T. G. Mackay, A. Lakhtakia
The Bruggeman formalism is implemented to estimate the refractive index of an isotropic, dielectric, homogenized composite medium (HCM). Invoking the well--known Hashin--Shtrikman bounds, we demonstrate that the group velocity in certain HCMs can exceed the group velocities in their component materials. Such HCMs should therefore be considered as metamaterials.
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Axionic electrodynamics predicts many peculiar magnetoelectric-based properties. Hitherto, simple structures such as one-dimensional multilayers were employed to explore these axionic magnetoelectric responses, and Fabry-Pérot interference mechanism was frequently applied to augment these effects. In this Letter, we propose a new mechanism, metamaterial-enhanced axionic magnetoelectric response, by taking advantage of intense enhancement of localized electromagnetic fields associated with plasmonic resonances. Through numerical simulations, we show that plasmonic metamaterial can enhance axion…
We examine layered metamaterial structures consisting of alternating films of epsilon-near-zero (ENZ) and dielectric material, and show that for such a stack it is possible to enhance the refractive, reflective or absorptive properties of the ENZ. The proposed structure takes advantage of resonances from several interfaces, guided modes, and plasmon excitations to achieve the desired enhancement, and it is not an effective medium. We use analytical modeling tools to show how the different degrees of freedom affect the properties of the stack, and propose experimentally feasible parameters for …
We suggest double-resonant (binary) metamaterials composed of two types of magnetic resonant elements, and demonstrate that in the nonlinear regime such metamaterials provide unique possibilities for phase-matched parametric interaction and enhanced second-harmonic generation.
Non-radiative coupling between conductive coils is a candidate mechanism for wireless energy transfer applications. In this paper, we propose a power relay system based on a near-field metamaterial superlens, and present a thorough theoretical analysis of this system. We use time-harmonic circuit formalism to describe all interactions between two coils attached to external circuits and a slab of anisotropic medium with homogeneous permittivity and permeability. The fields of the coils are found in the point-dipole approximation using Sommerfeld integrals, which are reduced to standard special …
We verify the extraordinary transmission enhancement and collimation induced by the material loss in anisotropic near-zero permittivity (ENZ) metamaterials, and reveal the physical mechanism of this exotic electromagnetic phenomenon via the iso-frequency contour (IFC) analysis. In addition, we demonstrate the possibility in realization of such loss enhanced transmission of Gaussian beam in realistic silver-germanium multilayered structures by applying full-wave numerical simulations.
Resonant metamaterials usually exhibit substantial dispersion, which is considered a shortcoming for many applications. Here we take advantage of the ability to tailor the dispersive response of a metamaterial introducing a new method of group-velocity dispersion compensation in telecommunication systems. The method consists of stacking a number of highly dispersive sheet metamaterials and is capable of compensating the dispersion of optical fibers with either negative or positive group-velocity dispersion coefficients. We demonstrate that the phase-engineered metamaterial can provide strong g…
We report on a numerical study of optical chirality. Intertwined gold helices illuminated with plane waves concentrate right and left circularly polarized electromagnetic field energy to sub-wavelength regions. These spots of enhanced chirality can be smoothly shifted in position and magnitude by varying illumination parameters, allowing for the control of light-matter interactions on a nanometer scale.
The active and nonlinear graphene properties are limited due to weak light matter interaction between the ultrathin graphene and the incident light. In this work, we present enhanced nonlinear effects at the low terahertz (THz) range by designing a new patterned graphene hyperbolic metamaterial (GHMM). More specifically, it is demonstrated that the third harmonic generation (THG) can be significantly enhanced by the proposed GHMM due to the field enhancement at the resonance as well as the supported slow light response that fosters strong light matter interaction.
