Entanglement lies at the heart of quantum mechanics and in recent years has been identified as an essential resource for quantum information processing and computation. Creating highly entangled multi-particle states is therefore one of the most challenging goals of modern experimental quantum mechanics, touching fundamental questions as well as practical applications. Here we report on the experimental realization of controlled collisions between individual neighbouring neutral atoms trapped in the periodic potential of an optical lattice. These controlled interactions act as an array of quantum gates between neighbouring atoms in the lattice and their massively parallel operation allows the creation of highly entangled states in a single operational step, independent of the size of the system. In the experiment, we observe a coherent entangling-disentangling evolution in the many-body system depending on the phase shift acquired during the collision between neighbouring atoms. This dynamics is indicative of highly entangled many-body states that present novel opportunities for theory and experiment.
We show how to construct a multi-qubit control gate on a quantum register of an arbitrary size N. This gate performs a single-qubit operation on a specific qubit conditioned by the state of other N-1 qubits. We provide an algorithm how to build up an array of networks consisting of single-qubit rotations and multi-qubit control-NOT gates for the synthesis of an arbitrary entangled quantum state of N qubits. We illustrate the algorithm on a system of cold trapped ions. This example illuminates the efficiency of the direct implementation of the multi-qubit CNOT gate compared to its decomposition…
For one-dimensional systems with delta-contact interactions, the convergence of the exact-diagonalization method is tested with a basis of harmonic oscillator eigenfunctions with frequency $Ω$ optimized through the minimization of the eigenenergy of the desired level. It is shown that within the framework of this approach the well-converged results can be achieved at much smaller dimensions of the Hamiltonian matrix than with the standard approach that uses $Ω=1$. We present calculations for model systems of identical bosons with harmonic and double-well potentials. Our results show promising …
We study the preparation and manipulation of states involving a small number of interacting particles. By controlling the splitting and fusing of potential wells, we show how to interconvert Mott-insulator-like and trapped BEC-like states. We also discuss the generation of "Schrödinger cat" states by splitting a microtrap and taking into practical consideration the asymmetry between the resulting wells. These schemes can be used to perform multiparticle interferometry with neutral atoms, where interference effects can be observed only when all the participating particles are measured.
An approach to fast entanglement generation based on Rydberg dephasing of collective excitations (spin-waves) in large, optically thick atomic ensembles is proposed. Long-range $1/r^3$ atomic interactions are induced by microwave mixing of opposite-parity Rydberg states. Required long coherence times are achieved via four-photon excitation and read-out of long wavelength spin-waves. The dephasing mechanism is shown to have favorable, approximately exponential, scaling for entanglement generation.
We study the particle-entanglement dynamics witnessed by the quantum Fisher information (QFI) of a trapped Bose-Einstein condensate governed by the kicked rotor Hamiltonian. The dynamics is investigated with a beyond mean-field approach. We link the time scales of the validity of this approximation in, both, classical regular and chaotic regions, with the maximum Lyapunov exponents of the classical system. This establishes an effective connection between the classical chaos and the QFI. We finally study the critical point of a quantum phase transition using the beyond mean-field approximation …
Among the various kinds of entangled states, the 'W state' plays an important role as its entanglement is maximally persistent and robust even under particle loss. Such states are central as a resource in quantum information processing and multiparty quantum communication. Here we report the scalable and deterministic generation of four-, five-, six-, seven- and eight-particle entangled states of the W type with trapped ions. We obtain the maximum possible information on these states by performing full characterization via state tomography, using individual control and detection of the ions. A…
Multiparticle entanglement leads to richer correlations than two-particle entanglement and gives rise to striking contradictions with local realism, inequivalent classes of entanglement, and applications such as one-way or topological quantum computing. When exposed to decohering or dissipative environments, multiparticle entanglement yields subtle dynamical features and access to new classes of states and applications. Here, using a string of trapped ions, we experimentally characterize the dynamics of entanglement of a multiparticle state under the influence of decoherence. By embedding an e…
We perform spectroscopy on the hyperfine splitting of $^{85}$Rb atoms trapped in far-off-resonance optical traps. The existence of a spatially dependent shift in the energy levels is shown to induce an inherent dephasing effect, which causes a broadening of the spectroscopic line and hence an inhomogeneous loss of atomic coherence at a much faster rate than the homogeneous one caused by spontaneous photon scattering. We present here a number of approaches for reducing this inhomogeneous broadening, based on trap geometry, additional laser fields, and novel microwave pulse sequences. We then sh…
We demonstrate electromagnetically induced transparency (EIT) in a sample of rubidium atoms, trapped in an optical dipole trap. Mixing a small amount of $σ^-$-polarized light to the weak $σ^+$-polarized probe pulses, we are able to measure the absorptive and dispersive properties of the atomic medium at the same time. Features as small as 4 kHz have been detected on an absorption line with 20 MHz line width.
