By means of a canonical transformation it is shown how it is possible to recast the equations for molecular nonlinear optics to completely eliminate ground-state static dipole coupling terms. Such dipoles can certainly play a highly important role in nonlinear optical response - but equations derived by standard methods, in which these dipoles emerge only as special cases of transition moments, prove unnecessarily complex. It has been shown that the elimination of ground-state static dipoles in favor of dipole shifts results in a considerable simplification in form of the nonlinear optical susceptibilities. In a fully quantum theoretical treatment the validity of such a procedure has previously been verified using an expedient algorithm, whose defense was afforded only by a highly intricate proof. In this paper it is shown how a canonical transformation method entirely circumvents such an approach; it also affords new insights into the formulation of quantum field interactions.
We study the resonance interaction between two quantum electric dipoles immersed in optically active surroundings. Quantum electrodynamics is employed to deal with dipole-vacuum interaction. Our results show that the optical activity of surroundings will not change the single atom behaviors while it can change the collective behaviors of the two dipoles, as well as greatly affect the dipole-dipole resonance interaction. Especially, if the orientations of two dipoles are orthogonal and respectively perpendicular to the interdipole axis, the interdipole resonance interaction can be established w…
Nonadiabtic dressed states and nonadiabatic induced dipole moment in the leading order of nonadiabaticity is proposed. The nonadiabatic induced dipole moment is studied in the femtosecond time domain.
We present a detailed analysis and design of a neutral atom quantum logic device based on atoms in optical traps interacting via dipole-dipole coupling of Rydberg states. The dominant physical mechanisms leading to decoherence and loss of fidelity are enumerated. Our results support the feasibility of performing single and two-qubit gates at MHz rates with decoherence probability and fidelity errors at the level of $10^{-3}$ for each operation. Current limitations and possible approaches to further improvement of the device are discussed.
We study a means of creating multiparticle entanglement of neutral atoms using pairwise controlled dipole-dipole interactions in a three dimensional optical lattice. For tightly trapped atoms the dipolar interaction energy can be much larger than the photon scattering rate, and substantial coherent evolution of the two-atom state can be achieved before decoherence occurs. Excitation of the dipoles can be made conditional on the atomic states, allowing for deterministic generation of entanglement. We derive selection rules and a figure-of-merit for the dipole-dipole interaction matrix elements,…
We present an implementation of quantum logic gates via internal state dependent displacements of ions in a linear Paul trap caused by optical dipole forces. Based on a general quantum analysis of the system dynamics we consider specific implementations with alkaline earth ions. For experimentally realistic parameters gate infidelities as low as $10^{-4}$ can be obtained.
Matrix-operator difference-differential equations for dynamics of spectroscopic transitions in 1D multiqubit exchange coupled (para)magnetic and optical systems by strong dipole-photon and dipole-phonon coupling are derived within the framework of quantum electrodynamics and quantum phonon field theory. It has been established, that in the model considered the relaxation processes are of pure quantum character, which is determined by the formation of the coherent system of the resonance phonons and by the appearence along with absorption process of EM-field energy the coherent emission process…
We consider a flat lattice of dipoles modeled by harmonic oscillators interacting with the electromagnetic field in dipole approximation. Eliminating the variables from the coupled equations of motion, we come to effective Maxwell equations. These allow for taking the lattice spacing $a$ to zero. As a result, we obtain reflection coefficients for the scattering of electromagnetic waves off the sheet. These are a generalization of that known from the hydrodynamic model. For instance, we get a non trivial scattering for polarizability perpendicular to the sheet. Also we show that the case of a s…
Microscopically controlled neutral atoms in optical tweezers and lattices have led to exciting advances in the study of quantum information and quantum many-body systems. The light shifts of atomic levels from the trapping potential in these systems can result in detrimental effects such as fluctuating dipole force heating, inhomogeneous detunings, and inhibition of laser cooling, which limits the atomic species that can be manipulated. In particular, these light shifts can be large enough to prevent loading into optical tweezers directly from a magneto-optical trap. We present a general solut…
Eliminating photon transport in long-baseline optical interferometry using quantum memories
NASA Glenn Research Center（美国国家航空航天局格伦研究中心）；University of Maryland, College Park（马里兰大学帕克分校）；Joint Center for Quantum Information and Computer Science, NIST/University of Maryland（量子信息与计算机科学联合中心，美国国家标准与技术研究院/马里兰大学）；Joint Quantum Institute, NIST/University of Maryland（量子研究所联合机构，美国国家标准与技术研究院/马里兰大学）；NSF NOIRLab（美国国家科学基金会NOIR实验室）
An analogy is explored between a setup of three atomic traps coupled via tunneling and an internal atomic three-level system interacting with two laser fields. Within this scenario we describe a STIRAP like process which allows to move an atom between the ground states of two trapping potentials and analyze its robustness. This analogy is extended to other robust and coherent transport schemes and to systems of more than a single atom. Finally it is applied to manipulate external degrees of freedom of atomic wave packets propagating in waveguides.
