Intermodal quantum key distribution over an 18 km free-space channel with adaptive optics and room-temperature detectors
Università degli Studi di Padova（帕多瓦大学）；ThinkQuantum s.r.l.（思量子有限公司）；Institute of Photonics and Nanotechnology, National Council of Research of Italy（意大利国家研究委员会光子与纳米技术研究所）
Edoardo Rossi, Ilektra Karakosta-Amarantidou, Matteo Padovan, Marco Nardi, Marco Avesani, Francesco Bruno Leonardo Santagiustina, Marco Taffarello, Antonio Vanz… 展开作者
Edoardo Rossi, Ilektra Karakosta-Amarantidou, Matteo Padovan, Marco Nardi, Marco Avesani, Francesco Bruno Leonardo Santagiustina, Marco Taffarello, Antonio Vanzo, Stefano Bonora, Giuseppe Vallone, Paolo Villoresi, Francesco Vedovato
Intermodal quantum key distribution at telecom wavelengths provides a hybrid interface between fiber connections and free-space links, both essential for the realization of scalable and interoperable quantum networks. Although demonstrated over short-range free-space links, long-distance implementations of intermodal quantum key distribution remain challenging, due to turbulence-induced wavefront aberrations which limit efficient single-mode fiber coupling at the optical receiver. Here, we demonstrate a real-time intermodal quantum key distribution field trial over an 18 km free-space link, connecting a remote terminal to an urban optical ground station equipped with a 40 cm-class telescope. An adaptive optics system, implementing direct wavefront sensing and high-order aberration correction, enables efficient single-mode fiber coupling and allows secure key generation of 200 bit/s using a compact state analyzer equipped with room-temperature detectors. We further validate through experimental data a turbulence-based model for predicting fiber coupling efficiency, providing practical design guidelines for future intermodal quantum networks.
Candidate overtone shear horizontal SAW resonators in thin-film lithium niobate for intermodal acousto-optic modulation
Wangzhijiang Innovation Center for Laser, Aerospace Laser Technology and System Department, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences（中国科学院上海光学精密机械研究所）；Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences（中国科学院大学物质科学与光电技术研究院）；School of Information Science and Technology, ShanghaiTech University（上海科技大学信息科学与技术学院）
Intermodal entanglement in a quantum optical model of HHG due to the back-action on the driving field
HUN-REN Wigner Research Centre for Physics（匈牙利研究与创新网络温格物理研究中心）；Institute of Physics, University of Pécs（佩奇大学物理研究所）；Laboratoire d’Optique Appliquée (LOA), CNRS, École polytechnique, ENSTA, Institut Polytechnique de Paris（巴黎理工学院应用光学实验室（CNRS、巴黎综合理工学院、ENSTA））
We present a theoretical and experimental study of the generation of photon pairs through the process of spontaneous four wave mixing (SFWM) in a few-mode, birefringent fiber. Under these conditions, multiple SFWM processes are in fact possible, each associated with a different combination of transverse modes for the four waves involved. We show that in the weakly guiding regime, for which the propagation modes may be well approximated by linearly polarized modes, the departure from circular symmetry due to the fiber birefringence translates into conservation rules which retain elements from a…
We report a versatile method to efficiently polarize single nuclear spins in diamond, which is based on optical pumping of a single NV color center and mediated by a level-anti crossing in its excited state. A nuclear spin polarization higher than 98% is achieved at room temperature for the 15N nuclear spin associated to the NV center, corresponding to $μ$K effective nuclear spin temperature. We then show simultaneous deterministic initialization of two nuclear spins (13C and 15N) in close vicinity to a NV defect. Such robust control of nuclear spin states is a key ingredient for further scali…
There has been much recent interest in extending the technique of magnetic resonance imaging (MRI) down to the level of single spins with sub-optical wavelength resolution. However, the signal to noise ratio for images of individual spins is usually low and this necessitates long acquisition times and low temperatures to achieve high resolution. An exception to this is the nitrogen-vacancy (NV) color center in diamond whose spin state can be detected optically at room temperature. Here we apply MRI to magnetically equivalent NV spins in order to resolve them with resolution well below the opti…
We demonstrate the Ramsey analogous experiment known as coherent control, taking place along an electrically-driven semiconductor optical amplifier operating at room temperature.
