Dysprosium (Dy) is the most magnetic element on the periodic table, making it excellent for studying dipolar atom-atom interactions. We report on a simple Dy MOT that captures atoms directly from the thermal beam using a single diode-laser system to generate the light. Additionally, the atoms are magnetically confined by the quadrupole magnetic field that also facilitates the MOT. The MOT loading time is $τ_\text{b} = 26~\text{ms}$. Atoms can decay to a dark state that is magnetically trapped. The time constant for loading into this magnetic trap is $τ_\text{d} = 410~\text{ms}$. The total magnetically trapped population is $1.14\times10^{5}$ atoms, with $85\%$ residing in the dark states. The magnetically trapped atoms have a temperature of $28~μ\text{K}$, significantly below the Doppler limit. This population fulfills the requirements for a range of future experiments.
We present our technique to create a magneto-optical trap for dysprosium atoms using the narrow-line cooling transition at 626$\,$nm to achieve suitable conditions for direct loading into an optical dipole trap. The magneto-optical trap is loaded from an atomic beam via a Zeeman slower using the strongest atomic transition at 421$\,$nm. With this combination of two cooling transitions we can trap up to $2.0\cdot10^8$ atoms at temperatures down to 6$\, μ$K. This cooling approach is simpler than present work with ultracold dysprosium and provides similar starting conditions for a transfer to an …
The efficiency of optical trapping of ultracold atoms depend on the atomic dynamic dipole polarizability governing the atom-field interaction. In this article, we have calculated the real and imaginary parts of the dynamic dipole polarizability of dysprosium in the ground and first excited level. Due to the high electronic angular momentum of those two states, the polarizabilities possess scalar, vector and tensor contributions that we have computed, on a wide range of trapping wavelengths, using the sum-over-state formula. Using the same formalism, we have also calculated the $C_6$ coefficien…
Magneto-optical traps (MOTs) of highly magnetic lanthanides open the door to explorations of novel phases of strongly correlated matter such as lattice supersolids and quantum liquid crystals. We recently reported the first MOTs of the five high abundance isotopes of the most magnetic atom, dysprosium. Described here are details of the experimental technique employed for repumper-free Dy MOTs containing up to half a billion atoms. Extensive characterization of the MOTs' properties---population, temperature, loading, metastable decay dynamics, trap dynamics---is provided.
A thermal atomic beam of dysprosium (Dy) atoms is cooled using the $4f^{10}6s^2 (J=8) \to 4f^{10}6s6p (J=9)$ transition at 421 nm. The cooling is done via a standing light wave orthogonal to the atomic beam. Efficient transverse cooling to the Doppler limit is demonstrated for all observable isotopes of dysprosium. Branching ratios to metastable states are demonstrated to be $<5\times10^{-4}$. A scheme for enhancement of the nonzero-nuclear-spin-isotope cooling, as well as a method for direct identification of possible trap states, is proposed.
Ultracold dysprosium gases, with a magnetic moment ten times that of alkali atoms and equal only to terbium as the most magnetic atom, are expected to exhibit a multitude of fascinating collisional dynamics and quantum dipolar phases, including quantum liquid crystal physics. We report the first laser cooling and trapping of half a billion Dy atoms using a repumper-free magneto-optical trap (MOT) and continuously loaded magnetic confinement, and we characterize the trap recycling dynamics for bosonic and fermionic isotopes. The first inelastic collision measurements in the few partial wave, 10…
We report on an apparatus for cooling and trapping of neutral dysprosium. We characterize and optimize the performance of our Zeeman slower and 2D molasses cooling of the atomic beam by means of Doppler spectroscopy on a 136 kHz broad transition at 626 nm. Furthermore, we demonstrate the characterization and optimization procedure for the loading phase of a magneto-optical trap (MOT) by increasing the effective laser linewidth by sideband modulation. After optimization of the MOT compression phase, we cool and trap up to $10^9$ atoms within 3 seconds in the MOT at temperatures of 9 μK and phas…
In the domain of quantum degenerate atomic gases, much interest has been raised recently by the use of Lanthanide atoms with large magnetic moments, in particular Dysprosium and Erbium. These species have been successfully brought to quantum degeneracy and are now excellent candidates for quantum simulations of physical phenom- ena due to long-range interactions. In this short article, we report on the progresses in the construction of a new experiment on Bose-Einstein condensation of Dysprosium atoms. After completing the vacuum and the laser setups, a magneto-optical trap on the narrow 626nm…
A two-dimensional magneto-optical trap of dysprosium atoms as a compact source for efficient loading of a narrow-line three-dimensional magneto-optical trap
We report the Bose-Einstein condensation (BEC) of the most magnetic atom, dysprosium. The Dy BEC is the first for an open f-shell lanthanide (rare-earth) element and is produced via forced evaporation in a crossed optical dipole trap loaded by an unusual, blue-detuned and spin-polarized narrow-line magneto-optical trap. Nearly pure condensates of 1.5x10^4 164Dy atoms form below T = 30 nK. We observe that stable BEC formation depends on the relative angle of a small polarizing magnetic field to the axis of the oblate trap, a property of trapped condensates only expected in the strongly dipolar …
