We have demonstrated a recoil-free spectroscopy on the ${}^1S_0-{}^3P_1$ transition of strontium atoms confined in a one-dimensional optical lattice. By investigating the wavelength and polarization dependence of the ac Stark shift acting on the ${}^1S_0$ and ${}^3P_1(m_J=0)$ states, we determined the {\it magic wavelength} where the Stark shifts for both states coincide. The Lamb-Dicke confinement provided by this Stark-free optical lattice enabled the measurement of the atomic spectrum free from Doppler as well as recoil shifts.
We report high-precision calculations of the nuclear recoil effect to the Lamb shift of hydrogen-like atoms to the first order in the electron-nucleus mass ratio and to all orders in the nuclear binding strength parameter $Zα$. The results are in excellent agreement with the known terms of the $Zα$ expansion and allow an accurate identification of the nonperturbative higher-order remainder. For hydrogen, the higher-order remainder was found to be much larger than anticipated. This result resolves the long-standing disagreement between the numerical all-order and the analytical $Zα$-expansion a…
We propose a scheme that combines velocity-selective coherent population trapping (CPT) and Raman sideband cooling (RSC) for subrecoil cooling of optically trapped atoms outside the Lamb-Dicke regime. This scheme is based on an inverted $\mathsf{Y}$ configuration in an alkali-metal atom. It consists of a $Λ$ formed by two Raman transitions between the ground hyperfine levels and the $D$ transition, allowing RSC along two paths and formation of a CPT dark state. Using state-dependent difference in vibration frequency of the atom in a circularly polarized trap, we can tune the $Λ$ to make only t…
The diffraction of fast atoms at crystal surfaces is ideal for a detailed investigation of the surface electronic density. However, instead of sharp diffraction spots, most experiments show elongated streaks characteristic of inelastic diffraction. This paper describes these inelastic profiles in terms of individual inelastic collisions with surface atoms taking place along the projectile trajectory and leading to vibrational excitation of the local Debye oscillator. A quasi-elastic regime where only one inelastic event contributes is identified as well as a mixed quantum-classical regime were…
Accurate calculations of the nuclear recoil effect to the Lamb shift of hydrogen-like atoms are presented. Numerical results are reported for the $ns$ states with $n \leq 5$ and for the $2p_{1/2}$ and $2p_{3/2}$ states. The calculations are performed to the first order in the electron-nucleus mass ratio and to all orders in the nuclear binding strength parameter $Zα$ (where $Z$ is the nuclear charge number and $α$ is the fine structure constant). The obtained results provide accurate predictions for the higher-order remainder beyond the known $Zα$-expansion terms. In the case of hydrogen, the …
We study the feasibility of nearly-degenerate two-photon rovibrational spectroscopy in ensembles of trapped, sympathetically cooled hydrogen molecular ions using a resonance-enhanced multiphoton dissociation (REMPD) scheme. Taking advantage of quasi-coincidences in the rovibrational spectrum, the excitation lasers are tuned close to an intermediate level to resonantly enhance two-photon absorption. Realistic simulations of the REMPD signal are obtained using a four-level model that takes into account saturation effects, ion trajectories, laser frequency noise and redistribution of population b…
We investigate the dynamics of cavity cooling of a single ion beyond the Lamb-Dicke regime and demonstrate a cooling limit of approximately 50% of the Doppler temperature using a high finesse cavity for the first time. We also study the statistical properties of the ion-cavity emission and present a model that maps the phonon states to the photon states. With this model, we explain the super-Poissonian photon distribution observed in our experiments and propose a method to estimate the ion temperature in a real-time manner based on the statistical behavior of the photon emission from the cavit…
Unlike photons, which are conveniently handled by mirrors and optical fibres without loss of coherence, atoms lose their coherence via atom-atom and atom-wall interactions. This decoherence of atoms deteriorates the performance of atomic clocks and magnetometers, and also hinders their miniaturisation. Here we report a novel platform for precision spectroscopy. Ultracold strontium atoms inside a kKagome-lattice hollow-core photonic crystal fibre (HC-PCF) are transversely confined by an optical lattice to prevent atoms from interacting with the fibre wall. By confining at most one atom in each …
We apply wave packet methods to study an ion-trap system in the strong excitation regime imposing neither the rotating wave nor the Lamb-Dicke approximations. By this approach we show the existence of states with restricted phase space evolution, as a genuine consequence of quantum interference between wave packet fractions. A particular instance of such a state oscillates between maximal entanglement and pure disentanglement between the constitute subsystems. The characteristic crossover time is very rapid making them suitable for state preparations of EPR or Schrodinger cat states. Over long…
