耦合在受激喇曼光谱超快脉冲整形选模激发中的作用
On the role of coupling in mode selective excitation using ultrafast pulse shaping in stimulated Raman spectroscopy
摘要:
两个,耦合的两个能级系统,代表半经典模型中的振动模式的相干性,计算在弱和强的领域为各种耦合方案和初始状态振幅之间的不同的相对相位。等于$π$的相对相位将系统投影到暗状态。两个,两个能级系统的选择性激发作为耦合强度和初始相位的函数进行了研究。
英文摘要:
The coherence of two, coupled two-level systems, representing vibrational modes in a semiclassical model, is calculated in weak and strong fields for various coupling schemes and for different relative phases between initial state amplitudes. A relative phase equal to $π$ projects the system into a dark state. The selective excitation of one of the two, two-level systems is studied as a function of coupling strength and initial phases.
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