Nonlinear 2D materials such as 3R-phase molybdenum disulfide (3R-MoS2) offer strong second-order optical nonlinearities in an atomically thin platform, making them attractive for on-chip frequency conversion, quantum light generation, and integrated nonlinear nanophotonics. However, the second harmonic generation (SHG) efficiency of monolayer or few-layer 3R-MoS2 deposited on planar substrates remains fundamentally limited by weak light-matter interaction, poor phase matching, and small interaction volumes. Here, we introduce NanoPhotoNet-PINL, a physics informed AI-driven inverse design framework based on a hybrid one-dimensional convolutional neural network and deep neural network autoencoder, tailored for nonlinear MLMs metasurfaces. The model directly maps target dual-resonant reflection spectra at the fundamental and second-harmonic wavelengths to the required multi-layer geometries and material compositions that maximize the effective nonlinear overlap with an embedded 3R-MoS2 sheet. By integrating Maxwell-based nonlinear electrodynamics into the inverse design loop, we compute the second-harmonic conversion efficiency and modal overlap factors for each predicted MLMs design, enabling physics-guided training and evaluation. Our approach achieves an inverse-design prediction efficiency exceeding ~99.2 % along the linear spectral manifold, while the optimized dual-resonant MLMs yield more than three orders of magnitude enhancement in SHG intensity compared to a bare 3R-MoS2 flake on a planar substrate. NanoPhotoNet-PINL establishes a generalizable paradigm for intelligent inverse design of nonlinear multi-layer metasurfaces and phase-matched dual-resonant cavities for high-efficiency second-order processes.
Frequency conversion of light can be dramatically enhanced using high quality factor ($Q$-factor) cavities. Unfortunately, the achievable conversion efficiencies and conversion bandwidths are fundamentally limited by the time-bandwidth limit of the cavity, restricting their use in frequency conversion of ultrashort pulses. Here, we propose and numerically demonstrate sum-frequency generation based frequency conversion using a metasurface-based cavity configuration that could overcome this limitation. The proposed experimental configuration takes use of the spatially dispersive responses of per…
An invisible cavity is an open resonant device that confines a localized field without producing any scattering outside of the device volume. By exploiting the scatter-less property of such device, it is possible to nest two invisible cavities, as the outer cavity would simply not notice the presence of the inner one, regardless of their relative position. As a result, the position of the inner cavity becomes a means to easily control the field localized inside the cavity and its quality factor. In this paper, we discuss the properties of nested invisible cavities as a simple method to achieve…
While nanoscale color generations have been studied for years, the high performance transmission structural color, simultaneously equipped with large gamut, high resolution, and optical multiplexing abilities, still remains as a hanging issue. Here, a silicon metasurface embedded Fabry-Pérot cavity is demonstrated to address this problem. By changing the planar geometries of metasurface units, the cavities provide transmission colors with 194% sRGB gamut coverage and 141111 DPI resolution, along with more than 300% enhanced angular tolerance. Such high density allows two-dimensional color mixi…
Chiral Nonlinear Polaritonics with van der Waals Metasurfaces
Ludwig-Maximilians-Universität München（慕尼黑大学）；Universidade Federal de Pernambuco（伯南布哥联邦大学）；Monash University（莫纳什大学）；Imperial College London（帝国理工学院）；Shubnikov Institute of Crystallography, National Research Centre "Kurchatov Institute"（库尔恰托夫国家研究中心舒比尼科夫晶体学研究所）；National University of Science and Technology ‘MISIS’（国立科技大学 MISIS）；Australian National University（澳大利亚国立大学）
Resonant structures in modern nanophotonics are non-Hermitian (leaky and lossy), and support quasinormal modes. Moreover, contemporary cavities frequently include 2D materials to exploit and resonantly enhance their nonlinear properties or provide tunability. Such materials add further modeling complexity due to their infinitesimally thin nature and strong dispersion. Here, a formalism for efficiently analyzing third harmonic generation (THG) in nanoparticles and metasurfaces incorporating 2D materials is proposed. It is based on numerically calculating the quasinormal modes in the nanostructu…
Hybrid Cavity from Tunable Coupling between Anapole and Fabry-Perot Resonance or Anti-resonance
Modern Matter Laboratory and Advanced Materials Thrust, The Hong Kong University of Science and Technology (Guangzhou)（现代物质实验室与先进材料组，香港科技大学（广州））；Department of Electrical and Electronic Engineering, The University of Hong Kong（电气电子工程学系，香港大学）
