pulse shape. The freedom to choose a pulse shape for the coherent drive enables an arbitrary position-basis measurement operator. Using this measurement operator, we outline a two pulse protocol that probabilistically generates a pure mechanical state with a desir…
We present a detailed analysis of the multimode quantum state embedded in an optical frequency comb generated by a Synchronously Pumped Optical Parametric Oscillator (SPOPO). The full covariance matrix of the state is obtained with homodyne detection where the local oscillator is spectrally controlled with pulse shaping techniques. The resulting matrix reveals genuine multipartite entanglement. Additionally, the beam is comprised of several independent eigenmodes that correspond to specific pulse shapes. The experimental data is confirmed with numerical simulations. Finally, the potential to c…
We experimentally demonstrate spectral broadening and shaping of exponentially-decaying nanosecond pulses via nonlinear mixing with a phase-modulated pump in a periodically-poled lithium niobate (PPLN) waveguide. A strong, 1550~nm pulse is imprinted with a temporal phase and used to upconvert a weak 980 nm pulse to 600 nm while simultaneously broadening the spectrum to that of a Lorentzian pulse up to 10 times shorter. While the current experimental demonstration is for spectral shaping, we also provide a numerical study showing the feasibility of subsequent spectral phase correction to achiev…
A method for time differentiation based on a Babinet-Soleil-Bravais compensator is introduced. The complex transfer function of the device is measured using polarization spectral interferometry. Time differentiation of both the pulse field and pulse envelope are demonstrated over a spectral width of about 100 THz with a measured overlap with the objective mode greater than 99.8%. This pulse shaping technique is shown to be perfectly suited to time metrology at the quantum limit.
Selective Excitation of Superconducting Qubits with a Shared Control Line through Pulse Shaping
The University of Osaka（大阪大学）；Center for Quantum Information and Quantum Biology, The University of Osaka（大阪大学量子信息与量子生物学中心）；QuEL, Inc.（QuEL公司）；e-trees.Japan, Inc.（e-trees.Japan公司）
Semiconductor quantum dots embedded in optical cavities are promising on-demand sources of single photons. Here, we theoretically study single photon emission from an optically driven two-photon Raman transition between the biexciton and the ground state of a quantum dot. The advantage of this process is that it allows all-optical control of the properties of the emitted single photon with a laser pulse. However, with the presence of other decay channels and excitation-induced quantum interference, on-demand emission of the single Raman photon is generally difficult to achieve. Here we show th…
We present a theoretical study of the shaping of the time-evolution of field-free orientation of linear molecules. We show the extend to which the degree of orientation can be steered along a desired periodic time-dependent signal. The objective of this study is not to optimize molecular orientation but to propose a general procedure to precisely control rotational dynamics through the first moment of the molecular axis distribution. Rectangular and triangular signals are taken as illustrative examples. At zero temperature, we compute the quantum states leading to such field-free dynamics. A T…
The temporal-mode (TM) basis is a prime candidate to perform high-dimensional quantum encoding. Quantum frequency conversion has been employed as a tool to perform tomographic analysis and manipulation of ultrafast states of quantum light necessary to implement a TM-based encoding protocol. While demultiplexing of such states of light has been demonstrated in the Quantum Pulse Gate (QPG), a multiplexing device is needed to complete an experimental framework for TM encoding. In this work we demonstrate the reverse process of the QPG. A dispersion-engineered difference frequency generation in no…
This work investigates the utility of femtosecond pulse shaping in increasing the efficiency of Raman excitation of molecules in the strong-field interaction regime. We study experimentally and theoretically the effect of pulse shaping on the strength of non-resonant coherent anti-Stokes Raman scattering in iodine vapor at laser intensities exceeding $10^{13}$ W/cm$^2$. We show that unlike the perturbative case, shaping strong non-resonant laser pulses can increase the signal strength beyond that observed with the transform-limited excitation. Both adiabatic and non-adiabatic schemes of excita…
We employ pulse shaping to abate single-qubit gate errors arising from the weak anharmonicity of transmon superconducting qubits. By applying shaped pulses to both quadratures of rotation, a phase error induced by the presence of higher levels is corrected. Using a derivative of the control on the quadrature channel, we are able to remove the effect of the anharmonic levels for multiple qubits coupled to a microwave resonator. Randomized benchmarking is used to quantify the average error per gate, achieving a minimum of 0.007+/-0.005 using 4 ns-wide pulse.
Uniting Quantum Processing Nodes of Cavity-coupled Ions with Rare-earth Quantum Repeaters Using Single-photon Pulse Shaping Based on Atomic Frequency Comb
Multimode entanglement is quintessential for the design and fabrication of quantum networks, which play a central role in quantum information processing and quantum metrology. However, an experimental setup is generally constructed with a specific network configuration in mind and therefore exhibits reduced versatility and scalability. The present work demonstrates an on-demand, reconfigurable quantum network simulator, using an intrinsically multimode quantum resource and a homodyne detection apparatus. Without altering either the initial squeezing source or experimen- tal architecture, we re…
We propose a mechanism to produce a superposition of atomic and molecular states by a train of ultrashort laser pulses combined with weak control fields. By adjusting the repetition rate of the pump pulses and the intensity of the coupling laser, one can suppress a transition while simultaneously enhancing the desired transitions. As an example, various superpositions of vibrational states of the $K_2$ molecule are shown.
