We show that a physical mechanism responsible for the enhanced transmission and reflection of femtosecond pulses by a single subwavelength nanoslit in a thick metallic film is the Fabry-Perot-like resonant excitation of stationary, quasistationary and nonstationary waves inside the slit, which leads to the field enhancement inside and around the slit. The mechanism is universal for any pulse-scatter system, which supports the stationary resonances. We point out that there is a pulse duration limit below which the slit does not support the intraslit resonance.
We report on fabrication of tubular optical waveguides buried in ZBLAN glass based on transverse femtosecond laser direct writing. Irradiation in ZBLAN with focused femtosecond laser pulses leads to decrease of refractive index in the modified region. Tubular optical waveguides of variable mode areas are fabricated by forming the four sides of the cladding with slit-shaped femtosecond laser pulses, ensuring single mode waveguiding with a mode field dimension as small as ~ 4 μm.
In this paper, the scattering/transmission inside a step-modulated subwavelength metal slit is investigated in detail. We firstly investigate the scattering in a junction structure by two types of structural changes. The variation of transmission and reflection coefficients depending on structural parameters are analyzed. Then a multi-mode multi-reflection model based on ray theory is proposed to illustrate the transmission in the step-modulated slit explicitly. The key parts of this model are the multi-mode excitation and the superposition procedure of the scatterings from all possible modes,…
To study the dynamical optical interactions of nano-scaled metal-insulator-metal (MIM) structures in temporal-frequency domain, femtosecond surface plasmon polariton (SPP) wave packets propagate over a surface with a MIM structure. The resonance nature of the SPP-cavity interaction is reflected as strong modulations in the spectra of transmitted and reflected SPP wavepackets, which show peaks and valleys, respectively, corresponding to the MIM cavity's eigenmode. These features indicate that the MIM structure acts as a Fabry-Perot etalon-type spectrum filter. With appropriate tuning of the res…
We report on fabrication of depressed cladding optical waveguides buried in lithium niobate crystal with shaped femtosecond laser pulses. Depressed cladding waveguides of variable mode-field sizes are fabricated by forming the four sides of the cladding using a slit-beam shaping technique. We show that the waveguides fabricated by our technique allows single-mode propagation of the light polarized in both vertical and horizontal directions.
The existence of resonant enhanced transmission and collimation of light waves by subwavelength slits in metal films [for example, see T.W. Ebbesen et al., Nature (London) 391, 667 (1998) and H.J. Lezec et al., Science, 297, 820 (2002)] leads to the basic question: Can a light pulse be enhanced and simultaneously localized in space and time by a subwavelength slit? To address this question, the spatial distribution of the energy flux of an ultrashort (femtosecond) wave-packet diffracted by a subwavelength (nanometer-size) slit was analyzed by using the conventional approach based on the Neerho…
The existence of resonant enhanced transmission and collimation of light waves by subwavelength slits in metal films [for example, see T.W. Ebbesen et al., Nature (London) 391, 667 (1998) and H.J. Lezec et al., Science, 297, 820 (2002)] leads to the basic question: Can a light be enhanced and simultaneously localized in space and time by a subwavelength slit? To address this question, the spatial distribution of the energy flux of an ultrashort (femtosecond) wave-packet diffracted by a subwavelength (nanometer-size) slit was analyzed by using the conventional approach based on the Neerhoff and…
Carrier and phonon dynamics in Bi2Se3 crystals are studied by a spatially resolved ultrafast pump-probe technique. Pronounced oscillations in differential reflection are observed with two distinct frequencies, and are attributed to coherent optical and acoustic phonons, respectively. The rising time of the signal indicates that the thermalization and energy relaxation of hot carriers are both sub-ps in this material. We found that the thermalization and relaxation time decreases with the carrier density. The expansion of the differential reflection profile allows us to estimate an ambipolar ca…
Under the sub-wavelength condition ($w<λ/2$), an analytical model of light transmission and reflection through $1$D metallo-dielectric gratings of real metals has been developed. It has been shown that the transmission intensity associated with the Fabry-Perot (FP) resonance of a $1$D metallo-dielectric grating of a real metal decreases with the increasing grating thickness and the dielectric constant of the ridge material. Further, it has also been demonstrated that the intensity of the FP resonance increases with the increasing slit width while it is independent of the grating period ($P$) a…
We present a concrete picture of spoof surface plasmons (SSPs) combined with cavity resonance to clarify the basic mechanism underlying extraordinary light transmission through metal films with subwavelength slits or holes. This picture may indicate a general mechanism of metallic nanostructure optics: When light is incident on a non-planar conducting surface, the free electrons cannot move homogeneously in response to the incident electric field, i.e., their movement can be impeded at the rough parts, forming inhomogeneous charge distributions. The oscillating charges/dipoles then emit photon…