We propose that macroscopic objects built from negative-permeability metamaterials may experience resonantly enhanced magnetic force in low-frequency magnetic fields. Resonant enhancement of the time-averaged force originates from magnetostatic surface resonances (MSR) which are analogous to the electrostatic resonances of negative-permittivity particles, well known as surface plasmon resonances in optics. We generalize the classical problem of MSR of a homogeneous object to include anisotropic metamaterials, and consider the most extreme case of anisotropy where the permeability is negative i…
Based on boundary condition and dispersion relation, the superluminal group velocity in an anisotropic metamaterial (AMM) is investigated. The superluminal propagation is induced by the hyperbolic dispersion relation associated with the AMM. It is shown that a modulated Gaussian beam exhibits a superluminal group velocity which depends on the choice of incident angles and optical axis angles. The superluminal propagation does not violate the theory of special relativity because the group velocity is the velocity of the peak of the localized wave packet which does not carry information. It is p…
Designing broadband enhanced chirality is of strong interest to the emerging fields of chiral chemistry and sensing, or to control the spin orbital momentum of photons in recently introduced nanophotonic chiral quantum and classical optical applications. However, chiral light-matter interactions have an extremely weak nature, are difficult to be controlled and enhanced, and cannot be made tunable or broadband. In addition, planar ultrathin nanophotonic structures to achieve strong, broadband, and tunable chirality at the technologically important visible to ultraviolet spectrum still remain el…
In this paper we theoretically show that the Raman scattering by a core-shell micron or submicron particle with epsilon-near-zero metamaterial shell and silica spherical or cylindrical core can combine useful features of cavity-enhanced and surface-enhanced Raman scattering. The cavity resonance together with the plasmon resonance lead to the giant enhancement of the field inside the metashell which is performed as a layer of silver or gold nanoparticles and is penetrable for molecules to be detected. This approach results in the significant increase of both effective volume in which molecules…
The gain-assisted plasmonic analogue of electromagnetically induced transparency (EIT) in a metallic metamaterial is investigated for the purpose to enhance the sensing performance of the EIT-like plasmonic structure. The structure is composed of three bars in one unit, two of which are parallel to each other (dark quadrupolar element) but perpendicular to the third bar (bright dipolar element), The results show that, in addition to the high sensitivity to the refractive-index fluctuation of the surrounding medium, the figure of merit for such active EIT-like metamaterials can be greatly enhan…
We propose a new class of metamaterials called magneto-optical metamaterials that offer enhanced angle of rotation in polarization compared to bulk magneto-optical materials. In the proposed approach, the permittivity tensor of a magneto-optical material is tailored by embedded wire meshes behaving as artificial plasma. We have shown that the angle of rotation in the magneto-optical metamaterial can be enhanced up to 9 times compared to bulk magneto-optical material alone while the polarization extinction ratio remains below -20dB and insertion loss is less than 1.5dB.
Hyperbolic metamaterials, horizontally stacked metal and dielectric multilayer, have recently been studied as a platform to observe optical spin Hall effect. However, the large optical spin Hall effect in the horizontal hyperbolic metamaterials accompanies extremely low transmission, which obstructs its practical applications. Reducing the sample thickness to augment the transmission causes diminishment of the shift. In this letter, we demonstrate that a vertical hyperbolic metamaterial can enhance the shift by several orders of magnitude in comparison to the shift of its horizontal counterpar…
The energy propagation of electromagnetic fields in the effective medium of a one-dimensional photonic crystal consisting of dielectric and metallic layers is investigated. We show that the medium behaves like Drude and Lorentz medium, respectively, when the electric field is parallel and perpendicular to the layers. For arbitrary time-varying electromagnetic fields in this medium, the energy density formula is derived. We prove rigorously that the group velocity of any propagating mode obeying the hyperbolic dispersion must be slower than the speed of light in vacuum, taking into account the …
We demonstrate a nonlinear metamaterial that can be switched between low and high transmission by controlling the power level of the incident beam. The origin of this nonlinear response is the superconducting Nb thin film employed in the metamaterial structure. We show that with moderate RF power of about 22 dBm it is possible to quench the superconducting state as a result of extremely strong current densities at the corners of the metamaterial's split-ring resonators. We measure a transmission contrast of 10 dB and a change in group delay of 70 ns between the low and high power states.
