石墨烯中取代式Mn的共振缺陷散射的光谱指纹
Spectral Fingerprints of Resonant Defect Scattering by Substitutional Mn in Graphene
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中文总结 AI 辅助
研究以石墨烯/Cu(111)的取代式Mn为模型点缺陷,结合STM与ARPES验证共振散射指纹,确定Mn为强共振散射体,建立了表征石墨烯共振无序的有效方法。
中文摘要 AI 辅助
以石墨烯/Cu(111)中的取代式Mn作为模型点缺陷,我们结合扫描隧道显微镜(STM)与角分辨光电子能谱(ARPES)对预测的共振散射指纹进行验证。当Mn浓度升至0.44%时,狄拉克点展宽达到0.52 eV,而动量展宽与能量无关。这些光谱指纹将取代式Mn归类为强共振散射体,并确立STM与ARPES的组合是识别和表征石墨烯中共振无序的有力方法。
英文摘要
Using substitutional Mn in graphene/Cu(111) as a model point defect, we combine scanning tunneling microscopy (STM) and angle-resolved photoemission spectroscopy (ARPES) to test the predicted fingerprints of resonant scattering. As the Mn concentration increases to 0.44%, the Dirac point stretching reaches 0.52 eV, while momentum broadening remains energy independent. These spectral fingerprints classify substitutional Mn as a strong resonant scatterer and establish the combination of STM and ARPES as a powerful approach to identify and characterize resonant disorder in graphene.