The detection of the DC diamagnetic state in pressurized Ruddlesden-Popper nickelates remained an unsolved experimental problem until recent experiments in which Zhu et al.$^1$ measured the DC diamagnetic responses in zero-field cooled (ZFC) mode in pressurized La4Ni3O10. Zhu et al.$^1$ reported that the ratio of the measured ZFC magnetic moment to the Meissner magnetic moment of the sample (and this ratio was termed the superconducting volume fraction$f$) reaches 81-86%. We regard outstanding experimental results$^1$; however, our calculations based on the reported experimental datasets$^1$ using the standard procedure showed the ratio to be 51-59%. Upon our request, Zhu et al.$^1$ provided detailed explanations and the equation they used to calculate$f$. To our knowledge, the procedure$^1$ and equation$^1$ for calculating $f$ have never been mentioned or described before, including in Ref.$^1$. Here we argue that the proposed equation$^1$ and procedure$^1$ are incorrect, and that this equation$^1$ results in multiple overestimations of the superconducting volume fraction in the sample. This overestimation error affects all superconducting volume fractions $f$ in Ruddlesden-Popper nickelates reported to date$^{1-4}$. Therefore, we describe the error we discovered in this paper.
Shear-stress-constrained superconductivity in Ruddlesden-Popper nickelates
Center for High Pressure Science & Technology Advanced Research(高压科学和技术先进研究中心);Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);Shanghai Key Laboratory of MFree, Shanghai Advanced Research in Physical Sciences(上海自由磁学重点实验室,上海物理科学先进研究)
Possible high-$T_c$ superconductivity due to incipient narrow bands originating from hidden ladders in Ruddlesden-Popper compounds
我们引入了双层Ruddlesden-Popper型化合物的隐藏梯子的概念:虽然晶体结构是双层的,但过渡金属的相关$t_{2g}$扇区中的$d_{xz}$($d_{yz}$)轨道沿着$x$($y$)形成了两条腿的梯子,因为$d_{xz}$($d_{yz}$)电子主要沿着腿方向$x$($y$)在横档$z$方向的顶部跳跃。通过第一性原理能带计算,我们预测Sr $_3$ Mo $_2$ O $_7$和Sr $_3$ Cr $_2$ O $_7$是具有合适位置$E_F$的隐梯材料的候选者.基于对这些系统的Eliashberg方程的分析,我们提出了这些材料中高温超导性的可能发生,其起因是阶梯上的宽带和“初始”窄带之间的带间对散射过程。
On estimating superconducting shielding volume fraction from susceptibility in pressurized Ruddlesden-Popper nickelates: Response to arXiv:2602.19282
Fudan University(复旦大学);Center for High Pressure Science and Technology Advanced Research(高压科学实验中心);Ocean University of China(中国海洋大学);Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);ShanghaiTech University(上海科技大学);Shandong University(山东大学)
Preparation and optimization of high-temperature superconducting Ruddlesden-Popper nickelate thin films
Southern University of Science and Technology(南方科技大学);Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area(粤港澳大湾区量子科学中心);Tsinghua University(清华大学)
Epitaxial growth of Ruddlesden-Popper neodymium nickelates Nd$_{n+1}$Ni$_{n}$O$_{3n+1}$ (${n}$ = 1-5)
采用反应分子束外延技术制备了一系列Ruddlesden-Popper镍酸盐(Nd $_{n+1}$ Ni $_{n}$ O $_{3n+1}$(${n}$ = 1-5))的稳定薄膜。X射线衍射和扫描透射电子显微镜证实了高结晶质量。X射线光电子能谱学表明这些化合物中镍的${n}$依赖价态。金属-绝缘体转变显示出明显的${n}$依赖于中间成员(${n}$ = 3-5),其低温电阻率显示对数依赖性,类似于在超导无限层镍酸盐的母体化合物中观察到的Kondo散射。
Interlayer electronic coherence links magnetism and superconductivity in Ruddlesden-Popper nickelates
State Key Laboratory of Surface Physics and Department of Physics, Fudan University(复旦大学表面物理国家重点实验室和物理系);Shanghai Research Center for Quantum Sciences(上海量子科学研究中心);Institute of Nanoelectronics and Quantum Computing, Fudan University(复旦大学纳米电子与量子计算研究所)
Expanding the trilayer Ruddlesden-Popper nickelate family: Synthesis and characterization of Sm$_4$Ni$_3$O$_{10-δ}$ single crystals
National Laboratory of Solid State Microstructures and Department of Physics, Center for Superconducting Physics and Materials, Collaborative Innovation Center of Advanced Microstructures, Nanjing University(南京大学固体微结构物理国家重点实验室、物理系、超导物理与材料中心、先进微结构协同创新中心)
Comparative Raman study of Ruddlesden-Popper nickelates and the monolayer-trilayer polymorph