Magneto-optical traps (MOTs) of Er and Dy have recently been shown to exhibit population-wide sub-Doppler cooling due to their near degeneracy of excited and ground state Lande g factors. We discuss here an additional, unusual intra-MOT sub-Doppler cooling mechanism that appears when the total Dy MOT cooling laser intensity and magnetic quadrupole gradient increase beyond critical values. Specifically, anisotropically sub-Doppler-cooled cores appear, and their orientation with respect to the quadrupole axis flips at a critical ratio of the MOT laser intensity along the quadrupole axis versus t…
We report a measurement of the dynamical polarizability of dysprosium atoms in their electronic ground state at the optical wavelength of 1064 nm, which is of particular interest for laser trapping experiments. Our method is based on collective oscillations in an optical dipole trap, and reaches unprecedented accuracy and precision by comparison with an alkali atom (potassium) as a reference species. We obtain values of 184.4(2.4) a.u. and 1.7(6) a.u. for the scalar and tensor polarizability, respectively. Our experiments have reached a level that permits meaningful tests of current theo- reti…
We produce Bose-Einstein condensates of $^{162}$Dy atoms employing an innovative technique based on a resonator-enhanced optical trap that allows efficient loading from the magneto-optical trap and fast evaporation. We characterize the scattering properties of the ultracold atoms for magnetic fields between 6 and 30 G. In addition to the typical chaotic distribution of narrow Feshbach resonances in Lanthanides, we discover two rather isolated broad features at around 22 G and 27 G. A characterization using the complementary measurements of losses, thermalization, anisotropic expansion and mole…
We present a numerical study of the behaviour of two magnetic dipolar atoms trapped in a harmonic potential and exhibiting the standard Einstein-de Haas effect while subject to a time dependent homogeneous magnetic field. Using a simplified description of the short range interaction and the full expression for the dipole-dipole forces we show, that under experimentally realisable conditions two dysprosium atoms may be pumped to a high ($l>20$) value of the relative orbital angular momentum.
We characterize the anisotropic differential ac-Stark shift for the Dy $626$ nm intercombination transition, induced in a far-detuned $1070$ nm optical dipole trap, and observe the existence of a "magic polarization" for which the polarizabilities of the ground and excited states are equal. From our measurements we extract both the scalar and tensorial components of the dynamic dipole polarizability for the excited state, $α_E^\text{s} = 188 (12)\,α_\text{0}$ and $α_E^\text{t} = 34 (12)\,α_\text{0}$, respectively, where $α_\text{0}$ is the atomic unit for the electric polarizability. We also p…
We report the observation of resonance-like loss in the trap population of ultracold dysprosium as a function of magnetic field, which we attribute to anisotropy-induced Fano-Feshbach resonances arising from Dy's large magnetic dipole moment and nonzero electronic orbital angular momentum. We recorded these resonances for four different isotopes, three bosonic and one fermionic, over a field range of 0-6 G and show that the number of resonances changes significantly as a function of temperature, even in the nK regime. Most of the observed resonances are of very narrow width. The fermionic isot…
We report on the first realization of a two-species magneto-optical trap (MOT) for erbium and dysprosium. The MOT operates on an intercombination line for the respective species. Owing to the narrow-line character of such a cooling transition and the action of gravity, we demonstrate a novel trap geometry employing only five beams in orthogonal configuration. We observe that the mixture is cooled and trapped very efficiently, with up to \num{5e8} Er atoms and \num{e9} Dy atoms at temperatures of about $10\,μK$. Our results offer an ideal starting condition for the creation of a dipolar quantum…
We demonstrate the use of spatial emission patterns to measure the magnetic fields used in a magneto-optical trap. The directional aspect of the Hanle effect gives a direct, visual presentation of the magnetic fields, in which brighter fluorescence indicates larger fields. It can be used to determine the direction as well as the magnitude of the field. It is particularly well suited for characterizing and aligning magneto-optical traps, requiring little additional equipment or setup beyond what is ordinarily used in a magneto-optical trap, and being most sensitive to fields of the size typical…
The loading dynamics of an alkali-atom magneto-optical trap can be used as a reliable measure of vacuum pressure, with loading time T indicating a pressure less than or equal to [2x10^(-8) Torr s]/T. This relation is accurate to approximately a factor of two over wide variations in trap parameters, background gas composition, or trapped alkali species. The low-pressure limit of the method does depend on the trap parameters, but typically extends to the 10^(-10) Torr range.