We report continuous Raman sideband cooling (CRSC) of a long ion chain to the motional ground state beyond the Lamb-Dicke (LD) regime. By driving multiple sideband transitions simultaneously, we show that nearly all axial modes of a 24-ion chain are cooled to the ground state, with an LD parameter as large as $η= 1.3$, spanning a frequency bandwidth of 4 MHz. Compared to traditional ground-state cooling methods such as pulsed sideband cooling or electromagnetic-induced-transparency (EIT) cooling, our method offers two key advantages: robustness to timing errors; and an ultra-wide bandwidth unl…
We present the results of simulations of optical sideband cooling of atomic ions in a trap with a shallow potential well. In such traps, an ion cannot be Doppler cooled near to the Lamb-Dicke regime ($η^2(2n+1) \ll 1$). Outside the Lamb-Dicke regime, the sideband cooling dynamics are altered by the existence of various Fock states where the cooling becomes very slow. A calcium ion trapped in our Penning trap realises such a situation, hence single stage cooling is inefficient to prepare the ion in the motional ground state. For these systems, it is necessary to study the cooling dynamics in de…
The results and main steps of an analytic calculation of radiative-recoil corrections of order $α(Zα)^5(m/M)m$ to the Lamb shift in hydrogen are presented. The calculations are performed in the infrared safe Yennie gauge. The discrepancy between two previous numerical calculations of these corrections existing in the literature is resolved. Our new result eliminates the largest source of the theoretical uncertainty in the magnitude of the deuterium-hydrogen isotope shift.
We report Raman sideband cooling of a single sodium atom to its three-dimensional motional ground state in an optical tweezer. Despite a large Lamb-Dicke parameter, high initial temperature, and large differential light shifts between the excited state and the ground state, we achieve a ground state population of $93.5(7)$% after $53$ ms of cooling. Our technique includes addressing high-order sidebands, where several motional quanta are removed by a single laser pulse, and fast modulation of the optical tweezer intensity. We demonstrate that Raman sideband cooling to the 3D motional ground st…
The Lamb shift in muonic hydrogen was measured some time ago to a high accuracy. The theoretical prediction of this value is very sensitive to the proton-finite-size effects. The proton radius extracted from muonic hydrogen is in contradiction with the results extracted from elastic electron-proton scattering. That creates a certain problem for the interpretation of the results from the muonic hydrogen Lamb shift. For the latter we need also to take into account the two-photon-exchange contribution with the proton finite size involved. The only way to describe it relies on the data from the sc…
We demonstrate the laser cooling of 85Rb atoms in a two-dimensional optical lattice. We follow the two-step degenerate Raman sideband cooling scheme [Kerman et al., Phys. Rev. Lett. 84, 439 (2000)], where a fast cooling of atoms to an auxiliary state is followed by a slow cooling to a dark state. This method has the advantage of independent control of the heating rate and cooling rate from the optical pumping beam. We operate the lattice at a Lamb-Dicke parameter eta=0.45 and show the cooling of spin-polarized 85Rb atoms to the recoil temperature in both dimension within 2.4 ms with the aid of…
Sympathetic cooling of trapped ions has been established as a powerful technique for manipulation of non-laser-coolable ions (Raizen1992,Waki1992,Bowe1999,Barrett2003). For molecular ions, it promises vastly enhanced spectroscopic resolution and accuracy. However, this potential remains untapped so far, with the best resolution achieved being not better than $5\times10^{-8}$ fractionally, due to residual Doppler broadening being present in ion clusters even at the lowest achievable translational temperatures (Bressel2012). Here we introduce a general and accessible approach that enables Dopple…
We propose and demonstrate a scheme for strongly radially confining a single neutral atom in a bichromatic far-off resonance optical dipole trap(BFORT) . BFORT is composed of a blue-detuned Laguerre-Gaussian $LG^1_ 0$ beam and a red-detuned Gaussian beam. The trapping radial dimension of a single atom trapped in the Gaussian FORT can be greatly compressed by imposing a blue-detuned Laguerre-Gaussian $LG^1_ 0$ beam with moderate potential depth. By modulating the potential depth of the Gaussian FORT we observed that the resonant and parametric excitation of the oscillatory motion of a single at…
Corrections to energy levels in light muonic atoms are investigated in order $α^2(Zα)^4m$. We pay attention to corrections which are specific for muonic atoms and include the electron vacuum polarization loop. In particular, we calculate relativistic and relativistic-recoil two-loop electron vacuum polarization contributions. The results are obtained for the levels with $n=1,2$ and in particular for the Lamb shift ($2p_{1/2}-2s_{1/2}$) and fine-structure intervals ($2p_{3/2}-2p_{1/2}$) in muonic hydrogen, deuterium, and muonic helium ions.
