arXivDaily arXiv每日学术速递 周一至周五更新
arXiv周末暂无论文更新,休息一下吧,周末愉快~~

亚周期多带电子动力学的脉冲持续时间控制拓展光驱动绝缘体中的高次谐波截止频率

Pulse-Duration Control of Subcycle Multiband Electron Dynamics Extends the High-Harmonic Cutoff in a Light-Driven Insulator

Hortense Allegre, Simon V. B. Jensen, Joseph J. Broughton, Tim Klee, Yan Li, Jon P. Marangos, Nicolas Tancogne-Dejean, Angel Rubio, John W. G. Tisch, Mary R. Matthews

arXiv 2608.06129首次发表:更新:

AI 中文总结

该研究通过调控激光脉冲的持续时间与强度,控制光驱动绝缘体的亚周期多带电子动力学,实现高次谐波产生的路径选择性,将高次谐波截止能量拓展至25-50 eV,为高能极紫外光源设计提供了新方法。

AI 中文摘要

我们通过联合调控激光脉冲持续时间(5-29 fs)和强度(0.8-74 TW/cm²),实现了对极紫外高次谐波产生的路径选择性控制。中等强度(约6 TW/cm²)的多周期脉冲会促使载流子在连续光学周期内发生累积转移,逐步占据更高的导带;相比之下,少周期、高强度(约22 TW/cm²)的脉冲则会驱动亚周期多带动力学,在退相干抑制相干发射前达到25-50 eV的光子能量。这些结果表明,脉冲持续时间和强度是调控高次谐波发射的关键旋钮,为设计基于能带结构的更高能量极紫外光源开辟了途径。

英文摘要

We demonstrate pathway-selective control of extreme-ultraviolet high-harmonic generation by jointly tuning laser pulse duration ($5$ - $29$ fs) and intensity ($0.8$ - $74$ TW/cm$^2$). Many-cycle pulses at moderate intensities, $\sim 6$ TW/cm$^2$, promote cumulative carrier transfer over successive optical cycles, progressively accessing higher conduction bands. In contrast, few-cycle, high-intensity, $\sim 22$ TW/cm$^2$, pulses drive subcycle multiband dynamics that reach $25$ - $50$ eV photon energies before decoherence can suppress coherent emission. These results reveal pulse duration and intensity as decisive control knobs for high-harmonic emission, opening a route to band-structure-guided pulse design for higher energy extreme-ultraviolet light sources.

论文原文

arXiv 摘要页 · PDF 原文 · HTML 原文

↑