We introduce a general scheme to detect various multiparticle entanglement structures from global non-permutationally invariant observables. In particular, we derive bounds on the variance of non-permutationally invariant and collective operators for the verification of $k$-party entanglement. For a family of observables related to the spin structure factor, we give quantitative bounds on entanglement that are independent of the total number of particles. We introduce highly non-symmetric states with genuine multipartite entanglement that is verifiable with the presented technique and discuss …
The radiation pressure of two detuned laser beams can create a stable trap for a suspended cavity mirror; here it is shown that such a configuration entangles the output light fields via interaction with the mirror. Intra-cavity, the opto-mechanical system can become entangled also. The degree of entanglement is quantified spectrally using the logarithmic negativity. Entanglement survives in the experimentally accessible regime of gram-scale masses subject to thermal noise at room temperature.
We have studied a general technique for laser cooling a cloud of polarized trapped atoms down to the Doppler temperature. A one-dimensional optical molasses using polarized light cools the axial motional degree of freedom of the atoms in the trap. Cooling of the radial degrees of freedom can be modelled by reabsorption of scattered photons in the optically dense cloud. We present experimental results for a cloud of chromium atoms in a magnetic trap. A simple model based on rate equations shows quantitative agreement with the experimental results. This scheme allows us to readily prepare a dens…
We study entanglement of the motional degrees of freedom of two tethered and optically trapped microdisks inside a single cavity. By properly choosing the position of the trapped objects in the optical cavity and driving proper modes of the cavity it is possible to equip the system with linear and quadratic optomechanical couplings. We show that a parametric coupling between the fundamental vibrational modes of two tethered mircodiscs can be generated via a time modulated input laser. For a proper choice of the modulation frequency, this mechanism can drive the motion of the microdisks into an…
We present a detailed analysis and design of a neutral atom quantum logic device based on atoms in optical traps interacting via dipole-dipole coupling of Rydberg states. The dominant physical mechanisms leading to decoherence and loss of fidelity are enumerated. Our results support the feasibility of performing single and two-qubit gates at MHz rates with decoherence probability and fidelity errors at the level of $10^{-3}$ for each operation. Current limitations and possible approaches to further improvement of the device are discussed.
Ultra-cold atoms trapped in an optical dipole trap and prepared in a coherent superposition of their hyperfine ground states, decohere as they interact with their environment. We demonstrate than the loss in coherence in an "echo" experiment, which is caused by mechanisms such as Rayleigh scattering, can be suppressed by the use of a new pulse sequence. We also show that the coherence time is then limited by mixing to other vibrational levels in the trap and by the finite lifetime of the internal quantum states of the atoms.