One of the most important goals of condensed matter physics is materials by design, i.e. the ability to reliably predict and design materials with a set of desired properties. A striking example is the deterministic enhancement of the superconducting properties of materials. Recent experiments have demonstrated that the metamaterial approach is capable of achieving this goal, such as tripling the critical temperature Tc in Al-Al2O3 epsilon near zero (ENZ) core-shell metamaterial superconductors. However, transport properties of such metamaterials remained much worse compared to conventional su…
We demonstrate nonlinear metamaterial split ring resonators (SRRs) on GaAs at terahertz frequencies. For SRRs on doped GaAs films, incident terahertz radiation with peak fields of ~20 - 160 kV/cm drives intervalley scattering. This reduces the carrier mobility and enhances the SRR LC response due to a conductivity decrease in the doped thin film. Above ~160 kV/cm, electric field enhancement within the SRR gaps leads to efficient impact ionization, increasing the carrier density and the conductivity which, in turn, suppresses the SRR resonance. We demonstrate an increase of up to 10 orders of m…
We investigate a class of multilayered metamaterials characterized by moderate-index inclusions and low average permittivity. Via first-principle calculations, we show that in such scenario first- and second-order spatial dispersion effects may exhibit a dramatic and non-resonant enhancement, and may become comparable to the local response. Their interplay gives access to a wealth of dispersion regimes encompassing additional extraordinary waves and topological phase transitions. In particular, we identify a novel configuration featuring bound and disconnected isofrequency contours. Since they…
One route to create tunable metamaterials is through integration with "on-demand" dynamic quantum materials, such as vanadium dioxide (VO2). This enables new modalities to create high performance devices for historically challenging applications. Indeed, dynamic materials have often been integrated with metamaterials to imbue artificial structures with some degree of tunability. Conversely, metamaterials can be used to enhance and extend the natural tuning range of dynamic materials. Utilizing a complementary split ring resonator array deposited on a VO2 film, we demonstrate enhanced terahertz…
We propose an approach to enhance and direct the spontaneous emission from isolated emitters embedded inside hyperbolic metamaterials into single photon beams. The approach rests on collective plasmonic Bloch modes of hyperbolic metamaterials which propagate in highly directional beams called quantum resonance cones. We propose a pumping scheme using the transparency window of the hyperbolic metamaterial that occurs near the topological transition. Finally, we address the challenge of outcoupling these broadband resonance cones into vacuum using a dielectric bullseye grating. We give a detaile…
We present an analytical model describing complex dynamics of a hybrid nonlinear system consisting of interacting carbon nanotubes (CNT) and a plasmonic metamaterial. Our model is based on the set of coupled equations, which incorporates well-established density matrix formalism appropriate for quantum systems (CNT are described as a two level system) and harmonic-oscillator approach ideal for modelling sub-wavelength plasmonic and optical resonators. We show that the saturation nonlinearity of CNT increases multifold in the resonantly enhanced near field of a metamaterial. In the framework of…
Optical materials with vanishing dielectric permittivity, known as epsilon-near-zero (ENZ) materials, have been shown to possess enhanced nonlinear optical responses in their ENZ region. These strong nonlinear optical properties have been firmly established in homogeneous materials; however, it is as of yet unclear whether metamaterials with effective optical parameters can exhibit a similar enhancement. Here, we probe an optical ENZ metamaterial composed of a subwavelength periodic stack of alternating Ag and SiO$_2$ layers and measure a nonlinear refractive index $n_2 = (1.2 \pm 0.1) \times …
Simultaneously enhanced reflectance and transmittance greater than 35 dB are demonstrated for the lasing spaser (or spasing) behavior in an active fishnet metamaterial. In mimicking a lasing cavity, an equivalent active slab with Lorentz dispersion for the index of refraction is established to model the spasing metamaterial through the Fabry-Perot effect. Numerical and theoretical results show good agreement in the equal enhancement of reflectance and transmittance, as well as the non-monotonic dependence of the spasing intensity on the gain coefficient. In addition, directed emission of the s…
Ultraviolet (UV) electro-optic modulation system based on graphene-plasmonic metamaterials nanomechanical system (NEMS) with superlubricity is investigated. Due to the strong optical absorption intensity of graphene in the UV region and the combination of metamaterial structure based on surface plasmons, the modulation depth of the UV NEMS electro-optic modulator approaches as high as 8.5 times compared to the counterpart modulator in visible light region. Meanwhile, the superlubricity significantly reduces the power consumption of the UV electro-optic modulation system due to its extremely lo…
Controlling the broadband enhanced light chirality with L-shaped dielectric metamaterials
本文设计了基于倾斜纳米柱的全介电硅基L形超材料，通过掠射角沉积实现晶圆级制备，在透射模式下获得宽带增强且振幅与频率均可调控的手性光学响应。
We derive the formula of the complex Doppler shift in a two-dimensional, dispersive metamaterial and we show that a moving, monochromatic radiation source generates multiple frequency modes. The role of the group velocity is stressed and the Doppler shifted radiation field exhibits features of the Cherenkov effect. The presented theory is also applicable to the case of a moving, nonoscillating charge and explains many peculiar characteristics of the Cherenkov radiation in lefthanded metamaterials such as the backward direction of power emission, the constant radiation angle and the lack of vel…
We present simulation results of a design for negative index materials that uses magnetic resonators to provide negative permeability and metal film for negative permittivity. We also discuss the possibility of using semicontinuous metal films to achieve better manufacturability and enhanced impedance matching.
