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arXiv 2602.09460cond-mat.mtrl-sci
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节点面与平板驱动的在Fe5Si3 epitaxial铁磁韦尔金属中的大异常纳维效应

Nodal-Surface and Flat-Band Driven Large Anomalous Nernst Effect in Epitaxial Ferromagnetic Weyl Metal Fe5Si3

Indian Institute of Technology Delhi(印度德里理工学院);Indian Institute of Technology Hyderabad(印度海得拉巴理工学院);National Institute for Materials Science(日本国立材料研究所)

Shubhashish Pati, Sonali Srotaswini Pradhan, Nanhe Kumar Gupta, Abhay Pandey, Nikita Sharma, Nakul Kumar, Saurav Singh, Yuya Sakuraba, V. Kanchana, Sujeet Chaudhary

AI总结:

Fe5Si3铁磁韦尔金属通过节点面和平板结构产生大异常纳维效应,揭示拓扑电子结构在热电转换中的主导作用。

摘要:

磁性拓扑材料如韦尔和狄拉克磁体表现出非传统电子性质,源于磁序与能带拓扑之间的相互作用,导致显著的热磁和热电效应。在这里,我们研究了韦尔铁磁体候选材料Fe5Si3的 epitaxial 薄膜中的ANP。在室温下观察到显著的横向纳维响应,超过约1.50微伏每开尔文,同时伴随着大约0.56的巨异常纳维角,表明热梯度与横向电场之间高效转换。除了异常贡献外,超过室温的显著拓扑纳维信号约为0.43微伏每开尔文,表明可能存在的与非平凡自旋纹理相关的实空间 Berry 曲率。第一性原理密度泛函理论计算结合对称性分析揭示了非传统的电子结构,其中韦尔节点线、节点面和近似平板在费米能级附近共存。这种罕见的多重拓扑能带特征产生了强烈增强且能量依赖性强的 Berry 曲率,这决定了所观察到的纳维响应的大小和温度演变。计算的异常纳维导电率与实验结果的定量一致,确立了拓扑电子结构作为所观察到的热磁输运的主要起源,突显Fe5Si3作为一种化学简单、成本低的二元拓扑磁体,用于探索实空间和动量空间 Berry 曲率驱动的热电现象。

英文摘要:

Magnetic topological materials such as Weyl and Dirac magnets exhibit unconventional electronic properties arising from the interplay between magnetic order and band topology, leading to remarkable thermomagnetic and thermoelectric effects. Here, we investigate the ANE in epitaxial thin films of the Weyl ferromagnet candidate Fe5Si3. A pronounced transverse Nernst response exceeding approximately 1.50 microvolt per kelvin is observed at room temperature, together with a giant anomalous Nernst angle of about 0.56, indicating highly efficient conversion between thermal gradients and transverse electric fields. Beyond the anomalous contribution, a sizable topological Nernst signal of approximately 0.43 microvolt per kelvin persists above room temperature, suggesting the possible presence of real-space Berry curvature associated with nontrivial spin textures. First-principles density functional theory calculations combined with symmetry analysis reveal an unconventional electronic structure in which Weyl nodal lines, nodal surfaces, and nearly flat bands coexist near the Fermi level. This rare concurrence of multiple topological band features produces a strongly enhanced and sharply energy-dependent Berry curvature, which governs both the magnitude and temperature evolution of the observed Nernst response. The close quantitative agreement between calculated anomalous Nernst conductivity and experimental results establishes the topological electronic structure as the dominant origin of the observed thermomagnetic transport, highlighting Fe5Si3 as a chemically simple, low-cost binary topological magnet for exploring both real-space and momentum-space Berry-curvature-driven thermoelectric phenomena.

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