We systematically investigate the bistable behavior and squeezing property of the librational mode of a levitated nonspherical nanoparticle trapped by laser beams. By expanding the librational potential to the forth order of the librational angle $θ$, we find that the nonlinear coefficient of this mode is dependent only on the size and material of nanoparticle, but independent of trapping potential shape. The bistability and hysteresis are displayed when the driving frequency is red-detuned to the librational mode. In the blue-detuned region, we have studied squeezing of the variance of librat…
Entanglement is a key ingredient for quantum technologies and a fundamental signature of quantumness in a broad range of phenomena encompassing many-body physics, thermodynamics, cosmology, and life sciences. For arbitrary multiparticle systems, entanglement quantification typically involves nontrivial optimisation problems, and may require demanding tomographical techniques. Here we develop an experimentally feasible approach to the evaluation of geometric measures of multiparticle entanglement. Our approach provides analytical results for particular classes of mixed states of N qubits, and c…
We investigate the emission of single photons from CdSe/CdS dot-in-rods which are optically trapped in the focus of a deep parabolic mirror. Thanks to this mirror, we are able to image almost the full 4$π$ emission pattern of nanometer-sized elementary dipoles and verify the alignment of the rods within the optical trap. From the motional dynamics of the emitters in the trap we infer that the single-photon emission occurs from clusters comprising several emitters. We demonstrate the optical trapping of rod-shaped quantum emitters in a configuration suitable for efficiently coupling an ensemble…
A tapered optical nanofiber simultaneously used to trap and optically interface of cold atoms through evanescent fields constitutes a new and well controllable hybrid quantum system. The atoms are trapped in two parallel 1D optical lattices generated by suitable far blue and red detuned evanescent field modes very close to opposite sides of the nanofiber surface. Collective electronic excitations (excitons) of each of the optical lattices are resonantly coupled to the second lattice forming symmetric and antisymmetric common excitons. In contrast to the inverse cube dependence of the individua…
We report the experimental demonstration of a quantum memory for collective atomic states in a far-detuned optical dipole trap. Generation of the collective atomic state is heralded by the detection of a Raman scattered photon and accompanied by storage in the ensemble of atoms. The optical dipole trap provides confinement for the atoms during the quantum storage while retaining the atomic coherence. We probe the quantum storage by cross-correlation of the photon pair arising from the Raman scattering and the retrieval of the atomic state stored in the memory. Non-classical correlations are ob…
We systematically investigate the multi-stability behaviour and cooling of both librational and translational modes of an optically levitated nonspherical nanoparticle. By expanding the trapping potential to the fourth order of both the translational and librational freedom degrees, we deduce the nonlinearity of them and their nonlinear coupling. Through stability analysis, we find that the system presents multi-stability when either the librational or the translational drive is red-detuned. The system will be stabilized if and only if these two drives are both blue-detuned. In the steady stat…
Atomic ensembles have many potential applications in quantum information science. Owing to collective enhancement, working with ensembles at high densities increases the overall efficiency of quantum operations, but at the same time also increases the collision rate and leads to faster decoherence. Here we report on experiments with optically trapped 87Rb atoms demonstrating a 20-fold increase of the coherence time when a dynamical decoupling sequence with more than 200 pi-pulses is applied. We perform quantum process tomography and demonstrate that using the decoupling scheme a dense ensemble…
We report the finding of "triply magic" conditions (the doubly magic frequency-intensity conditions of an optical dipole trap plus the magic magnetic field) for the microwave transitions of optically trapped alkali-metal atoms. The differential light shift (DLS) induced by a degenerate two-photon process is adopted to compensate a DLS associated with the one-photon process. Thus, doubly magic conditions for the intensity and frequency of the optical trap beam can be found. Moreover, the DLS decouples from the magnetic field in a linearly polarized optical dipole trap, so that the magic conditi…
Optically trapped nanoparticles have recently emerged as exciting candidates for tests of quantum mechanics at the macroscale and as versatile platforms for ultrasensitive metrology. Recent experiments have demonstrated parametric feedback cooling, nonequilibrium physics, and temperature detection, all in the classical regime. Here we provide the first quantum model for trapped nanoparticle cooling and force sensing. In contrast to existing theories, our work indicates that the nanomechanical ground state may be prepared without using an optical resonator; that the cooling mechanism correspond…