Optical activation function using a metamaterial waveguide for an all-optical neural network
本研究通过在硅波导中集成超材料结构增强非线性光学系数，提出一种光学激活函数，在手写识别中实现98.36%准确率，助力开发更节能紧凑的全光神经网络。
The authors introduce a general mechanism, based on electrostatic and magnetostatic considerations, for designing three-dimensional isotopic metamaterials that possess an enhanced refractive index over an extremely large frequency range. The mechanism allows nearly independent control of effective electric permittivity and magnetic permeability without the use of resonant elements.
The paper considers an opportunity for the creation of an artificial two-component metamaterial with a negative refractive index within the radio and optical frequency band, which possesses a spatial dispersion. It is shown that there exists a spectral region where, under certain ratio of volume fraction unit occupied with components, the metamaterial appears transparent without attenuating the electromagnetic wave passing through it and possessing a phase and group velocity of the opposite sign.
Space-time varying metamaterials based on uniform-velocity modulation have spurred considerable interest over the past decade. We present here the first extensive investigation of accelerated modulation space-time metamaterials. Using the tools of general relativity, we establish their electrodynamic principles and describe their fundamental phenomena, in comparison with the physics of moving-matter media. We show that an electromagnetic beam propagating in an accelerated modulation metamaterial is bent in its course, which reveals that such a medium curves space-time for light, similarly to g…
Accessing both electrochemical SEIRA and SERS with ultrasensitive metamaterials for enhanced molecular identification
提出一种电化学可清洁的超材料，实现流动中实时联合SEIRA和SERS，通过纳米间隙折射率变化（1400 nm/RIU）实现超灵敏检测，并追踪分子电化学转化和对称性破缺。
Photonic metamaterials are man-made structures composed of tailored micro- or nanostructured metallo-dielectric sub-wavelength building blocks that are densely packed into an effective material. This deceptively simple, yet powerful, truly revolutionary concept allows for achieving novel, unusual, and sometimes even unheard-of optical properties, such as magnetism at optical frequencies, negative refractive indices, large positive refractive indices, zero reflection via impedance matching, perfect absorption, giant circular dichroism, or enhanced nonlinear optical properties. Possible applicat…
We study theoretically the effect of ultraslow phase and group velocities in an anisotropic metamaterial. The ultraslow phase propagation is induced by the hyperbolic dispersion relation. While the inherent physics underlying the slow group velocity are collective operations of the frequency and spatial dispersion. We show that a Gaussian wave packet exhibits simultaneous slow phase and group velocities which depend on the choice of incident angles and principal axis angles. The anisotrocpic metamaterial slab can be constructed and the ultraslow phase and group velocities can be measured exper…
In the close vicinity of a chiral nanostructure, the circular dichroism of a biomolecule could be greatly enhanced, due to the interaction with the local superchiral fields. Modest enhancement of optical activity using a planar metamaterial, with some chiral properties, and achiral nanoparticles has been previously reported. A more substantial chirality enhancement can be achieved in the local filed of a chiral nanostructure with a three-dimensional arrangement. Using an embossed chiral nanostructure designed for chiroptical sensing, we measure the circular dichroism spectra of two biomolecule…
Comment on "Non-reciprocal topological solitons in active metamaterials"
本文指出，活性超材料中非互易拓扑孤子速度的常微分方程不仅可由逆散射变换微扰理论导出，也可由能量平衡方法得到。
We demonstrate a metamaterial that cannot be described by a single set of refractive-index and impedance values, even for fixed frequency and polarization. The metamaterial structure is a stack of dissimilar waveguides with subwavelength width and spacing, which guide light at different phase velocities. This multi-refractive-index metamaterial (MRIM) can be viewed as a spatial superposition of multiple homogeneous materials. Using full-wave simulations, we demonstrate several optical components based on MRIMs, including prisms that deflect light to multiple angles, lenses with multiple focal …