Electromagnetically induced absorption (EIA) was observed on a sample of $% ^{85}Rb$ in a magneto-optical trap using low intensity cw copropagating pump and probe optical fields. At moderate trapping field intensity, the EIA spectrum is determined by the Zeeman effect produced on the atomic ground-state by the trapping quadrupolar magnetic field. The use of EIA spectroscopy for the magnetic field mapping of cold atomic samples is illustrated.
We explore the phase diagram of a finite-sized dysprosium dipolar Bose-Einstein condensate in a cylindrical harmonic trap. We monitor the final state after the scattering length is lowered from the repulsive BEC regime to the quantum droplet regime. Either an adiabatic transformation between a BEC and a quantum droplet is obtained or, above a critical trap aspect ratio $λ_{\rm c}=1.87(14)$, a modulational instability results in the formation of multiple droplets. This is in full agreement with the predicted structure of the phase diagram with a crossover region below $λ_{\rm c}$ and a multista…
Measurements of rubidium lifetime in a dark magneto-optical trap (DMOT) was performed at various populations of the bright and dark hyperfine states of the trapped atoms. The rubidium lifetime in the trap appeared to be shorter if the atom spent more time in the bright state. A simple explanation of this effect is based on the increase of the cross-section of rubidium collisions with the surrounding warm atoms upon rubidium electronic excitation.
We present experimental results from a new scheme for magneto-optically trapping strontium monofluoride (SrF) molecules, which provides increased confinement compared to our original work. The improved trap employs a new approach to magneto-optical trapping presented by M. Tarbutt, \emph{arXiv preprint} 1409.0244, which provided insight for the first time into the source of the restoring force in magneto-optical traps (MOTs) where the cycling transition includes dark Zeeman sublevels (known as type-II MOTs). We measure a radial spring constant $20\times$ greater than in our original work with …
Large clouds of cold atoms prepared in a magneto-optical trap can develop spatio-temporal instabilities when the frequency of the trapping lasers is brought close to the atomic resonance. This system bears close similarities with trapped plasmas, whereby effective Coulomb interactions are induced by the exchange of scattered photons and lead to collective nonlinear dynamics of the trapped atoms. We report in this paper a detailed experimental study of the instability threshold, and comparisons with three-dimensional simulations of the interacting, laser-driven cloud.
We investigate the scaling behavior of a very large magneto-optical trap (VLMOT) containing up to $1.4 \times 10^{11}$ Rb$^{87}$ atoms. By varying the diameter of the trapping beams, we are able to change the number of trapped atoms by more than 5 orders of magnitude. We then study the scaling laws of the loading and size of the VLMOT, and analyze the shape of the density profile in this regime where the Coulomb-like, light-mediated repulsive interaction between atoms is expected to play an important role.
The influence of gravity on antihydrogen dynamics in magnetic traps is studied. The advantages and disadvantages of various techniques for measuring the ratio of the gravitational mass to the inertial mass of antihydrogen are discussed. Theoretical considerations and numerical simulations indicate that stochasticity may be especially important for some experimental techniques in vertically oriented traps.
An exhaustive kinetic model for the atoms in a 1D Magneto-Optical Trap is derived, without any approximations. It is shown that the atomic density is described by a Vlasov-Fokker-Planck equation, coupled with two simple differential equations describing the trap beam propagation. The analogy of such a system with plasmas is discussed. This set of equations is then simplified through some approximations, and it is shown that corrective terms have to be added to the models usually used in this context.