The incumbent technology for bringing light to the nanoscale, the near-field scanning optical microscope, has notoriously small throughput efficiencies - of the order of 10^(-4) - 10^(-5), or less. We report on a broadband, topological, unidirectionally-guiding structure, not requiring adiabatic tapering and in principle enabling near-perfect (ideally, ~100%) optical transmission through an unstructured single (POTUS) arbitrarily-subdiffraction slit at its end. Specifically, for a slit width of just lambda_eff / 72 (lambda_0 / 138) the attained normalized transmission coefficient reaches a val…
Oscillator-driven broadband femtosecond transient microspectroscopy with supercontinuum probes generated in a photonic crystal fiber
Osaka Metropolitan University（大阪公立大学）；Institute for Molecular Science, National Institutes of Natural Sciences（国立自然科学研究所分子科学研究所）；Instituto de Ciencia de Materiales de Madrid (ICMM-CSIC)（马德里材料科学研究所）
We present an innovative beamline for extreme ultraviolet (XUV)-infrared (IR) pump-probe reflection spectroscopy in solids with attosecond temporal resolution. The setup uses an actively stabilized interferometer, where attosecond pulse trains or isolated attosecond pulses are produced by high-order harmonic generation in gases. After collinear recombination, the attosecond XUV pulses and the femtosecond IR pulses are focused twice in sequence by toroidal mirrors, giving two spatially separated interaction regions. In the first region, the combination of a gas target with a time-of-flight spec…
The theory and experiments concerned with the electron-ion thermal relaxation and melting of overheated crystal lattice constitute the subject of this paper. The physical model includes two-temperature equation of state, many-body interatomic potential, the electron-ion energy exchange, electron thermal conductivity, and optical properties of solid, liquid, and two phase solid-liquid mixture. Two-temperature hydrodynamics and molecular dynamics codes are used. An experimental setup with pump-probe technique is used to follow evolution of an irradiated target with a short time step 100 fs betwe…
We demonstrate numerically a method of focusing two-photon field inside one-dimensional random media. The approach is based on coherent control of backscattering achieved by adaptive spectral pulse shaping. The spectral phases of a femtosecond laser pulse are adjusted for the constructive interference of its backward-traveling components, resulting in an enhanced reflection from within the random system. A delayed forward-propagating second pulse overlaps with the controlled reflection, increasing the inter-pulse multi-photon field at a location determined by the delay between the two pulses. …
In this work we present a new mechanism for designing phase-gradient metasurfaces (PGMs) to control an electromagnetic wavefront with high efficiency. Specifically, we design a transmission-type PGM formed by a periodic subwavelength metallic slit array filled with identical dielectrics of different heights. It is found that when Fabry-Perot (FP) resonances occur locally inside the dielectric regions, in addition to the common phenomenon of complete transmission, the transmitted phase differences between two adjacent slits are exactly the same, being a non-zero constant. These local FP resonan…
Carrier dynamics in single-layer graphene grown by chemical vapor deposition (CVD) is studied using spatially and temporally resolved pump-probe spectroscopy by measuring both differential transmission and differential reflection. By studying the expansion of a Gaussian spatial profile of carriers excited by a 1500-nm pump pulse with a 1761-nm probe pulse, we observe a diffusion of hot carriers of 5500 square centimeter per second. We also observe that the expansion of the carrier density profile decreases to a slow rate within 1 ps, which is unexpected. Furthermore, by using an 810-nm probe p…
Scattering of femtosecond laser pulses on resonant transmission and reflection gratings made of dispersive (Drude metals) and dielectric materials is studied by a time-domain numerical algorithm for Maxwell's theory of linear passive (dispersive and absorbing) media. The algorithm is based on the Hamiltonian formalism in the framework of which Maxwell's equations for passive media are shown to be equivalent to the first-order equation, $\partial Ψ/\partial t = {\cal H}Ψ$, where ${\cal H}$ is a linear differential operator (Hamiltonian) acting on a multi-dimensional vector $Ψ$ built of the elec…
We propose a novel scheme to generate single-cycle terahertz (THz) pulses via reflection of an optical femtosecond pulse train from a thin layer of nonlinear resonant medium. Our method is based on a coherent control of low-frequency oscillations and free induction decay in the medium. The specific single-cycle shape of generated THz pulses requires a plane wavefront and detection in the near field. Our theoretical results pave the way to a new, simple and high-efficiency way to generate single-cycle waveshape-tunable terahertz pulses.
We combine scattering theory, Fourier, traveling wave and asymptotic analyses together with numerical simulations to present interesting and practically useful properties of femtosecond pulse interaction with thin films. The dispersive material is described by a single resonance Lorentz model and its nonlinear extension with a cubic Duffing-type nonlinearity. A key feature of the Lorentz dielectric function is that its real part becomes negative between its zero and its pole, generating a forbidden region. We illustrate numerically the linear interaction of the pulse with the film using both s…
