arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2601.04097cond-mat.str-el
收藏

超导性、Kondo物理与磁序:通过3d和4f相关电子的相互作用调控La$_{1-x}$Ce$_x$FeSiH固溶体的基态

Superconductivity, Kondo physics and magnetic order: Tuning the groundstate in the La$_{1-x}$Ce$_x$FeSiH solid solution through the interplay between $3d$ and $4f$ correlated electrons

University of Bordeaux(波尔多大学);CNRS(法国国家科学研究中心);Helmholtz-Zentrum Dresden-Rossendorf(亥姆霍兹德累斯顿-罗斯多夫中心)

J. Sourd, B. Vignolle, E. Gaudin, S. Burdin, S. Tencé

AI总结:

通过调控La$_{1-x}$Ce$_x$FeSiH固溶体中的铈含量,研究3d和4f相关电子的Kondo纠缠,揭示超导态与Kondo相干态的转变。

摘要:

我们报告了对La$_{1-x}$Ce$_x$FeSiH固溶体(0 ≤ x ≤ 1)的研究,这是一种具有ZrCuSiAs型结构的金属氢化物家族,空间群为P4/nmm。对于低浓度的铈(x ≤ 0.20),我们观察到超导性的存在,其起源于铁的关联3d电子。超导区域随着铈的取代逐渐被抑制。对于中等浓度的铈(0.07 ≤ x ≤ 0.50),我们观察到单离子Kondo效应的证据,且在2 K以下没有磁相变。对于0.07 ≤ x ≤ 0.20,单离子Kondo效应与低温下的超导基态共存。对于x > 0.50,我们观察到Kondo相干和低温下的重费米液体区域。最后,在高浓度的铈(x ≥ 0.85)下,我们观察到低温下的磁序特征。我们通过引入与超导性、Kondo效应和磁序相关的温度尺度,构建了一个丰富的相图(温度与铈含量x)。这表明,通过使用铈浓度x作为唯一控制参数,可以探索3d和4f相关电子之间的Kondo纠缠,这表明超导态(与3d电子相关)与Kondo相干态(涉及3d和4f电子)之间存在异常的变化。

英文摘要:

We report a study of the La$_{1-x}$Ce$_x$FeSiH solid solution ($0 \leq x \leq 1$), a family of intermetallic hydrides of ZrCuSiAs-type structure, with space group $P4/nmm$. For low cerium concentrations $x \leq 0.20$, we observe the presence of superconductivity, which originates from the correlated $3d$ electrons of iron. The superconducting regime is progressively suppressed by the cerium substitution. For moderate cerium concentration $0.07 \leq x \leq 0.50$, we observe evidence of the single-ion Kondo effect and no magnetic phase transition down to 2 K. For $0.07 \leq x \leq 0.20$, the single-ion Kondo effect coexists with a superconducting ground state at low temperatures. From $x > 0.50$, we observe signatures of Kondo coherence and a heavy Fermi liquid regime at low temperature. Finally, at high cerium concentration $x \geq 0.85$, we observe signatures of magnetic ordering at low temperatures. We discuss our results by introducing temperature scales related to superconductivity, the Kondo effect, and magnetic order, which permits building a rich phase diagram temperature versus cerium content $x$. This shows that using the cerium concentration $x$ as a unique control parameter, we can explore the Kondo entanglement between correlated $3d$ and $4f$ electrons, which suggests an unusual change between the superconducting state related to the $3d$ electrons and the Kondo coherent state involving both $3d$ and $4f$ electrons.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