We theoretically investigate the interaction of a single quantum dipole with the modes of a fiber-coupled semiconductor waveguide. Through a combination of tight modal confinement and phase-matched evanescent coupling, we predict that approximately 70 % of the dipole's emission can be collected into a single mode optical fiber. Calculations further show that the dipole strongly modifies resonant light transmission through the system, with over an order of magnitude change possible for an appropriate choice of fiber-waveguide coupler geometry.
We introduce quantum optical dipole radiation fields defined in terms of photon creation and annihilation operators. These fields are identified through their spatial dependence, as the components of the total fields that survive infinitely far from the dipole source. We use these radiation fields to perturbatively evaluate the electromagnetic radiated energy-flux of the excited dipole. Our results indicate that the standard interpretation of a bare atom surrounded by a localised virtual photon cloud, is difficult to sustain, because the radiated energy-flux surviving infinitely far from the s…
We report a study on the optical dipole force in a ladder like three level atomic systems in the context of coherent population transfer with the chirped few-cycle-pulse laser fields. The phenomenon of coherent population transfer is investigated by numerically solving the appropriate density matrix equations beyond the rotating wave approximation. On the other hand, optical dipole force is calculated by numerically solving the force equation and density matrix equations self-consistently. By analysing the centre-of-mass motion, it is shown that the optical dipole force with chirped pulses may…
We derive a set of optical Bloch equations (OBEs) directly from the minimal-coupling Hamiltonian density of the bound-state quantum electrodynamics (bound-state QED). Such optical Bloch equations are beyond the former widely-used ones due to that there is no electric dipole approximation (EDA) on the minimal-coupling Hamiltonian density of the bound-state QED. Then our optical Bloch equations can describe a two-level atom interacting with a monochromatic light of arbitrary wavelength, which are suitable to study the spectroscopy and the Rabi oscillations of two-level atoms in X-ray laser beams…
The permanent electric dipole moment (EDM) of the $^{171}$Yb $(I=1/2)$ atom is measured with atoms held in an optical dipole trap (ODT). By enabling a cycling transition that is simultaneously spin-selective and spin-preserving, a quantum non-demolition measurement with a spin-detection efficiency of 50$\%$ is realized. A systematic effect due to parity mixing induced by a static E field is observed, and is suppressed by averaging between measurements with ODTs in opposite directions. The coherent spin precession time is found to be much longer than 300 s. The EDM is determined to be $d({\rm^{…
Optical dipole-traps are used in various scientific fields, including classical optics, quantum optics and biophysics. Here, we propose and implement a dipole-trap for nanoparticles that is based on focusing from the full solid angle with a deep parabolic mirror. The key aspect is the generation of a linear-dipole mode which is predicted to provide a tight trapping potential. We demonstrate the trapping of rod-shaped nanoparticles and validate the trapping frequencies to be on the order of the expected ones. The described realization of an optical trap is applicable for various other kinds of …
We propose a scheme for scalable and universal quantum computation using diatomic bits with conditional dipole-dipole interaction, trapped within an optical lattice. The qubit states are encoded by the scattering state and the bound heteronuclear molecular state of two ultracold atoms per site. The conditional dipole-dipole interaction appears between neighboring bits when they both occupy the molecular state. The realization of a universal set of quantum logic gates, which is composed of single-bit operations and a two-bit controlled-NOT gate, is presented. The readout method is also discusse…
Single atoms in dipole microtraps or optical tweezers have recently become a promising platform for quantum computing and simulation. Here we report a detailed theoretical analysis of the physics underlying an implementation of a Rydberg two-qubit gate in such a system -- a cornerstone protocol in quantum computing with single atoms. We focus on a blockade-type entangling gate and consider various decoherence processes limiting its performance in a real system. We provide numerical estimates for the limits on fidelity of the maximally entangled states and predict the full process matrix corres…
Two-photon excitation (TPE) proceeds via a "virtual" pathway, which depends on the accessibility of one or more intermediate states, and, in the case of non-centrosymmetric molecules, an additional "dipole" pathway involving the off-resonance dipole-allowed one-photon transitions and the change in the permanent dipole moment between the initial and final states. Here, we control the quantum interference between these two optical excitation pathways by using phase-shaped femtosecond laser pulses. We find enhancements by a factor of up to 1.75 in the two-photon-excited fluorescence of the photob…