We confine 4 10^8 fermionic 6Li atoms simultaneously with 9 10^9 bosonic 7Li atoms in a magneto-optical trap based on an all-semiconductor laser system. We optimize the two-isotope sample for sympathetic evaporative cooling. This is an essential step towards the production of a quantum-degenerate gas of fermionic lithium atoms.
We investigate the limiting factors in the standard implementation of the Ca magneto-optical trap. We find that intercombination transitions from the 4s5p 1P1 state used to repump electronic population from the 3d4s 1D2 state severely reduce the trap lifetime. We explore seven alternative repumping schemes theoretically and investigate five of them experimentally. We find all five of these schemes yield a significant increase in trap lifetime and consequently improve the number of atoms and peak atom density by as much as ~20x and ~6x, respectively. One of these transitions, at 453 nm, is show…
We demonstrate a scheme for magneto-optically trapping strontium monofluoride (SrF) molecules at temperatures one order of magnitude lower and phase space densities three orders of magnitude higher than obtained previously with laser-cooled molecules. In our trap, optical dark states are destabilized by rapidly and synchronously reversing the trapping laser polarizations and the applied magnetic field gradient. The number of molecules and trap lifetime are also significantly improved from previous work by loading the trap with high laser power and then reducing the power for long-term trapping…
We have integrated magneto-optical traps (MOTs) into an atom chip by etching pyramids into a silicon wafer. These have been used to trap atoms on the chip, directly from a room temperature vapor of rubidium. This new atom trapping method provides a simple way to integrate several atom sources on the same chip. It represents a substantial advance in atom chip technology and offers new possibilities for atom chip applications such as integrated single atom or photon sources and molecules on a chip.
A few 85Rb atoms were trapped in a micron-size magneto-optical trap with a high quadrupole magnetic-field gradient and the number of atoms was precisely controlled by suppressing stochastic loading and loss events via real-time feedback on the magnetic field gradient. The measured occupation probability of single atom was as high as 99%. Atoms up to five were also trapped with high occupation probabilities. The present technique could be used to make a deterministic atom source.
We analyze the dynamics of a paramagnetic, dipolar molecule in a generic "magneto-electrostatic'' trap where both magnetic and electric fields may be present. The potential energy that governs the dynamics of the molecules is found using a reduced molecular model that incorporates the main features of the system. We discuss the shape of the trapping potentials for different field geometries, as well as the possibility of nonadiabatic transitions to untrapped states, i.e., the analog of Majorana transitions in a quadrupole magnetic atomic trap. Maximizing the lifetime of molecules in a trap is …
We present a theoretical model describing recently observed collective effects in large magneto-optically trapped atomic ensembles. Based on a kinetic description we develop an efficient test particle method, which in addition to the single atom light pressure accounts for other relevant effects such as laser attenuation and forces due to multiply scattered light with position dependent absorption cross sections. Our calculations confirm the existence of a dynamical instability and provide deeper insights into the observed system dynamics.
Magneto-optical trapping forces for molecules are far weaker than for alkali atoms because the photon scattering rate is reduced when there are multiple ground states, and because of optical pumping into dark states. The force is further reduced when the upper state has a much smaller Zeeman splitting than the lower state. We use a rate model to estimate the strength of the trapping and damping forces in a magneto-optical trap (MOT) of CaF molecules, using either the A$^{2}Π_{1/2}$ - X$^{2}Σ^{+}$ transition or the B$^{2}Σ^{+}$ - X$^{2}Σ^{+}$ transition. We identify a new mechanism of magneto-o…
The cloud of cold atoms produced by a Magneto-Optical Trap is known to exhibit instabilities. We examine in this paper in which limits it could be possible to realize an experimental trap similar to the configurations studied theoretically, i.e. mainly traps where one direction is privileged. We study the static behavior of an anisotropic trap, where anisotropy results essentially from the use of two different laser frequencies for the arms of the trap. Such a trap has very surprising behaviors, in particular the cloud disappears for some laser frequencies, while it exists for smaller and larg…
We describe an apparatus designed to trap and cool a Yb and Cs mixture. The apparatus consists of a dual species effusive oven source, dual species Zeeman slower, magneto-optical traps in a single ultra-high vacuum science chamber, and the associated laser systems. The dual species Zeeman slower is used to load sequentially the two species into their respective traps. Its design is flexible and may be adapted for other experiments with different mixtures of atomic species. The apparatus provides excellent optical access and can apply large magnetic bias fields to the trapped atoms. The apparat…
Radiative decay from the excited $^1P_1$ state to metastable $^3P_2$ and $^3P_0$ states is expected to limit attainable trapped atomic population in a magneto-optic trap of ytterbium (Yb) atoms. In experiments we have carried out with optical repumping of $^3P_{0,2}$ states to $^3P_1$, we observe enhancement of trapped atoms yield in the excited $^1P_1$ state. The individual decay rate to each metastable state is measured and the results show an excellent agreement with the theoretical values.
