Response of Superheated Droplet Detectors of the PICASSO Dark Matter Search Experiment
The PICASSO Collaboration, M. Barnabe-Heider, E. Behnke, K. Clark, M. Di Marco, P. Doane, W. Feighery, M. -H. Genest, R. Gornea, R. Guenette, S. Kanagalingam, C… 展开作者
The PICASSO Collaboration, M. Barnabe-Heider, E. Behnke, K. Clark, M. Di Marco, P. Doane, W. Feighery, M. -H. Genest, R. Gornea, R. Guenette, S. Kanagalingam, C. B. Krauss, C. Leroy, L. Lessard, I. Levine, J. -P. Martin, C. Muthusi, A. J. Noble, R. Noulty, U. Wichoski, V. Zacek
We present results of systematic studies of the radiation response of superheated liquid droplet detectors, which are used in the PICASSO dark matter search experiment. This detection technique is based on the phase transitions of superheated liquid Freon droplets dispersed and trapped in a polymerized gel. Phase transitions can be induced by nuclear recoils following particle interactions and, in particular, interactions with Weakly Interacting Massive Particles (WIMPs). These detectors are threshold devices since a minimal energy deposition is necessary to induce a phase transition and their sensitivity to various types of radiation depends strongly on the operating temperature and pressure. The sensitivity to neutrons, alpha particles and gamma rays was determined as a function of these operating parameters and the results are compared with simulations. In particular, we present a complete characterization of the response of detector modules already in use for a dark matter search at the SNO site to detect WIMPs and discuss possible background sources.
The PICASSO project is a cold dark matter (CDM) search experiment relying on the superheated droplet technique. The detectors use superheated freon liquid droplets (active material) dispersed and trapped in a polymerized gel. This detection technique is based on the phase transition of superheated droplets at about room temperature and ambient pressure. The phase transition is induced by nuclear recoils when an atomic nucleus in the droplets interacts with incoming subatomic particles. This includes CDM particles candidate as the neutralino (a yet-to-discover particle predicted in extensions o…
Superheated droplets are proven to be excelent detectors for neutrons and could be used as a neutron dosimeter. To detect accurately the volume of the vapour formed upon nucleation and hence to observe the nucleation quantitatively an air displacement system has been developed.
R-134a (C2H2F4) is a low cost, easily available and chlorine free refrigerant, which in its superheated state can be used as an efficient neutron detector. Due to its high solubility in water the R-134a based superheated droplet detectors (SDD) are usually very unstable unless the detector is fabricated using a suitable additive, which stabilizes the detector. The SDD is known to have superheated droplets distributed in a short-lived and in a relatively longer-lived metastable states. We have studied the detector response to neutrons using a 241AmBe neutron source and obtained the temperature …
The bubble nucleation in superheated liquid can be controlled by adjusting the ambient pressure and temperature. At higher pressure the threshold energy for bubble nucleation increases and we have observed that the amplitude of the acoustic emission during vaporisation of superheated droplet decreases with increase in pressure at any given temperature. Other acoustic parameters such as the primary harmonic frequency and the decay time constant of the acoustic signal also decrease with increase in pressure. It is independent of the type of superheated liquid. The decrease in signal amplitude li…
The combined measurement of dark matter interactions with different superheated liquids has recently been suggested as a cross-correlation technique in identifying WIMP candidates. We describe the fabrication of high concentration superheated droplet detectors based on the light nuclei liquids C3F8, C4F8, C4F10 and CCl2F2, and investigation of their irradiation response with respect to C2ClF5. The results are discussed in terms of the basic physics of superheated liquid response to particle interactions, as well as the necessary detector qualifications for application in dark matter search inv…
At present, application of Superheated Droplet Detectors (SDDs) in WIMP dark matter searches has been limited to the spin-dependent sector, owing to the general use of fluorinated refrigerants which have high spin sensitivity. Given their recent demonstration of a significant constraint capability with relatively small exposures and the relative economy of the technique, we consider the potential impact of heavy versions of such devices on the spin-independent sector. Limits obtainable from a $\mathrm{CF_{3}I}$-loaded SDD are estimated on the basis of the radiopurity levels and backgrounds alr…
The bubble nucleation process in superheated droplet detector (SDD) is associated with the emission of an acoustic pulse that can be detected by an acoustic sensor. We have studied the neutron and gamma-ray induced nucleation events in a SDD with the active liquid R-12 (CCl2F2, b.p. -29.8oC) using a condenser microphone sensor. A comparative study in the low frequency region (~ 0-10kHz) for the neutron and gamma-ray induced nucleation is presented here. From the analysis of the waveforms we observe a significant difference between the neutron and gamma-ray induced acoustic events.
