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arXiv 2603.25504cond-mat.mtrl-sci
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伯瑞曲率诱导的巨量异常和自旋纹理驱动的Hall响应在层状kagome反铁磁体GdTi3Bi4中

Berry curvature induced giant anomalous and spin texture driven Hall responses in the layered kagome antiferromagnet GdTi3Bi4

Indian Institute of Technology Delhi(印度德里理工学院);Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences(中国科学院金属研究所沈阳材料科学国家研究中心);Institute for Materials Research, Tohoku University(东北大学物质材料研究所学部);Center for Science and Innovation in Spintronics, Tohoku University(东北大学自旋电子学科学与创新中心)

Shobha Singh, Shivam Rathod, Rong chen, Lipika, Sneh, Rie Y. Umetsu, Yan Sun, Kaustuv Manna

AI总结:

研究通过单晶生长和磁化测量揭示GdTi3Bi4的反铁磁特性,发现其具有巨量异常霍尔电导和自旋纹理驱动的Hall响应,为探索自旋纹理物理和低维自旋电子功能提供了平台。

摘要:

近年来,层状kagome磁体作为伯瑞曲率工程和非常规输运现象的有希望平台而崭露头角。本文报道了层状范德瓦耳斯样反铁磁体GdTi3Bi4的单晶生长、磁化和电输运表征。该系统表现出明显的场诱导一级相变。全面的频率、温度和场依赖的交流磁化率测量和霍尔分析揭示了由非列线自旋纹理引起的自旋团簇状玻璃磁相。此外,该系统在2 K时表现出巨大的异常霍尔电导σ_xy^A~8.6(7)×10^3 Ohm⁻¹ cm⁻¹。详细的尺度分析揭示了斜散射和内在伯瑞曲率贡献共同作用于异常霍尔效应。第一性原理计算突出显示了费米能级附近的扁平带,Gd离子的f电子贡献了大的内在霍尔响应。因此,GdTi3Bi4成为一种罕见的层状kagome磁体,表现出伯瑞曲率诱导的巨量异常和自旋纹理驱动的霍尔响应,为探索自旋纹理物理和推进低维自旋电子功能提供了多功能平台。

英文摘要:

In recent years, layered kagome magnets have emerged as promising platforms for Berry-curvature engineering and unconventional transport phenomena. Here, we present the single-crystal growth, magnetization, and electrical transport characterizations of the van der Waals-like layered antiferromagnet GdTi3Bi4. The system exhibits pronounced field-induced first-order phase transitions. Comprehensive frequency, temperature, and field-dependent ac susceptibility measurements, and Hall analysis, reveals the formation of a spin-cluster-like glassy magnetic phase attributed to noncollinear spin textures. Additionally, the system demonstrates a colossal anomalous Hall conductivity σ_xy^{A}~ 8.6(7)10^{3} Ohm-1 cm-1 at 2 K). Detailed scaling analyses reveal the coexistence of skew scattering and intrinsic Berry-curvature contributions to the anomalous Hall effect. First-principles calculations highlight flat-band near the Fermi level, with f-electrons of the Gd ion contributing large intrinsic Hall response. Thus, GdTi3Bi4 emerges as a rare layered kagome magnet, exhibiting Berry curvature-induced giant anomalous and spin texture-driven Hall responses, providing a versatile platform for exploring spin-texture physics and advancing low-dimensional spintronic functionalities.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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