We demonstrate a dispersive measurement pulse shaping technique that allows for arbitrarily fast quantum non-demolition, single-quadrature measurements of non-linear systems and unconditionally leaves the measurement resonator empty. For single-qubit measurements, current measurements are limited to the 99% fidelity range due to relaxation during the process. However, trying to go to shorter times to circumvent this with square or composite digital pulses leads to leftover cavity population after measurement of the same order of error. These effects can be suppressed using simple smooth pulse …
Dynamic coupling of cavities to a quantum network is of major interest to distributed quantum information processing schemes based on cavity quantum electrodynamics. This can be achieved by active tuning a mediating atom-cavity system. In particular, we consider the dynamic coupling between two coupled cavities, each interacting with a two-level atom, realized by tuning one of the atoms. One atom-field system can be controlled to become maximally and minimally coupled with its counterpart, allowing high fidelity excitation confinement, Q-switching and reversible state transport. As an applicat…
We explore the effects of ultrafast shaped pulses for two-level systems that do not have a single photon resonance by developing a multiphoton density-matrix approach. We take advantage of the fact that the dynamics of the intermediate virtual states are absent within our laser pulse timescales. Under these conditions, the multiphoton results are similar to the single photon and that it is possible to extend the single photon coherent control ideas to develop multiphoton coherent control.
We study theoretically and experimentally the influence of temporally shaping the light pulses in an atom interferometer, with a focus on the phase response of the interferometer. We show that smooth light pulse shapes allow rejecting high frequency phase fluctuations (above the Rabi frequency) and thus relax the requirements on the phase noise or frequency noise of the interrogation lasers driving the interferometer. The light pulse shape is also shown to modify the scale factor of the interferometer, which has to be taken into account in the evaluation of its accuracy budget. We discuss the …
We vary the time-frequency mode structure of ultrafast pulse-pumped modulational instability (MI) twin beams in an argon-filled hollow-core kagomé-style PCF by adjusting the pressure, pump pulse chirp, fiber length and parametric gain. Compared to solid-core systems, the pressure dependent dispersion landscape brings increased flexibility to the tailoring of frequency correlations and we demonstrate that the pump pulse chirp can be used to tune the joint spectrum of femtosecond-pumped sources. We also characterize the resulting mode content, not only by measuring the multimode second-order cor…
The shape of a few-cycle terahertz (THz) laser pulse can be optimized to provide control over conduction band populations in graphene. To demonstrate this control in a theoretical way, a spectral parametrization of the driving pulse using $B$-splines is used in order to obtain experimentally realistic pulses of bandwidth $\sim$ 30 THz. Optimization of the spectral shape is performed via differential evolution, using the $B$-splines expansion coefficients as decision variables. Numerical results show the possibility of changing the carrier density in graphene by a factor of 4 for a fixed pulse …
The paper investigates cold molecules formation in the photoassociation of two cold atoms by a strong laser pulse applied at short interatomic distances, which lead to a molecular dynamics taking place in the light-induced (adiabatic) potentials. A two electronic states model in the cesium dimer is used to analyse the effects of this strong coupling regime and to show specific results: i) acceleration of the ground state population to the inner zone due to a non-impulsive regime of coupling at short and intermediate interatomic distances; ii) formation of cold molecules in strongly bound level…
Controlling the wave function of free electrons is important to improve the spatial resolution of electron microscopes, the efficiency of electron interaction with sample modes of interest, and our ability to probe ultrafast materials dynamics at the nanoscale. In this context, attosecond electron compression has been recently demonstrated through interaction with the near fields created by scattering of ultrashort laser pulses at nanostructures followed by free electron propagation. Here, we show that control over electron pulse shaping, compression, and statistics can be improved by replacin…
We show that detuned optical pulse trains with a modest spectral width can polarize nuclear spins in InAs quantum dots. The pulse bandwidth is large enough to excite a coherent superposition of both electron spin eigenstates in these negatively charged dots but narrow enough to give partial spectral selectivity between the eigenstates. The coherent precession of electron spin states and periodic excitation focuses the nuclear spin distribution, producing a discrete set of precession modes. The spectral selectivity generates a net nuclear polarization, through a mechanism that relies on optical…
We experimentally demonstrate shaping of the two-photon wavefunction of entangled photon-pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the two-photon wavefunction exactly like a coherent ultrashort pulse. To observe the shaping we perform sum-frequency generation (SFG) with an ultrahigh flux of entangled photons. At the appropriate conditions, SFG performs as a coincidence detector with an ultrashort response time (~100 fs), enabling a direct observation of the two-photon wavefunction. This property also enables us to demonstrate backg…