The current discrepancy of theory and experiment observed recently in muonic hydrogen necessitates a reinvestigation of all corrections to contribute to the Lamb shift in muonic hydrogen muH, muonic deuterium muD, the muonic 3He ion, as well as in the muonic 4He ion. Here, we choose a semi-analytic approach and evaluate a number of higher-order corrections to vacuum polarization (VP) semi-analytically, while remaining integrals over the spectral density of VP are performed numerically. We obtain semi-analytic results for the second-order correction, and for the relativistic correction to VP. T…
We calculate radiative corrections to the Lamb shift of order $α^3(Zα)^5m$ and radiative corrections to hyperfine splitting of order $α^3(Zα)E_F$ generated by the diagrams with insertions of radiative photons and electron polarization loops in the graphs with two external photons. We also obtain the radiative-recoil correction to hyperfine splitting in muonium generated by the diagrams with the $τ$ polarization loop.
We review the theory of the Lamb shift for muonium, provide an updated numerical value and present the prospects of the Mu-MASS collaboration at PSI to improve upon their recent measurement. Due to its smaller nuclear mass, the contributions of the higher-order recoil corrections (160kHz level) and nucleus self-energy 40kHz level) are enhanced for muonium compared to hydrogen where those are below the level of the latest measurement performed by Hessels et al. and thus could not be tested yet. The ongoing upgrades to the Mu-MASS setup will open up the possibility to probe these contributions a…
We present a precise calculation of the Lamb shift $(2P_{1/2}-2S_{1/2})$ in muonic ions $(μ^6_3Li)^{2+},~(μ^7_3Li)^{2+}$, $(μ^9_4Be)^{3+},~(μ^{10}_4Be)^{3+}$, $(μ^{10}_5B)^{4+},~(μ^{11}_5B)^{4+}$. The contributions of orders $α^3\divα^6$ to the vacuum polarization, nuclear structure and recoil, relativistic effects are taken into account. Our numerical results are consistent with previous calculations and improve them due to account of new corrections. The obtained results can be used for the comparison with future experimental data, and extraction more accurate values of nuclear charge radii.
To describe the grazing scattering of keV atoms at surface, a new quantum binary collision model have been proposed where the dynamical properties of the surface atoms are considered via the wave-function of the local Debye harmonic oscillator. This leads to a finite probability of elastic scattering where the momentum transferred during the successive binary collisions is not associated with a change of energy. This Lamb-Dicke regime of the multiple collisions at the surface produces the same coherence ratio as the modified Debye-Waller factor adapted to grazing angle fast atom diffraction (G…
Supplementary information is presented on the recent work by W. Kim et al. on the matter-wave-tunneling-induced broadening in the near-resonant spectra of a single rubidium atom localized in a three-dimensional optical lattice in a strong Lamb-Dicke regime.
