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近魔角扭曲双层化学气相沉积石墨烯中平带的直接观测

Direct observation of flat bands in near-magic-angle twisted bilayer CVD graphene

Gianluigi Baiardi, Alex Boschi, Giulia Piccinini, Vaidotas Mišeikis, Lorenzo Cavicchi, Aaron Bostwick, Chris Jozwiak, Eli Rotenberg, Kenji Watanabe, Takashi Taniguchi, Marco Polini, Fabio Beltram, Antonio Rossi, Stiven Forti, Sergio Pezzini, Camilla Coletti

arXiv 2609.02403首次发表:更新:

发表机构

Istituto Italiano di Tecnologia; Scuola Normale Superiore; Lawrence Berkeley National Laboratory; National Institute for Materials Science; Università di Pisa; Istituto Nanoscienze - CNR(意大利理工大学; 比萨高等师范学院; 劳伦斯伯克利国家实验室; 国立材料研究所; 比萨大学; 纳米科学研究所-国家研究委员会)

机构由 AI 辅助整理,请以论文原文为准。

AI 中文总结

本研究通过室温nano-ARPES,在生长-堆叠法制备的近魔角CVD TBG样品中直接观测到平带,其电子能带与剥离法样品可比,畴尺寸适配输运实验,推动CVD石墨烯平带物理研究。

AI 中文摘要

化学气相沉积(CVD)技术的进展已将石墨烯晶体质量提升至前所未有的水平,但仍未知该路线能否实现魔角(MA)扭曲双层石墨烯(TBG)中脆弱的平带及关联态。本研究采用基于铜上石墨烯低压CVD的生长-堆叠协议组装的近MA TBG样品,通过室温纳米角分辨光电子能谱(nano-ARPES)实验观测到了平带。研究表明,其电子能带与机械剥离法制备样品的测量结果完全可比,且确定了最大近MA畴的尺寸与电子输运实验兼容,为CVD石墨烯平带物理的进一步实验提供了动力。

英文摘要

Advances in chemical vapor deposition (CVD) growth have driven graphene crystal quality to unprecedented levels, yet it is still unknown whether this route can realize the fragile flat-band and correlated states of the magic-angle (MA) twisted bilayer graphene (TBG). Here, we report on the experimental observation by room-temperature nano-angle-resolved photoemission spectroscopy (nano-ARPES) of flat bands in a TBG sample close to the MA, assembled via a grow-and-stack protocol based on low-pressure CVD of graphene on copper. Our study indicates electronic bands fully comparable to those measured in exfoliation-based samples and determines the size of the largest near-MA domain to be compatible with electronic transport experiments, motivating further experiments on flat band physics in CVD-graphene.

DOI:10.1021/acs.nanolett.6c01400

论文原文

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