We theoretically investigate an ensemble of three-level room-temperature atoms in a two-mode optical cavity, focusing on the case of counterpropagating light fields. We find that in the limit of large detunings the problem admits relatively simple and intuitive solutions. When a classical field drives one of the transitions, the system becomes equivalent to an ensemble of two-level atoms with suppressed Doppler broadening. In contrast, when the same transition is driven with a single photon, the system collectively behaves like a single two-level atom. This latter result is particularly releva…
Recent progress in nonlinear optical materials and microresonators has brought quantum computing with bulk optical nonlinearities into the realm of possibility. This platform is of great interest, not only because photonics is an obvious choice for quantum networks, but also because it may be the only feasible route to quantum information processing at room temperature. We introduce a paradigm for room-temperature photonic quantum logic that significantly simplifies the realization of various quantum circuits, and in particular, of error correction. It uses only the strongest available bulk no…
Lasers have revolutionized optical science and technology, but their microwave counterpart, maser, has not realized its great potential due to its demanding work conditions (high-vacuum for gas maser and liquid-helium temperature for solid-state maser). Room-temperature solid-state maser is highly desirable, but under such conditions the lifetimes of emitters (usually electron spins) are usually too short (~ns) for population inversion. The only room-temperature solid-state maser is based on a pentacene-doped p-terphenyl crystal, which has long spin lifetime (~0.1 ms). This maser, however, ope…
Rabi nutations of a single electron spin in a single defect center have been detected. The coherent evolution of the spin quantum state is followed via optical detection of the spin state. Coherence times up to several microseconds at room temperature have been measured. Optical readout of the spin states leads to decoherence, equivalent to the so-called Zeno effect. Quantum beats between electron spin transitions in a single spin Hahn echo experiment are observed. A closer analysis reveals that beats also result from the hyperfine coupling of the electron spin to a single 14N nuclear spin. Th…
Optically addressable spins associated with defects in wide-bandgap semiconductors are versatile platforms for quantum information processing and nanoscale sensing, where spin-dependent inter-system crossing (ISC) transitions facilitate optical spin initialization and readout. Recently, the van der Waals material hexagonal boron nitride (h-BN) has emerged as a robust host for quantum emitters (QEs), but spin-related effects have yet to be observed. Here, we report room-temperature observations of strongly anisotropic photoluminescence (PL) patterns as a function of applied magnetic field for s…
Optical self-cooling of a membrane oscillator in a cavity optomechanical experiment at room temperature
Università di Firenze（佛罗伦萨大学）；Institute of Materials for Electronics and Magnetism, Nanoscience-Trento-FBK Division（电子与磁性材料研究所，纳米科学-特伦托-FBK分部）；Istituto Nazionale di Fisica Nucleare (INFN), Trento Institute for Fundamental Physics and Application（意大利国家核物理研究所（INFN），特伦托基础物理与应用研究所）；CNR-INO（意大利国家研究委员会-光学研究所）；INFN, Sezione di Firenze（意大利国家核物理研究所，佛罗伦萨分部）；Delft University of Technology（代尔夫特理工大学）
Just as classical information systems require buffers and memory, the same is true for quantum information systems. The potential that optical quantum information processing holds for revolutionising computation and communication is therefore driving significant research into developing optical quantum memory. A practical optical quantum memory must be able to store and recall quantum states on demand with high efficiency and low noise. Ideally, the platform for the memory would also be simple and inexpensive. Here, we present a complete tomographic reconstruction of quantum states that have b…
Bulk 13C polarization can be strongly enhanced in diamond at room-temperature based on the optical pumping of nitrogen-vacancy color centers. This effect was confirmed by irradiating suitably aligned single-crystals at a ~50 mT field promoting anti-crossings between electronic excited-state levels, followed by shuttling of the sample into a custom-built NMR setup and by subsequent 13C detection. A nuclear polarization of ~0.5% - equivalent to the 13C polarization achievable by thermal polarization at room temperature at fields of ~2000 T - was measured, and its bulk nature determined based on …
Entanglement between optical mode and microwave mode is a critical issue in illumination systems. Traditionally, optomechanical systems are applied to couple the optical mode to microcavity modes. However, due to some restrictions of this system such as sensitivity to the thermal noise at room temperature, a novel optoelectronic system is designed in this study to fix the recent system problems. Unlike recent optomechanical systems, the optical modes are directly coupled to the microwave cavity through the optoelectronic elements with no need mechanical system. The main objective of this work …