Max-Planck-Institute for Solid State Research(马克斯·普朗克固体的研究所);Hefei National Laboratory(合肥国家实验室);University of Science and Technology Beijing(北京科技大学);University of Stuttgart(斯图加特大学);Institute of Theoretical Physics, Chinese Academy of Sciences(中国科学院理论物理研究所)
Contrasting Spin Excitations in Octahedral and Square-Planar n=8 Ruddlesden-Popper Nickelates
Yale University(耶鲁大学);Flatiron Institute(平顿研究所);Harvard University(哈佛大学);Donostia International Physics Center (DIPC)(多诺斯蒂亚国际物理中心);University of California San Diego(加利福尼亚大学圣迭戈分校);European Synchrotron Radiation Facility(欧洲同步辐射装置)
Itinerant Nature of Spin-Density-Wave Order in Ruddlesden-Popper Nickelates
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);School of Physical Sciences, University of Chinese Academy of Sciences(中国科学院大学物理科学学院)
Three-Dimensional Electronic Structures in Superconducting Ruddlesden-Popper Bilayer Nickelate Films
Southern University of Science and Technology(南方科技大学);Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area(粤港澳大湾区量子科学中心);University of Science and Technology of China(中国科学技术大学);Shanghai Jiao Tong University(上海交通大学);Tsinghua University(清华大学)
Electronic structures across superconductor-insulator transition in Ruddlesden-Popper bilayer nickelate films
University of Science and Technology of China(中国科学技术大学);Hefei National Laboratory, University of Science and Technology of China(合肥国家实验室,中国科学技术大学);Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China(微观尺度物理科学合肥国家研究中心,中国科学技术大学);Southern University of Science and Technology(南方科技大学);Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area(粤港澳大湾区量子科学中心);Nanjing University(南京大学);Shanghai Jiao Tong University(上海交通大学);Tsinghua University(清华大学)
Dissecting superconductivity in the Ruddlesden-Popper nickelates: The role of electron correlation and interlayer magnetic exchange
Diamond Light Source(钻石光源);National Synchrotron Radiation Laboratory and School of Nuclear Science and Technology, University of Science and Technology of China(中国科学技术大学核科学与技术学院/国家同步辐射实验室);Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-Sen University(中山大学物理学院/广东省铁电与磁器件重点实验室);Department of Physics, University of Oxford(牛津大学物理系);National Laboratory of Solid State Microstructures and Department of Physics, Nanjing University(南京大学固体微结构物理国家重点实验室/物理学院);Collaborative Innovation Center of Advanced Microstructures, Nanjing University(南京大学先进微结构协同创新中心)
Thermodynamic phase transition, pairing symmetry and Fermi surface topology in Ruddlesden-Popper nickelate films
University of Science and Technology of China(中国科学技术大学);Hefei National Laboratory, University of Science and Technology of China(合肥国家实验室,中国科学技术大学);Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China(中国科学院微观结构国家重点实验室,中国科学技术大学)
General trends of electronic structures, superconducting pairing, and magnetic correlations in the Ruddlesden-Popper nickelate $m$-layered superconductors La$_{m+1}$Ni$_{m}$O$_{3m+1}$
Electronically Inactive Intercalated La$_2$NiO$_4$ Layer in Superconducting La$_5$Ni$_3$O$_{11}$
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences(北京凝聚态物理国家实验室和中国科学院物理研究所);Kavli Institute for Theoretical Sciences, University of Chinese Academy of Sciences(中国科学院大学卡尔·萨根理论科学研究所);School of Physical Sciences, University of Chinese Academy of Sciences(中国科学院大学物理科学学院);New Cornerstone Science Laboratory, Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences(新基石科学实验室、北京凝聚态物理国家实验室和中国科学院物理研究所)
Electronic Origin of Density Wave Orders in a Trilayer Nickelate
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所凝聚态物理国家实验室);School of Physical Sciences, University of Chinese Academy of Sciences(中国科学院大学物理科学学院);Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-Sen University(中山大学物理学院广东省磁电物理与器件重点实验室);Technical Institute of Physics and Chemistry, Chinese Academy of Sciences(中国科学院化学物理研究所);Institute of Theoretical Physics, Chinese Academy of Sciences(中国科学院理论物理研究所)
