“水巴基球”的化学、催化和宇宙意义
"Water Buckyballs" Chemical, Catalytic, and Cosmic Implications
摘要：
基于电子和振动理论和实验，讨论了具有“巴基球”对称性的带电五角十二面体水团簇可能的化学、催化和宇宙作用。电子结构结合动态Jahn-Teller效应被认为是水巴基球催化剂和含氧化合物，用于燃料燃烧和生物系统中的活性剂。水巴基球宽广的电子和独特的低频电子振动谱可以解释某些弥漫的星际带，远红外，紫外和x射线宇宙背景辐射，以及一些“缺失的宇宙重子物质”。水巴基球的液体和超临界水的性质的相关性总结的文件。
英文摘要：
Possible chemical, catalytic, and cosmic roles of charged pentagonal dodecahedral water clusters having "buckyball-like" symmetry are discussed on the basis of electronic and vibronic theory and experiment. The electronic structure in conjunction with the dynamic Jahn-Teller effect is argued to make water buckyballs catalysts and oxygenates for fuel combustion and active agents in biological systems. The broad electronic and unique low-frequency vibronic spectra of water buckyballs may explain certain diffuse interstellar bands, far-infrared, ultraviolet, and x-ray cosmic background radiation, and some "missing cosmic baryonic matter". The relevance of water buckyballs to the properties of liquid and supercritical water concludes the paper.
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