Manipulation of solid-state spin coherence is an important paradigm for quantum information processing. Current systems either operate at very low temperatures or are difficult to scale-up. Developing low-cost, scalable materials whose spins can be coherently manipulated at room temperature is thus highly-attractive for a sustainable future of quantum information science. Here we report ambient-condition all-optical initialization, manipulation and readout of single-hole spins in an ensemble of solution-grown CsPbBr3 perovskite QDs. Single-hole spins are obtained by sub-picosecond electron sca…
Future quantum photonic networks require coherent optical memories for synchronizing quantum sources and gates of probabilistic nature. We demonstrate a fast ladder memory (FLAME) mapping the optical field onto the superposition between electronic orbitals of rubidium vapor. Employing a ladder level-system of orbital transitions with nearly degenerate frequencies simultaneously enables high bandwidth, low noise, and long memory lifetime. We store and retrieve 1.7-ns-long pulses, containing 0.5 photons on average, and observe short-time external efficiency of 25%, memory lifetime (${1/e}$) of 8…
The nuclear spin singlet order involving coupled pairs of spins-1/2 may be used to store nuclear spin hyperpolarization in a room temperature liquid for a time much longer than the spin-lattice relaxation time $T_1$. There both are observations of long-lived homonuclear and heteronuclear spin-singlet order. Although hyperpolarized singlet order of the same species are accessible, hyperpolarized heteronuclear spin-singlet order has not been presented yet. Here we show hyperpolarized singlet order is achievable in the sample of $^{13}$C-labeled formic acid solution at room temperature by using o…
Quantum measurements of mechanical systems can produce optical squeezing via ponderomotive forces. Its observation requires high environmental isolation and efficient detection, typically achieved by using optical cavities and cryogenic cooling. Here we realize these conditions by measuring the position of an optically levitated nanoparticle at room temperature and without the overhead of an optical cavity. We use a fast heterodyne detection to reconstruct simultaneously orthogonal optical quadratures, and observe a noise reduction of $9\%\pm0.5\%$ below shot noise. Our experiment offers a nov…
A paradigm for universal quantum information processing with integrated acousto-optic frequency beamsplitters
Purdue University（普渡大学）；Oak Ridge National Laboratory（橡树岭国家实验室）；Northern Arizona University（北亚利桑那大学）；Sandia National Laboratories（桑迪亚国家实验室）；Qunnect Inc.（Qunnect公司）
We have shown that a coherently driven solid state medium can potentially produce strong controllable short pulses of THz radiation. The high efficiency of the technique is based on excitation of maximal THz coherence by applying resonant optical pulses to the medium. The excited coherence in the medium is connected to macroscopic polarization coupled to THz radiation. We have performed detailed simulations by solving the coupled density matrix and Maxwell equations. By using a simple $V$-type energy scheme for ruby, we have demonstrated that the energy of generated THz pulses ranges from hund…
We report a photon shot-noise-limited (SNL) optical magnetometer based on amplitude modulated optical rotation using a room-temperature $^{85}$Rb vapor in a cell with anti-relaxation coating. The instrument achieves a room-temperature sensitivity of $70$ fT/$\sqrt{\mathrm{Hz}}$ at $7.6$ $μ$T. Experimental scaling of noise with optical power, in agreement with theoretical predictions, confirms the SNL behaviour from $5$ $μ$T to $75$ $μ$T. The combination of best-in-class sensitivity and SNL operation makes the system a promising candidate for application of squeezed light to a state-of-the-art …
We report bulk, room-temperature hyperpolarization of 13C nuclear spins observed via high-field nuclear magnetic resonance (NMR). The hyperpolarization is achieved by optical pumping (OP) of nitrogen vacancy defect centers in diamond accompanied by dynamic nuclear polarization (DNP). The technique harnesses the large optically-induced spin polarization of NV- centers at room temperature, which is many orders of magnitude greater than thermal equilibrium polarization and typically achievable only at sub-Kelvin temperatures. Transfer of the spin polarization to the 13C nuclear spins is accomplis…
Silicon vacancies in silicon carbide have been proposed as an alternative to nitrogen vacancy centers in diamonds for spintronics and quantum technologies. An important precondition for these applications is the initialization of the qubits into a specific quantum state. In this work, we study the optical alignment of the spin 3/2 negatively charged silicon vacancy in 6H-SiC. Using a time-resolved optically detected magnetic resonance technique, we coherently control the silicon vacancy spin ensemble and measure Rabi frequencies and spin-lattice relaxation time of all three transitions. Then t…