The quantum walk is the quantum analogue of the well-known random walk, which forms the basis for models and applications in many realms of science. Its properties are markedly different from the classical counterpart and might lead to extensive applications in quantum information science. In our experiment, we implemented a quantum walk on the line with single neutral atoms by deterministically delocalizing them over the sites of a one-dimensional spin-dependent optical lattice. With the use of site-resolved fluorescence imaging, the final wave function is characterized by local quantum state…
We experimentally investigate the coherence properties of a qubit stored in the Zeeman substates of the 5S1/2, F=1 hyperfine ground level of a single optically trapped Rb-87 atom. Larmor precession of a single atomic spin-1 system is observed by preparing the atom in a defined initial spin-state and then measuring the resulting state after a programmable period of free evolution. Additionally, by performing quantum state tomography, maximum knowledge about the spin coherence is gathered. By using an active magnetic field stabilization and without application of a magnetic guiding field we achi…
Optical trapping of molecules with long coherence times is crucial for many protocols in quantum information and metrology. However, the factors that limit the lifetimes of the trapped molecules remain elusive and require improved understanding of the underlying molecular structure. Here we show that measurements of vibronic line strengths in weakly and deeply bound $^{88}$Sr$_2$ molecules, combined with \textit{ab initio} calculations, allow for unambiguous identification of vibrational quantum numbers. This, in turn, enables the construction of refined excited potential energy curves that in…
Recent developments in space technology like micro-propulsion systems for drag-free control, thermal shielding, ultra-stable laser sources and stable optical cavities set an ideal platform for quantum optomechanical experiments with optically trapped dielectric spheres. Here, we will provide an overview of the results of recent studies aiming at the realization of the space mission MAQRO to test the foundations of quantum physics in a parameter regime orders of magnitude beyond existing experiments. In particular, we will discuss DECIDE, which is an experiment to prepare and then study a Schrö…
The fidelity of the gate operation and the coherence time of neutral atoms trapped in an optical dipole trap are figures of merit for the applications. The motion of the trapped atom is one of the key factors which influence the gate fidelity and coherence time. The motion has been considered as a classical oscillator in analyzing the influence. Here we treat the motion of the atom as a quantum oscillator. The population on the vibrational states of the atom are considered in analyzing the gate fidelity and decoherence. We show that the fidelity of a coherent rotation gate is dramatically limi…
Cold inelastic collisions between confined cesium (Cs) atoms and Cs$\_2$ molecules are investigated inside a CO$\_2$ laser dipole trap. Inelastic atom-molecule collisions can be observed and measured with a rate coefficient of $\sim 2.5 \times 10^{-11} $cm$^3$ s$^{-1}$, mainly independent of the molecular ro-vibrational state populated. Lifetimes of purely atomic and molecular samples are essentially limited by rest gas collisions. The pure molecular trap lifetime ranges 0,3-1 s, four times smaller than the atomic one, as is also observed in a pure magnetic trap. We give an estimation of the i…
Collective coherent scattering of laser light induces strong light forces between polarizable point particles. These dipole forces are strongly enhanced in magnitude and distance within the field of an optical waveguide so that at low temperature the particles self-order in strongly bound regular patterns. The stationary configurations typically exhibit super-radiant scattering with strong particle and light confinement. Here we study collective excitations of such self-consistent crystalline particle-light structures as function of particle number and pump strength. Multiple scattering and ab…
Optically trapped ensembles are of crucial importance for frequency measurements and quantum memories, but generally suffer from strong dephasing due to inhomogeneous density and light shifts. We demonstrate a drastic increase of the coherence time to 21 s on the magnetic field insensitive clock transition of Rb-87 by applying the recently discovered spin self-rephasing. This result confirms the general nature of this new mechanism and thus shows its applicability in atom clocks and quantum memories. A systematic investigation of all relevant frequency shifts and noise contributions yields a s…
