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统一声子磁效应的微观理论

Unifying microscopic theories for the phono-magnetic effect

Natalia Shabala, Finja Tietjen, Ylva Liljegren, R. Matthias Geilhufe

arXiv 2608.04754首次发表:更新:

AI 中文总结

本文对比三种方法推导声子有效磁场,证明其在低频极限下等效,确定声子对磁化的两类贡献,为声子磁效应建立统一理论提供关键基础。

AI 中文摘要

声子角动量会诱导出有效磁场,这一现象被称为声子磁效应,已测得其大小存在显著差异。本文利用电子-声子耦合与轨道磁性,对比了三种推导声子有效磁场的方法:绝热方法假设离子运动缓慢,使电子保持在基态;微扰方法将电子-声子相互作用视为对电子基态的微扰;弗洛凯方法则基于离子圆周运动的时间周期性。我们证明,在低频极限下,这三种方法均能得到相同的有效哈密顿量,这使我们更接近建立声子磁效应的统一理论。此外,我们确定了样品磁化强度的两种声子贡献:自发贡献与感应贡献,从而阐明了有效磁场在声子诱导磁化强度中的作用。最后,我们给出了SrTiO₃中有效磁场的数值估计。

英文摘要

Phonon angular momentum induces an effective magnetic field, a phenomenon called phono-magnetic effect, which has been measured to vary significantly in size. Here, we compare three approaches for deriving the effective magnetic field of a phonon, using electron-phonon coupling and orbital magnetism. The adiabatic approach assumes a slow ionic motion, keeping electrons in the ground state. The perturbative approach treats the electron-phonon interaction as a perturbation to the electronic ground state, and the Floquet approach is based on the time-periodicity of the circular ionic motion. We show that all three approaches lead to the same effective Hamiltonian in the low-frequency limit, which moves us closer towards a unified theory of the phono-magnetic effect. Furthermore, we identify two phononic contributions to the sample magnetization, spontaneous and induced. Thus, we clarify the role of the effective magnetic field in the phonon-induced magnetization. We conclude by providing a numerical estimate for the effective magnetic field in SrTiO$_3$.

Comments10 pages, 2 figures

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