Extraordinary features of optical parametric amplification of Stokes electromagnetic waves are investigated, which originate from three-wave mixing of two ordinary electromagnetic and one backward phonon wave with negative group velocity. A similarity with the counterpart in the negative-index plasmonic metamaterials and differences with those utilizing contra-propagating ordinary electromagnetic waves as well as electromagnetic and acoustic phonon waves are shown. They stem from backwardness of optical phonons with negative dispersion. Nonlinear-optical photonic devices with the properties si…
Enhanced Magneto-Optical Kerr Effect in Nano-Magnetic Metamaterials with Near-Perfect Coherent Absorption
本研究通过相干光学干涉在坡莫合金纳米磁体超表面中实现近完美吸收（>95%），并增强磁光克尔效应，为纳米磁性系统的光控提供通用方案。
Hyperbolic Metamaterials for Enhanced Scintillation
提出光栅耦合双曲超材料，结合CsPbBr₃层与靶心光栅，通过高k模式和双曲共振锥增强闪烁信号，宽带增强超3倍，峰值约5倍，为高性能闪烁体提供实用途径。
Metamaterials offer unprecedented flexibility for manipulating the optical properties of matter, including the ability to access negative index, ultra-high index and chiral optical properties. Recently, metamaterials with near-zero refractive index have drawn much attention. Light inside such materials experiences no spatial phase change and extremely large phase velocity, properties that can be applied for realizing directional emission, tunneling waveguides, large area single mode devices, and electromagnetic cloaks. However, at optical frequencies previously demonstrated zero- or negative-r…
We demonstrate that the broadband nonlinear optical response of graphene can be resonantly enhanced by more than an order of magnitude through hybridization with a plasmonic metamaterial,while retaining an ultrafast nonlinear response time of ~1 ps. Transmission modulation close to ~1% is seen at a pump uence of ~0.03 mJ/cm^2 at the wavelength of ~1600 nm. This approach allows to engineer and enhance graphene's nonlinearity within a broad wavelength range enabling applications in optical switching, mode-locking and pulse shaping.
Multipolar electromagnetic phenomena in sub-wavelength resonators are at the heart of metamaterial science and technology. In this letter, we demonstrate selective and enhanced coupling to specific multipole resonances via beam engineering. We first derive an analytical method for determining the scattering and absorption of spherical nanoparticles (NPs) that depends only on the local electromagnetic field quantities within an inhomogeneous beam. Using this analytical technique, we demonstrate the ability to drastically manipulate the scattering properties of a spherical NP by varying illumina…
High-index dielectric materials are in great demand for nanophotonic devices and applications, from ultrathin optical elements to metal-free sub-diffraction light confinement and waveguiding. Here we show that chalcogenide topological insulators are particularly apt candidates for dielectric nanophotonic architectures in the infrared spectral range by reporting metamaterial resonances in chalcogenide crystals sustained well inside the mid-infrared, choosing Bi$_2$Te$_3$ as case study within this family of materials. Strong resonant modulation of the incident electromagnetic field is achieved t…
We propose a scheme for creating of a maximally entangled state comprising two field quanta. In our scheme, two weak light fields, which are initially prepared in either coherent or polarization states, interact with a composite medium near an interface between a dielectric and a negative index metamaterial. Such interaction leads to a large Kerr nonlinearity, reduction of the group velocity of the light and significant confinement of the light fields while simultaneously avoiding amplitude losses of the incoming radiation. All these considerations make our scheme efficient.
