自组织动态反应器：产物-凝聚体反馈加速反应
Self-Organized Dynamic Reactors: Product-Condensate Feedback Accelerates Reactions
浏览论文内容
中文总结 AI 辅助
本研究提出产物-凝聚体反馈机制，通过自发对称性破缺使凝聚体动态重组，在保留反应物富集的同时移离产物，从而加速反应，适用于生物与合成系统。
中文摘要 AI 辅助
凝聚体可通过富集反应物来加速反应，然而产物积累会消除这一优势。我们表明，产物诱导的凝聚抑制通过自发对称性破缺产生旋转、变形和传播的凝聚体域。它们的重组将反应位点移离积累的产物，同时保留反应物富集，从而获得高于静态凝聚体和均相状态的速率。因此，反应流可将凝聚体自组织为动态反应器，这对生物和合成系统具有重要意义。
英文摘要
Condensates can accelerate reactions by concentrating reactants, yet product accumulation can eliminate this advantage. We show that product-induced suppression of condensation generates rotating, deforming, and propagating condensate domains through spontaneous symmetry breaking. Their reorganization shifts reaction sites away from accumulated products while retaining reactant enrichment, yielding rates above those of static condensates and homogeneous states. Reaction flows can thus self-organize condensates into dynamic reactors, with implications for biological and synthetic systems.
发表机构
- Niels Bohr Institute, University of Copenhagen（尼尔斯·玻尔研究所，哥本哈根大学）
机构由 AI 辅助整理，请以论文原文为准。
