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光发射及其逆过程的统一理论框架:互易性、自旋与光子偏振

A Unified Theoretical Framework for Photoemission and Its Inverse: Reciprocity, Spin, and Photon Polarization

Frank O. Schumann, Jürgen Henk

arXiv 2608.20192首次发表:更新:

AI 中文总结

该研究提出SARPES与SARIPES的统一理论框架,基于响应张量利用偏振层析成像重构张量元素,以W(110)表面为例,实现从SARPES计算直接预测SARIPES强度。

AI 中文摘要

我们提出了自旋分辨角分辨光电子能谱(SARPES)及其逆过程(SARIPES)的统一理论框架,将二者置于同等地位处理。该公式基于一个响应张量,其编码了两个过程之间的互易性。我们证明,SARPES计算中的偏振层析成像为重构张量元素提供了系统途径。对称性约束使独立分量的数量显著减少,进而可得到描述自旋反转过程和强度调制的显式表达式。该形式主义以W(110)表面为例进行说明。所得框架提供了表面自旋依赖光跃迁的对称性适配描述,可从SARPES计算直接预测SARIPES强度。

英文摘要

We present a unified theoretical framework for spin- and angle-resolved photoemission spectroscopy (SARPES) and its inverse process (SARIPES), treating both on an equal footing. The formulation is based on a response tensor that encodes the reciprocity between the two processes. We show that polarization tomography within SARPES calculations provides a systematic route for reconstructing the tensor elements. The number of independent components is significantly reduced by symmetry constraints, which in turn allows for explicit expressions describing spin-reversal processes and intensity modulations. The formalism is illustrated for the W(110) surface. The resulting framework provides a symmetry-adapted description of spin-dependent optical transitions at surfaces and enables the direct prediction of SARIPES intensities from SARPES calculations.

Comments27 pages, 7 Figures

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