We propose deep-subwavelength optical waveguides based on metal-dielectric multilayer indefinite metamaterials with ultrahigh effective refractive indices. Waveguide modes with different mode orders are systematically analyzed with numerical simulations based on both metal-dielectric multilayer structures and the effective medium approach. The dependences of waveguide mode indices, propagation lengths and mode areas on different mode orders, free space wavelengths and sizes of waveguide cross sections are studied. Furthermore, waveguide modes are also illustrated with iso-frequency contours in…
We study numerically the propagation of two-color light pulses through a metamaterial doped with active atoms such that the carrier frequencies of the pulses are in resonance with two atomic transitions in the $Λ$ configuration and that one color propagates in the regime of positive refraction and the other in the regime of negative refraction. In such a metamaterial, one resonant color of light propagates with positive and the other with negative group velocity. We investigate nonlinear interaction of these forward- and backward-propagating waves, and find self-trapped waves, counter-propagat…
Photoacoustic imaging systems offer a platform with high resolution to explore body tissues, food, and artwork. On the other hand, plasmonics constitutes a source of resonant heating and thermal expansion to generate acoustic waves. However, its associated techniques are seriously limited to laser penetration and nonspecific hyperthermia in the sample. To address this issue, the present work adopts a paradigm shift in photoacoustics. By simulating microparticles made of random composites, the calculated pressure can be made similar or superior to that calculated via plasmonic optoacoustics. Th…
Molecule-by-molecule nanoresolved picosecond Purcell-enhanced emission at room-temperature in hollow plasmonic nanocone metamaterials
本研究提出基于三维空心等离子体纳米晶格的新型材料平台，结合单分子超分辨成像与时间相关单光子计数技术，实现纳米级分辨的三维电磁场传感与光-物质相互作用精准调控，可用于室温单光子源调控及分子传感等量子应用。
A wedge-shaped structure made of split-ring resonators (SRR) and wires is numerically simulated to evaluate its refraction behavior. Four frequency bands, namely, the stop band, left-handed band, ultralow-index band, and positive-index band, are distinguished according to the refracted field distributions. Negative phase velocity inside the wedge is demonstrated in the left-handed band and the Snell's law is conformed in terms of its refraction behaviors in different frequency bands. Our results confirmed that negative index of refraction indeed exists in such a composite metamaterial and also…
A new formalism for electromagnetic and mechanical momenta in a metamaterial is developed by means of the technique of wave-packet integrals. The medium has huge mass density and can therefore be regarded as almost stationary upon incident electromagnetic waves. A clear identification of momentum density and momentum flow, including their electromagnetic and mechanical parts, is obtained by employing this formalism in a lossless dispersive metamaterial (including the cases of impedance matching and mismatching with vacuum). It is found that the ratio of the electromagnetic momentum density to …
Extreme mid-infrared field enhancement and anapoles in high-index plasmonic metamaterials
本文基于金纳米颗粒自组装超材料，实现中红外波段有效折射率超过15且间隙场增强两个数量级，并通过设计支持anapole的紧凑超材料器件进一步增强纳米间隙场，使量子发射器的受激辐射响应增强三个数量级。
We investigate numerically the use of a negative-permeability "perfect lens" for enhancing wireless power transfer between two current carrying coils. The negative permeability slab serves to focus the flux generated in the source coil to the receiver coil, thereby increasing the mutual inductive coupling between the coils. The numerical model is compared with an analytical theory that treats the coils as point dipoles separated by an infinite planar layer of magnetic material [Urzhumov et al., Phys. Rev. B, 19, 8312 (2011)]. In the limit of vanishingly small radius of the coils, and large wid…
Photonic metamaterials allow for a range of exciting applications unattainable with ordinary dielectrics. However, the metallic nature of their meta-atoms may result in increased optical losses. Gain-enhanced metamaterials are a potential solution to this problem, but the conception of realistic, three-dimensional designs is a challenging task. Starting from fundamental electrodynamic and quantum-mechanical equations we establish and deploy a rigorous theoretical model for the spatial and temporal interaction of lightwaves with free and bound electrons inside and around metallic (nano-) struct…
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