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铁电反铁磁体界面拓扑绝缘体中的电场控制自旋输运

Electric field controlled spin transport in a topological insulator interfaced with a ferroelectric antiferromagnet

Yogesh Kumar, Pushpendra Gupta, Xinyan Li, Richa Mudgal, Ashish Omar, Ryan Chen, Mito Funatsu, Maya Ramesh, Nicholas Reiterer, Yuanqi Lyu, Yiping Zeng, Darrell G. Schlom, Alessandra Lanzara, Robert J. Birgeneau, James G. Analytis, Ramamoorthy Ramesh, Sajid Husain

arXiv 2607.14031首次发表:更新:

AI 中文总结

研究拓扑绝缘体Bi$_2$Te$_3$与反铁磁多铁性BiFeO$_3$界面的自旋-电荷转换,利用非局部自旋输运装置,通过研究自旋输运厚度依赖性揭示拓扑表面态主导特征,展示了高效转换,突出Bi$_2$Te$_3$平台价值,为自旋基器件设计提供途径。

AI 中文摘要

拓扑绝缘体通过磁界面的自旋-电荷相互转换已被广泛研究,但其自旋-电荷转换的真实响应,尤其是在没有外部磁场的情况下,仍有待研究。本文利用非局部自旋输运装置,报道了在拓扑绝缘体Bi$_2$Te$_3$与反铁磁多铁性BiFeO$_3$中自旋-电荷转换的电场控制。系统研究了Bi$_2$Te$_3$和BiFeO$_3$界面自旋输运的厚度依赖性,揭示了双层系统中拓扑表面态主导的自旋输运特征。自旋-电荷转换在厚度大于10nm时保持稳健,但随厚度减小而迅速下降,在5nm时消失,这与平凡绝缘相的出现一致。这些结果表明自旋-动量锁定表面态在解耦状态下主导界面自旋输运。这项工作不仅展示了在完全绝缘磁界面上的高效自旋-电荷相互转换,还突出了溅射沉积的Bi$_2$Te$_3$作为将量子材料集成到器件中的高质量、可扩展平台。本文提出的非局部自旋输运方法为自旋-电荷转换提供了简单直接的证据,并为设计节能自旋基器件开辟了有效实用的途径。

英文摘要

Topological insulators have been explored extensively for spin-charge interconversion via magnetic interfaces, yet the true response of their spin-charge conversion, particularly in the absence of an external magnetic field, remains to be studied. Here, we report electric-field control of spin-charge conversion in the topological insulator Bi$_2$Te$_3$ with the antiferromagnetic multiferroic BiFeO$_3$, employing a nonlocal spin transport device. A systematic thickness dependence of the spin transport across the interface between Bi$_2$Te$_3$ and BiFeO$_3$ reveals a signature of topological surface-state-dominated spin transport in the bilayer system. The spin-charge conversion remains robust for thicknesses above 10 nm but falls rapidly with reducing thickness and vanishes at 5 nm. This is consistent with the hybridization-induced emergence of a trivial insulating phase, which is supported by the coherency factor estimated from the magnetoconductance of Bi$_2$Te$_3$. These results establish that spin-momentum-locked surface states dominate interfacial spin transport in the decoupled regime. Beyond presenting efficient spin-charge interconversion at an entirely insulating magnetic interface, this work also highlights sputter-deposited Bi$_2$Te$_3$ as a high-quality and scalable platform for integrating quantum materials into devices. The nonlocal spin transport approach presented here provides a simple and direct evidence of spin-charge conversion and opens an efficient and practical pathway toward designing energy-efficient spin-based devices.

Comments23 pages, 4 Figures

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