Hadronic vacuum polarization in hydrogen-like atoms and ions amid the interplay of recoil and finite-size effects
Institut für Kernphysik and PRISMA ++ Cluster of Excellence, Johannes Gutenberg-Universität Mainz（美因茨约翰内斯·古腾堡大学核物理研究所与PRISMA++卓越集群）；LPNHE, Sorbonne Université, Université Paris Cité, CNRS/IN2P3（巴黎萨克雷大学、巴黎西岱大学及法国国家科学研究中心/欧洲核子研究组织高能物理实验室）
An ultra-stable optical clock based on coherent population trapping effect of alkaline-earth ions, such as Ca$^+$, Sr$^+$, Ba$^+$, is analyzed here. The proposed transitions use the odd isotopes, so that the frequency shift is insensitive to the applied magnetic field. To enhance the signal, a large number of ions are trapped in a linear Paul trap, and laser cooled to crystallize such that the ions are in the Lamb-Dicke regime to avoid first order Doppler shift. Other relevant frequency shifts are also analyzed. Further techniques to improve the stability of the clock signal are discussed.
We consider the $1s$ Lamb shift in hydrogen and helium ions, a quantity, required for an accurate determination of the Rydberg constant and the proton charge radius by means of hydrogen spectroscopy, as well as for precision tests of the bound-state QED. The dominant QED contribution to the uncertainty originates from $α^8m$ external-field contributions (i.e., the contributions at the non-recoil limit). We discuss the two- and three-loop cases and in particular, we revisit calculations of the coefficients $B_{61}, B_{60}, C_{50}$ in standard notation. We have found a missing logarithmic contri…
The electron Lamb shift $(2P-2S)$ and the energy interval $(2S-1S)$ in muon-electron ions of lithium, beryllium, and boron have been calculated within the framework of the perturbation theory method for the fine structure constant and the electron-muon mass ratio. The corrections of the first and second orders of the perturbation theory, which include the effects of vacuum polarization, nuclear structure and recoil, are taken into account. The obtained analytical results in perturbation theory are compared with the results of calculations within the variational approach. The obtained values fo…
In a recent paper, we have proposed a novel laser cooling scheme for reducing collisional energy of a pair of atoms by using photoassociative transitions. In that paper, we considered two atoms in free space, that is we have not considered the effects of trap on the cooling process. Here in this paper, we qualitatively discuss the possibility of extending this idea for Raman sideband cooling of a pair of interacting atoms trapped in Lamb-Dicke (LD) regime. Apart from cooling, our method may be important for manipulating on-site interaction of atoms in an optical lattice.
We demonstrate quantum entanglement of two trapped atomic ion qubits using a sequence of ultrafast laser pulses. Unlike previous demonstrations of entanglement mediated by the Coulomb interaction, this scheme does not require confinement to the Lamb-Dicke regime and can be less sensitive to ambient noise due to its speed. To elucidate the physics of an ultrafast phase gate, we generate a high entanglement rate using just 10 pulses, each of $\sim20$ ps duration, and demonstrate an entangled Bell-state with $(76\pm1)$% fidelity. These results pave the way for entanglement operations within a lar…
Spin-dependent optical potentials allow us to use microwave radiation to manipulate the motional state of trapped neutral atoms (Förster et al. 2009 Phys. Rev. Lett. 103, 233001). Here, we discuss this method in greater detail, comparing it to the widely-employed Raman sideband coupling method. We provide a simplified model for sideband cooling in a spin-dependent potential, and we discuss it in terms of the generalized Lamb-Dicke parameter. Using a master equation formalism, we present a quantitative analysis of the cooling performance for our experiment, which can be generalized to other exp…
We control the quantum mechanical motion of neutral atoms in an optical lattice by driving microwave transitions between spin states whose trapping potentials are spatially offset. Control of this offset with nanometer precision allows for adjustment of the coupling strength between different motional states, analogous to an adjustable effective Lamb-Dicke factor. This is used both for efficient one-dimensional sideband cooling of individual atoms to a vibrational ground state population of 97%, and to drive coherent Rabi oscillation between arbitrary pairs of vibrational states. We further sh…
We present an experimental study of a four beam optical lattice using the light scattered by the atoms in the lattice. We use both intensity correlations and observations of the transient behavior of the scattering when the lattice is suddenly switched on. We compare results for 3 different configurations of the optical lattice. We create situations in which the Lamb-Dicke effect is negligible and show that, in contrast to what has been stated in some of the literature, the damping rate of the 'coherent' atomic oscillations can be much smaller than the inelastic photon scattering rate.
