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arXiv 2602.02463physics.opticscond-mat.mtrl-sci
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数值优化FROG结果用于研究多频率拉曼生成中红移谱

Numerically optimized FROG results for the study of red-shifted spectra in multi-frequency Raman generation

IIT Madras(印度理工学院马德拉斯分校);University of Waterloo(滑铁卢大学);Meta;Indian Institute of Science(印度科学学院);IIT Bhubaneswar(印度理工学院布巴内斯瓦尔分校);RWTH Aachen University(亚琛工业大学)

Sakthi Priya Amirtharaj, Zujun Xu, Donna Strickland, Borun Chowdhury, Sagnik Acharya, Priyam Samantray, Anil Prabhakar, Kisor Kumar Sahu, Franz Bamer, S. Swayamjyoti

AI总结:

本研究利用FROG技术分析多频率拉曼生成中红移谱的演变,通过双脉冲干涉模型和自适应学习算法揭示了线性拉曼过程在两光子 dressed-state 框架中的作用。

摘要:

当双脉冲压缩泵浦脉冲驱动多频率拉曼散射进入暂态区域时,所产生的反斯托克斯阶次表现出向低频方向不对称的谱展宽,导致每个阶次中出现特征性的双峰结构。在本通信中,利用频率分辨光学门(FROG)研究了第一反斯托克斯拉曼成分的谱演变。为解释观测到的特征,我们引入了双脉冲干涉模型,并采用基于自适应学习的重建算法,使用Adam优化器来恢复时间场演变。模拟结果与实验测量结果具有良好的一致性。我们的分析表明,观测到的红移谱成分源于两光子 dressed-state 框架内的线性拉曼过程。

英文摘要:

When multifrequency Raman scattering is driven in the transient regime by two chirped pump pulses, the resulting anti-Stokes orders exhibit asymmetric spectral broadening toward lower frequencies, leading to a characteristic double-peaked structure in each order. In this Letter, frequency-resolved optical gating (FROG) is used to investigate the spectral evolution of the first anti-Stokes Raman component. To interpret the observed features, we introduce a double-pulse interference model and employ an adaptive learning-based reconstruction algorithm using the Adam optimizer to retrieve the temporal field evolution. The simulation results show good agreement with the experimental measurements. Our analysis indicates that the observed red-shifted spectral component originates from linear Raman processes within the two-photon dressed-state framework.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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