Theoretical analysis on the possibility of superconductivity in a trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ under pressure and its experimental examination: comparison with La$_3$Ni$_2$O$_7$
Distinguishing Electronic Band Structure of Single-layer and Bilayer Ruddlesden-Popper Nickelates Probed by in-situ High Pressure X-ray Absorption Near-edge Spectroscopy
Electronic structure, magnetic correlations, and superconducting pairing in the reduced Ruddlesden-Popper bilayer La$_3$Ni$_2$O$_6$ under pressure: different role of $d_{3z^2-r^2}$ orbital compared with La$_3$Ni$_2$O$_7$
Spin-density-wave transition in monolayer-trilayer La3Ni2O7 single crystals
ShanghaiTech University(上海科技大学);Songshan Lake Materials Laboratory(松山湖材料实验室);Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);Beijing National Laboratory for Condensed Matter Physics(北京凝聚态物理国家研究中心);University of Chinese Academy of Sciences(中国科学院大学);Center for High Pressure Science and Technology Advanced Research(高压科学先进研究发展中心);Shanghai Key Laboratory of Material Frontiers Research in Extreme Environments (MFree)(极端环境材料前沿研究上海市重点实验室);Institute for Shanghai Advanced Research in Physical Sciences (SHARPS)(上海高等研究院物理科学研究所);ShanghaiTech Laboratory for Topological Physics(上海科技大学拓扑物理实验室);Shanghai Key Laboratory of High-resolution Electron Microscopy(高分辨电子显微学上海市重点实验室);Department of Physics, Clarendon Laboratory, University of Oxford(牛津大学克拉伦登实验室物理系);School of Physical Sciences, Great Bay University(大湾区大学物理科学学院)
Unveiling pressurized bulk superconductivity in a trilayer nickelate Pr4Ni3O10 single crystal
ShanghaiTech University(上海科技大学);Songshan Lake Materials Laboratory(松山湖材料实验室);Center for High Pressure Science and Technology Advanced Research(高压科学前沿研究中心);Institute for Shanghai Advanced Research in Physical Sciences (SHARPS)(上海物理科学研究院);Beijing University of Technology(北京工业大学);Japan Synchrotron Radiation Research Institute(日本同步辐射研究机构);University of Oxford(牛津大学);Tsinghua University(清华大学)
Nearly perfect Fermi surface nesting in hole-doped La$_3$Ni$_2$O$_7$ enables bulk superconductivity without pressure or strain
NYU-ECNU Institute of Physics, NYU Shanghai(纽约大学-华东师范大学物理研究所,上海纽约大学);Key Laboratory of Polar Materials and Devices, Ministry of Education, East China Normal University(华东师范大学极化材料与器件教育部重点实验室);Department of Physics, Brown University(布朗大学物理系);Department of Physics, New York University(纽约大学物理系)
Bulk superconductivity up to 96 K in pressurized nickelate single crystals
State Key Laboratory of Crystal Materials, Institute of Crystal Materials, Shandong University(山东大学晶体材料研究所);Center for High Pressure Science and Technology Advanced Research(高压科学和技术先进研究中心);Shanghai Key Laboratory of Material Frontiers Research in Extreme Environments (MFree), Shanghai Advanced Research in Physical Sciences (SHARPS)(极端环境材料前沿研究上海市重点实验室(MFree),上海物理科学先进研究中心(SHARPS));Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所,凝聚态物理国家实验室);School of Physical Sciences, University of Chinese Academy of Sciences(中国科学院大学物理科学学院);CAS Key Laboratory of Standardization and Measurement for Nanotechnology, National Center for Nanoscience and Technology(中国科学院纳米技术标准化与计量重点实验室,国家纳米科学中心);Key Laboratory of Materials Physics, Ministry of Education, School of Physics, Zhengzhou University(郑州大学物理学院,教育部材料物理重点实验室);Institute of Quantum Materials and Physics, Henan Academy of Sciences(河南省科学院量子材料与物理研究所);NSF’s ChemMatCARS, The University of Chicago(芝加哥大学,美国国家科学基金会化学-材料束线组合站(ChemMatCARS));School of Materials and Energy, University of Electronic Science and Technology of China(电子科技大学材料与能源学院);Huzhou Key Laboratory of Smart and Clean Energy, Yangtze Delta Region Institute (Huzhou), University of Electronic Science and Technology of China(电子科技大学长三角研究院(湖州),湖州市智能清洁能源重点实验室);Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences(中国科学院上海高等研究院,上海同步辐射光源);Japan Synchrotron Radiation Research Institute(日本同步辐射研究机构);NanoTerasu Promotion Division, Japan Synchrotron Radiation Research Institute (JASRI)(日本同步辐射研究机构(JASRI)纳米terasu推进部)