We review recent works on optomechanics of optically trapped microspheres and nanoparticles in vacuum, which provide an ideal system for studying macroscopic quantum mechanics and ultrasensitive force detection. An optically trapped particle in vacuum has an ultrahigh mechanical quality factor as it is well-isolated from the thermal environment. Its oscillation frequency can be tuned in real time by changing the power of the trapping laser. Furthermore, an optically trapped particle in vacuum may rotate freely, a unique property that does not exist in clamped mechanical oscillators. In this re…
We propose a search for low mass dark matter particles through momentum recoils caused by their scattering from trapped, nm-scale objects. Our projections show that even with a modest array of fg-mass sensors, parameter-space beyond the reach of existing experiments can be explored. The case of smaller, ag-mass sensors is also analyzed - where dark matter can coherently scatter from the entire sensor - enabling a large enhancement in the scattering cross-section relative to interactions with single nuclei. Large arrays of such sensors have the potential to explore new parameter space down to d…
We use microwave induced adiabatic passages for selective spin flips within a string of optically trapped individual neutral Cs atoms. We position-dependently shift the atomic transition frequency with a magnetic field gradient. To flip the spin of a selected atom, we optically measure its position and sweep the microwave frequency across its respective resonance frequency. We analyze the addressing resolution and the experimental robustness of this scheme. Furthermore, we show that adiabatic spin flips can also be induced with a fixed microwave frequency by deterministically transporting the …
Dimensionality serves as an indispensable ingredient in any attempt to formulate the low-dimensional physics, and studying the dimensional crossover at a fundamental level is challenging. The purpose of this work is to study the hierarchical dimensional crossovers, namely the crossover from three dimensions (3D) to quasi-2D and then to 1D. Our system consists of a 3D Bose-Einstein condensate (BEC) trapped in an anisotropic 2D optical lattice characterized by the lattice depths $V_1$ along the $x$ direction and $V_2$ along the $y$ direction, respectively, where the hierarchical dimensional cros…
Laser-cooled atoms coupled to nanophotonic structures constitute a powerful research platform for the exploration of new regimes of light-matter interaction. While the initialization of the atomic internal degrees of freedom in these systems has been achieved, a full preparation of the atomic quantum state also requires controlling the center of mass motion of the atoms at the quantum level. Obtaining such control is not straightforward, due to the close vicinity of the atoms to the photonic system that is at ambient temperature. Here, we demonstrate cooling of individual neutral Cesium atoms,…
We demonstrate size selective optical trapping and transport for nanoparticles near an optical nanofiber taper. Using a two-wavelength, counter-propagating mode configuration, we show that 100 nm diameter and 150 nm diameter gold nanospheres (GNSs) are trapped by the evanescent field in the taper region at different optical powers. Conversely, when one nanoparticle species is trapped the other may be transported, leading to a sieve-like effect. Our results show that sophisticated optical manipulation can be achieved in a passive configuration by taking advantage of mode behavior in nanophotoni…
Detecting dark matter using optically trapped Rydberg atom tweezer arrays
Massachusetts Institute of Technology（麻省理工学院）；The University of Tokyo（东京大学）；Kyoto University（京都大学）；KEK（高能加速器研究机构）；Tohoku University（东北大学）；University of Toronto（多伦多大学）
Using an optical tweezers apparatus, we demonstrate three-dimensional control of nanodiamonds in solution with simultaneous readout of ground-state electron-spin resonance (ESR) transitions in an ensemble of diamond nitrogen-vacancy (NV) color centers. Despite the motion and random orientation of NV centers suspended in the optical trap, we observe distinct peaks in the measured ESR spectra qualitatively similar to the same measurement in bulk. Accounting for the random dynamics, we model the ESR spectra observed in an externally applied magnetic field to enable d.c. magnetometry in solution. …
We propose a novel cooling scheme for realising single photon sideband cooling on particles trapped in a state-dependent optical potential. We develop a master rate equation from an ab-initio model and find that in experimentally feasible conditions it is possible to drastically reduce the average occupation number of the vibrational levels by applying a frequency sweep on the cooling laser that sequentially cools all the motional states. Notably, this cooling scheme works also when a particle experiences a deeper trap in its internal ground state than in its excited state, a condition for whi…
The apparent conflict between general relativity and quantum mechanics remains one of the unresolved mysteries of the physical world. According to recent theories, this conflict results in gravity-induced quantum state reduction of "Schrödinger cats", quantum superpositions of macroscopic observables. In recent years, great progress has been made in cooling micromechanical resonators towards their quantum mechanical ground state. This work is an important step towards the creation of Schrödinger cats in the laboratory, and the study of their destruction by decoherence. A direct test of the gra…