The ability to induce, observe and control quantum coherent interactions in room temperature, electrically driven optoelectronic devices is of outmost significance for advancing quantum science and engineering towards practical applications. We demonstrate here a quantum interference phenomena, Ramsey fringes, in an inhomogeneously broadened InAs/InP quantum dot (QD) ensemble in the form of a 1.5 mm long optical amplifier operating at room temperature. Observation of Ramsey fringes in semiconductor QD was previously achieved only at cryogenic temperatures and only in isolated single dot system…
Diamond is a proven solid-state platform for spin-based quantum technology. The nitrogen-vacancy (NV) center in diamond has been used to realize small-scale quantum information processing (QIP) and quantum sensing under ambient conditions. A major barrier in the development of large-scale QIP in diamond is the connection of NV spin registers by a quantum bus at room temperature. Given that diamond is expected to be an ideal spin transport material, the coherent transport of spin directly between the spin registers offers a potential solution. Yet, there has been no demonstration of spin transp…
By shining laser light through a nanomechanical beam, we measure the beam's thermally driven vibrations and perturb its motion with optical forces at a level dictated by the Heisenberg measurement-disturbance uncertainty relation. Such quantum backaction is typically difficult to observe at room temperature where the motion driven by optical quantum intensity fluctuations is many orders of magnitude smaller than the thermal motion. We demonstrate a cross-correlation technique to distinguish optically driven motion from thermally driven motion, observing this quantum backaction signature up to …
We demonstrate dispersive readout of the spin of an ensemble of Nitrogen-Vacancy centers in a high-quality dielectric microwave resonator at room temperature. The spin state is inferred from the reflection phase of a microwave signal probing the resonator. Time-dependent tracking of the spin state is demonstrated, and is employed to measure the T1 relaxation time of the spin ensemble. Dispersive readout provides a microwave interface to solid state spins, translating a spin signal into a microwave phase shift. We estimate that its sensitivity can outperform optical readout schemes, owing to th…
Optically addressable spins in materials are important platforms for quantum technologies, such as repeaters and sensors. Identification of such systems in two-dimensional (2d) layered materials offers advantages over their bulk counterparts, as their reduced dimensionality enables more feasible on-chip integration into devices. Here, we report optically detected magnetic resonance (ODMR) from previously identified carbon-related defects in 2d hexagonal boron nitride (hBN). We show that single-defect ODMR contrast can be as strong as 6% and displays a magnetic-field dependence with both positi…
Optically pumped magnetometers are becoming a promising alternative to cryogenically-cooled superconducting magnetometers for detecting and imaging biomagnetic fields. Magnetic field detection is a completely non-invasive method, which allows one to study the function of excitable human organs with a sensor placed outside the human body. For instance, magnetometers can be used to detect brain activity or to study the activity of the heart. We have developed a highly sensitive miniature optically pumped magnetometer based on cesium atomic vapor kept in a paraffin-coated glass container. The mag…
In quantum optics, orbital angular momentum (OAM) is very promising to achieve high-dimensional quantum states due to the nature of infinite and discrete eigenvalue, which is quantized by the topological charge of l. Here, a heralded single-photon source with switchable OAM modes is proposed and demonstrated on silicon chip. At room-temperature, the heralded single photons with 11 OAM modes (l=2~6, -6~-1) have been successfully generated and switched through thermo-optical effect. We believe that such an integrated quantum source with multiple OAM modes and operating at room-temperature would …
Dynamic Nuclear Polarization (DNP) is a powerful suite of techniques that deliver multifold signal enhancements in NMR and MRI. The generated athermal spin states can also be exploited for quantum sensing and as probes for many-body physics. Typical DNP methods require use of cryogens, large magnetic fields, and high power microwaves, which are expensive and unwieldy. Nanodiamond particles, rich in Nitrogen-Vacancy (NV) centers, have attracted attention as alternative DNP agents because they can potentially be optically hyperpolarized at room temperature. Indeed the realization of a miniature …
We investigate the optical properties of Dibenzoterrylene (DBT) molecules in a spin-coated crystalline film of anthracence. By performing single molecule studies, we show that the dipole moments of the DBT molecules are oriented parallel to the plane of the film. Despite a film thickness of only 20 nm, we observe an exceptional photostability at room temperature and photon count rates around one million per second from a single molecule. These properties together with an emission wavelength around 800 nm make this system attractive for applications in nanophotonics and quantum optics.