We report on a novel Magneto-Optical Trap (MOT) geometry involving the retroreflection of one of the six MOT beams in order to create an atom cloud close to the surface of a prism which does not have optical access along one axis. A MOT of Rb$^{85}$ with $\sim 4 \times 10^7$ atoms can be created 700 um from the surface. The MOT lies close to the minimum of an evanescent Gravito-Optical Surface Trap (GOST) allowing for transfer into the GOST with potentially minimal losses.
We have demonstrated that the ion current resulting from collisions between metastable krypton atoms in a magneto-optical trap can be used to precisely measure the trap loading rate. We measured both the ion current of the abundant isotope Kr-83 (isotopic abundance = 11%) and the single-atom counting rate of the rare isotope Kr-85 (isotopic abundance ~ 1x10^-11), and found the two quantities to be proportional at a precision level of 0.9%. This work results in a significant improvement in using the magneto-optical trap as an analytical tool for noble-gas isotope ratio measurements, and will be…
First laser cooling and trapping of the heavy alkaline earth element barium has been achieved based on the strong 6s$^2$ $^1$S$_0$ - 6s6p $^1$P$_1$ transition for the main cooling. Due to the large branching into metastable D-states several additional laser driven transitions are required to provide a closed cooling cycle. A total efficiency of $0.4(1) \cdot 10^{-2}$ for slowing a thermal atomic beam and capturing atoms into a magneto optical trap was obtained. Trapping lifetimes of more than 1.5 s were observed. This lifetime is shortened at high laser intensities by photo ionization losses. …
We demonstrate a 1D magneto-optical trap of the polar free radical calcium monohydroxide (CaOH). A quasi-closed cycling transition is established to scatter $\sim 10^3$ photons per molecule, predominantly limited by interaction time. This enables radiative laser cooling of CaOH while compressing the molecular beam, leading to a significant increase in on-axis beam brightness and reduction in temperature from 8.4 mK to 1.4 mK.
We have developed a unique neutralizer device that uses an yttrium target surrounded by a platinum wall to magneto-optically trap radioactive atoms. In general, the radioactive nucleus produced in a nuclear reaction is extracted and transported in ion form. For the magneto-optical trap, thermal neutralization must occur on the surface of a metal with a small work function. The converter can produce a neutral atomic beam with small angular divergence that, given the recycling of atoms and ions, converts ions into neutral atoms with remarkable efficiency. We demonstrated the ion neutralization p…
Magneto-optical trapping (MOT) is a key technique on the route towards ultracold molecular ensembles. However, the realization and optimization of magneto-optical traps with their wide parameter space is particularly difficult. Here, we present a very general method for the optimization of molecular magneto-optical trap operation by means of Bayesian optimization (BO). As an example for a possible application, we consider the optimization of a calcium fluoride (CaF) MOT for maximum capture velocity. We find that both the $X^2Σ^+\,$ to $A^2Π_{1/2}\,$ and the $X^2Σ^+\,$ to $B^2Σ^+\,$ transition …
A large cloud of $^{87}$Rb atoms confined in a magneto-optical trap exhibits, in a certain regime of parameters, spatio-temporal instabilities with a dynamics resembling that of a turbulent fluid. We apply the methods of turbulence theory based on structure function analysis to extract scaling exponents which are compared to known turbulent regimes. This analysis also allows us to make a clear distinction between different instability regimes.