The superheated droplet detector (SDD) is known to be gamma insensitive below a threshold temperature which made them excellent candidates for neutron detection in the presence of gamma rays. Above the threshold temperature, the gamma ray detection efficiency increases with increase in temperature. In this work the gamma ray threshold temperature has been studied for SDD using R404A as the active liquid and is compared to the theoretical prediction. The temperature variation of gamma ray detection efficiency and interstate transition kinetics has also been studied using a two-state model. The …
Energy calibration of superheated droplet detector is discussed in terms of the effective recoil nucleus threshold energy and the reduced superheat. This provides a universal energy calibration curve valid for different liquids used in this type of detector. Two widely used liquids, R114 and C4F10, one for neutron detection and the other for WIMPs dark matter search experiment, have been compared. Liquid having recoil nuclei with larger values of LET provides better neutron and gamma discrimination. Gamma response of C4F10 has also been studied and the results are discussed. Behaviour of nucle…
The PICASSO collaboration observed for the first time a significant difference between the acoustic signals induced by neutrons and alpha particles in a detector based on superheated liquids. This new discovery offers the possibility of improved background suppression and could be especially useful for dark matter experiments. This new effect may be attributed to the formation of multiple bubbles on alpha tracks, compared to single nucleations created by neutron induced recoils.
The simulation of the neutron background for Phase II of the SIMPLE direct dark matter search experiment is fully reported with various improvements relative to previous estimates. The model employs the Monte Carlo MCNP neutron transport code, using as input a realistic geometry description, measured radioassays and material compositions, and tabulated (α,n) yields and spectra. Developments include the accounting of recoil energy distributions, consideration of additional reactions and materials and examination of the relevant (α,n) data. A thorough analysis of the simulation results is perfor…
Superheated Droplet Detectors (SDDs) are becoming commonplace in neutron personnel dosimetry. Their total insensitivity to minimum ionizing radiation (while responsive to nuclear recoils of energies ~ few keV), together with their low cost, ease of production, and operation at room temperature and 1 atm makes them ideal for Cold Dark Matter (CDM) searches. SDD's are optimal for the exploration of the spin-dependent neutralino coupling due to their high fluorine content. The status of SIMPLE (Superheated Instrument for Massive ParticLe Experiments) is presented. Under realistic background consi…
SIMPLE (Superheated Instrument for Massive ParticLE searches) employs superheated droplet detectors (SDDs) to search for Weakly Interacting Massive Particle (WIMP) dark matter. As a result of the intrinsic SDD insensitivity to minimum ionizing particles and high fluorine content of target liquids, competitive WIMP limits were already obtained at the early prototype stage. We comment here on the expected immediate increase in sensitivity of the program and on future plans to exploit this promising technnique.
We report on the fabrication aspects and calibration of the first large active mass ($\sim15$ g) modules of SIMPLE, a search for particle dark matter using Superheated Droplet Detectors (SDDs). While still limited by the statistical uncertainty of the small data sample on hand, the first weeks of operation in the new underground laboratory of Rustrel-Pays d'Apt already provide a sensitivity to axially-coupled Weakly Interacting Massive Particles (WIMPs) competitive with leading experiments, confirming SDDs as a convenient, low-cost alternative for WIMP detection.
SIMPLE 2000 (Superheated Instrument for Massive ParticLE searches) will consist of an array of eight to sixteen large active mass ($\sim15$ g) Superheated Droplet Detectors(SDDs) to be installed in the new underground laboratory of Rustrel-Pays d'Apt. Several factors make of SDDs an attractive approach for the detection of Weakly Interacting Massive Particles (WIMPs), namely their intrinsic insensitivity to minimum ionizing particles, high fluorine content, low cost and operation near ambient pressure and temperature. We comment here on the fabrication, calibration and already-competitive firs…
The PICASSO dark matter search experiment operated an array of 32 superheated droplet detectors containing 3.0 kg of C$_{4}$F$_{10}$ and collected an exposure of 231.4 kgd at SNOLAB between March 2012 and January 2014. We report on the final results of this experiment which includes for the first time the complete data set and improved analysis techniques including \mbox{acoustic} localization to allow fiducialization and removal of higher activity regions within the detectors. No signal consistent with dark matter was observed. We set limits for spin-dependent interactions on protons of $σ_p^…
We report new results obtained in calibrations of superheated liquid droplet detectors used in dark matter searches with different radiation sources (n,$α$,$γ$). In particular, detectors were spiked with alpha-emitters located inside and outside the droplets. It is shown that the responses are different, depending on whether alpha particles or recoil nuclei create the signals. The energy thresholds for $α$-emitters are compared with test beam measurements using mono-energetic neutrons, as well as with theoretical predictions. Finally a model is presented which describes how the observed intens…
Phase II of SIMPLE (Superheated Instrument for Massive ParticLe Experiments) searched for astroparticle dark matter using superheated liquid C$_{2}$ClF$_{5}$ droplet detectors. Each droplet generally requires an energy deposition with linear energy transfer (LET) $\gtrsim$ 150 keV/$μ$m for a liquid-to-gas phase transition, providing an intrinsic rejection against minimum ionizing particles of order 10$^{-10}$, and reducing the backgrounds to primarily $α$ and neutron-induced recoil events. The droplet phase transition generates a millimetric-sized gas bubble which is recorded by acoustic means…
Bubble chambers and droplet detectors used in dosimetry and dark matter particle search experiments use a superheated metastable liquid in which nuclear recoils trigger bubble nucleation. This process is described by the classical heat spike model of F. Seitz [Phys. Fluids (1958-1988) 1, 2 (1958)], which uses classical nucleation theory to estimate the amount and the localization of the deposited energy required for bubble formation. Here we report on direct molecular dynamics simulations of heat-spike-induced bubble formation. They allow us to test the nanoscale process described in the class…