A coherent superposition of rotational states in D$_2$ has been excited by nonresonant ultrafast (12 femtosecond) intense (2 $\times$ 10$^{14}$ Wcm$^{-2}$) 800 nm laser pulses leading to impulsive dynamic alignment. Field-free evolution of this rotational wavepacket has been mapped to high temporal resolution by a time-delayed pulse, initiating rapid double ionization, which is highly sensitive to the angle of orientation of the molecular axis with respect to the polarization direction, $θ$. The detailed fractional revivals of the neutral D$_2$ wavepacket as a function of $θ$ and evolution tim…
We demonstrate coherent storage and retrieval of pulsed light using the atomic frequency comb quantum memory protocol in a room temperature alkali vapour. We utilise velocity-selective optical pumping to prepare multiple velocity classes in the $F=4$ hyperfine ground state of caesium. The frequency spacing of the classes is chosen to coincide with the $F'=4 - F'=5$ hyperfine splitting of the $6^2$P$_{3/2}$ excited state resulting in a broadband periodic absorbing structure consisting of two usually Doppler-broadened optical transitions. Weak coherent states of duration $2\,\mathrm{ns}$ are map…
Realization of practical terahertz wireless communications still faces many challenges. The receiver with high sensitivity is important for THz wireless communications. Here we demonstrate a terahertz receiver based on the cesium Rydberg atoms in a room-temperature vapor cell. The minimum detectable THz electric field is calibrated. With this receiver, the phase-sensitive conversion of amplitude-modulated or frequency-modulated terahertz waves into optical signals is performed. The results show that the atomic receiver has many advantages due to its quantum properties. Especially, the long dis…
We demonstrate room temperature detection of single 20 nm super-paramagnetic nanoparticles (SPNs) with a wide-field optical microscope platform suitable for biological integration. The particles are made of magnetite (Fe3O4) and are thus non-toxic and biocompatible. Detection is accomplished via optically detected magnetic resonance imaging using nitrogen-vacancy defect centers in diamond, resulting in a DC magnetic field detection limit of 2.3 μT. This marks a large step forward in the detection of SPNs, and we expect that it will allow for the development of magnetic-field-based biosensors c…
Dynamic nuclear polarization via contact with electronic spins has emerged as an attractive route to enhance the sensitivity of nuclear magnetic resonance (NMR) beyond the traditional limits imposed by magnetic field strength and temperature. Among the various alternative implementations, the use of nitrogen vacancy (NV) centers in diamond - a paramagnetic point defect whose spin can be optically polarized at room temperature - has attracted widespread attention, but applications have been hampered by the need to align the NV axis with the external magnetic field. Here we overcome this hurdle …
Optically addressable spins in widebandgap semiconductors have become one of the most prominent platforms for exploring fundamental quantum phenomena. While several candidates in 3D crystals including diamond and silicon carbide have been extensively studied, the identification of spindependent processes in atomically thin 2D materials has remained elusive. Although optically accessible spin states in hBN are theoretically predicted, they have not yet been observed experimentally. Here, employing rigorous electron paramagnetic resonance techniques and photoluminescence spectroscopy, we identif…
The strong-coupling regime between an electronic transition and the photonic mode of a optical resonator manifests itself in the lifting of the degeneracy between the two modes and the creation of two polariton states with mixed optical and electronic character. This phenomenon has been studied in atoms, excitons in semiconductors and quantum electrodynamics circuits based on Josephson junctions. Recently, there is also strong interest to study similar effects using intersubband transitions in quantum wells in the terahertz, where the ultra strong coupling regime can be reached and new physica…