We propose an experiment using optically trapped and cooled dielectric microspheres for the detection of short-range forces. The center-of-mass motion of a microsphere trapped in vacuum can experience extremely low dissipation and quality factors of $10^{12}$, leading to yoctonewton force sensitivity. Trapping the sphere in an optical field enables positioning at less than 1 $μ$m from a surface, a regime where exotic new forces may exist. We expect that the proposed system could advance the search for non-Newtonian gravity forces via an enhanced sensitivity of $10^5-10^7$ over current experime…
We present a technique for the dissipative preparation of highly entangled multiparticle states of atoms coupled to common oscillator modes. By combining local spontaneous emission with coherent couplings we engineer many-body dissipation that drives the system from an arbitrary initial state into a Greenberger-Horne-Zeilinger state. We demonstrate that using our technique, highly entangled steady states can be prepared efficiently in a time that scales polynomially with the system size. Our protocol assumes generic couplings and will thus enable the dissipative production of multiparticle ent…
Multiplexed bi-layered realization of fault-tolerant quantum computation over optically networked trapped-ion modules
University of Pittsburgh（匹兹堡大学）；Wyant College of Optical Sciences, University of Arizona（亚利桑那大学怀恩特光学科学学院）；A. James Clark School of Engineering, University of Maryland（马里兰大学A·詹姆斯·克拉克工程学院）
We present a Ramsey-type atom interferometer operating with an optically trapped sample of 10^6 Bose-condensed Rb-87 atoms. The optical trap allows us to couple the |F =1, mF =0>\rightarrow |F =2, mF =0> clock states using a single photon 6.8GHz microwave transition, while state selective readout is achieved with absorption imaging. Interference fringes with contrast approaching 100% are observed for short evolution times. We analyse the process of absorption imaging and show that it is possible to observe atom number variance directly, with a signal-to-noise ratio ten times better than the at…
Searching for Ultralight Dark Matter with MOLeQuTE: a Massive Optically Levitated Quantum Tabletop Experiment
INFN Naples（意大利国家核物理研究所那不勒斯分部）；Institut für Physik, Johannes Gutenberg-Universität Mainz（美因茨约翰内斯·古腾堡大学物理研究所）；DAMTP, Cambridge University（剑桥大学应用数学与理论物理系）；Center for Cosmology and Particle Physics, Department of Physics, New York University（纽约大学物理系宇宙学与粒子物理中心）；Department of Physics and Astronomy, University College London（伦敦大学学院物理与天文学系）；Center for Fundamental Physics and Center for Interdisciplinary Exploration and Research in Astrophysics, Department of Physics and Astronomy, Northwestern University（西北大学物理与天文学系基础物理中心及天体物理学跨学科探索研究中心）
Optically trapped dielectric objects are well suited for reaching the quantum regime of their center of mass motion in an ultra-high vacuum environment. We show that ground state cooling of an optically trapped nanosphere is achievable when starting at room temperature, by sympathetic cooling of a cold atomic gas optically coupled to the nanoparticle. Unlike cavity cooling in the resolved sideband limit, this system requires only a modest cavity finesse and it allows the cooling to be turned off, permitting subsequent observation of strongly-coupled dynamics between the atoms and sphere. Nanos…
Trapped ions form an advanced technology platform for quantum information processing with long qubit coherence times, high-fidelity quantum logic gates, optically active qubits, and a potential to scale up in size while preserving a high level of connectivity between qubits. These traits make them attractive not only for quantum computing but also for quantum networking. Dedicated, special-purpose trapped-ion processors in conjunction with suitable interconnecting hardware can be used to form quantum repeaters that enable high-rate quantum communications between distant trapped-ion quantum com…
Since the early work by Ashkin in 1970, optical trapping has become one of the most powerful tools for manipulating small particles, such as micron sized beads or single atoms. The optical trapping mechanism is based on the interaction energy of a dipole and the electric field of the laser light. In atom trapping, the dominant contribution typically comes from the allowed optical transition closest to the laser wavelength, whereas for mesoscopic particles it is given by the bulk polarizability of the material. These two different regimes of optical trapping have coexisted for decades without a…
Oscillating magnetic fields and field gradients can be used to implement single-qubit rotations and entangling multi-qubit quantum gates for trapped-ion quantum information processing (QIP). With fields generated by currents in microfabricated surface-electrode traps, it should be possible to achieve gate speeds that are comparable to those of optically induced gates for realistic distances between the ion crystal and the electrode surface. Magnetic-field-mediated gates have the potential to significantly reduce the overhead in laser beam control and motional state initialization compared to c…