We report the first observation of a non-dipole transition in an ultra-cold atomic vapor. We excite the 3P-4P electric quadrupole (E2) transition in $^{23}$Na confined in a Magneto-Optical Trap(MOT), and demonstrate its application to high-resolution spectroscopy by making the first measurement of the hyperfine structure of the 4P$_{1/2}$ level and extracting the magnetic dipole constant A $=$ 30.6 $\pm$ 0.1 MHz. We use cw OODR (Optical-Optical Double Resonance) accompanied by photoinization to probe the transition.
We demonstrate the simultaneous magneto-optical trapping (MOT) of Rb and Sr and examine the characteristic loss of Rb in the MOT due to photoionization by the cooling laser for Sr. The photoionization cross section of Rb in the $5P_{3/2}$ state at 461 nm is determined to be $1.4(1)\times10^{-17}$ cm$^2$. It is important to consider this loss rate to realize a sufficiently large number of trapped Rb atoms to achieve a quantum degenerate mixture of Rb and Sr.
We present a study on characteristics of a magneto-optical trap (MOT) as an optical lattice. Fluorescence spectra of atoms trapped in a MOT with a passively phase-stabilized beam configuration have been measured by means of the photon-counting heterodyne spectroscopy. We observe a narrow Rayleigh peak and well-resolved Raman sidebands in the fluorescence spectra which clearly show that the MOT itself behaves as a three-dimensional optical lattice. Optical-lattice-like properties of the phase-stabilized MOT such as vibrational frequencies and lineshapes of Rayleigh peak and Raman sidebands are …
We report the laser-cooling and confinement of Cd atoms in a magneto-optical trap, and characterize the loading process from the background Cd vapor. The trapping laser drives the 1S0-1P1 transition at 229 nm in this two-electron atom and also photoionizes atoms directly from the 1P1 state. This photoionization overwhelms the other loss mechanisms and allows a direct measurement of the photoionization cross section, which we measure to be 2(1)x10^(-16)cm^(2) from the 1P1 state. When combined with nearby laser-cooled and trapped Cd^(+) ions, this apparatus could facilitate studies in ultracold …
This article presents a new experiment aiming at BEC of metastable helium atoms. It describes the design of a high flux discharge source of atoms and a robust laser system using a DBR diode coupled with a high power Yb doped fiber amplifier for manipulating the beam of metastable atoms. The atoms are trapped in a small quartz cell in an extreme high vacuum. The trapping design uses an additional laser (repumper) and allows the capture of a large number of metastable helium atoms (approximately $10^9$) in a geometry favorable for loading a tight magnetostatic trap.
We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler laser cooled in an optical molasses, to a temperature of 110(4) $μ$K. The temperatures and densities achieved here make CaOH a viable candidate for a wide variety of quantum science applications, including the creation of optical tweezer arrays of CaOH molecules. This work also suggests that laser cooling and magneto-optical trapping of many other polyatomi…
We propose different experimental methods to measure the analog of the Debye length in a very large Magneto-Optical Trap, which should characterize the spatial correlations in the atomic cloud. An analytical, numerical and experimental study of the response of the atomic cloud to an external modulation potential suggests that this Debye length, if it exists, is significantly larger than what was expected.
We present a Dual Isotope Magneto Optical Trap produced using a single diode laser. We generate all the optical frequencies needed for trapping both species using a fiber intensity modulator. All the optical frequencies are amplified simultaneously using a tapered amplifier. The independent control of each frequency is on the RF side rather than on the optical side. This introduces an enormous simplification for laser cooling applications that often require an acousto-optic modulator for each laser beam. Frequency changing capabilities are limited by the modulator bandwidth (10 GHz). Traps for…
Low intensity white light was used to increase the loading rate of $^{87}$Rb atoms into a vapor cell magneto-optic trap by inducing non-thermal desorption of Rb atoms from the stainless steel walls of the vapor cell. An increased Rb partial pressure reached a new equilibrium value in less than 10 seconds after switching on the broadband light source. After the source was turned off, the partial pressure returned to its previous value in $1/e$ times as short as 10 seconds.
We demonstrate a Magneto-Optical Trap (MOT) configuration which employs optical forces due to light scattering between electronically excited states of the atom. With the standard MOT laser beams propagating along the {\it x}- and {\it y}- directions, the laser beams along the {\it z}-direction are at a different wavelength that couples two sets of {\it excited} states. We demonstrate efficient cooling and trapping of cesium atoms in a vapor cell and sub-Doppler cooling on both the red and blue sides of the two-photon resonance. The technique demonstrated in this work may have applications in …