arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2510.04431cond-mat.supr-concond-mat.mtrl-sci
收藏

关联无限层La$_{1-x}$Sr$_x$NiO$_2$中超导配对强度与塞贝克系数的系统演化

Systematic evolution of superconducting pairing strength and Seebeck coefficients in correlated infinite-layer La$_{1-x}$Sr$_x$NiO$_2$

Motoki Osada, Shusaku Imajo, Yuji Seki, Kousuke Ishida, Tsutomu Nojima, Kohei Fujiwara, Koichi Kindo, Yusuke Nomura, Atsushi Tsukazaki

AI总结:

本研究系统探究无限层(La,Sr)NiO$_2$的超导特性,发现其强耦合超导可突破泡利极限,且正常态热电性质演化与超导配对强度、各向异性演化相关联,证实电子关联与强耦合超导的明确联系,助力非常规超导统一理解框架的构建。

摘要:

近期发现的无限层镍酸盐提供了一个全新平台,可用于探索多带系统中面向高温超导及相关丰富量子相的奇异配对机制,这与铜氧化物形成对比。本文中,我们证明无限层(La,Sr)NiO$_2$表现出强耦合超导性,在最佳掺杂下可承受超过47 T的面内磁场——这一数值是传统BCS超导体泡利极限的两倍以上。这种违背效应在欠掺杂区域变得显著,表明配对胶存在引人关注的演化。在该区域意外观测到的正塞贝克系数,说明存在非平凡的电子关联。此外,我们对整个超导穹顶的综合研究显示,正常态(热)电性质的演化——具体而言是霍尔系数和塞贝克系数的符号变化——与超导各向异性和配对强度的演化相一致。这证明了(La,Sr)NiO$_2$中电子关联与强耦合超导性之间存在明确关联,为理解非常规超导的统一框架提供了支撑。

英文摘要:

The recently discovered superconducting infinite-layer nickelates offer a novel platform to explore an exotic pairing mechanism in multi-band systems towards high-temperature superconductivity and associated rich quantum phases, contrasting with cuprates. Here, we show that infinite-layer (La,Sr)NiO$_2$ exhibits strong-coupling superconductivity, resilient to in-plane magnetic fields exceeding 47 T at optimal doping - more than twice the Pauli limit for conventional BCS superconductors. This violation becomes pronounced towards the underdoped regime, implying an intriguing evolution of pairing glue. The unexpected observation of positive Seebeck coefficients in this regime indicates the presence of nontrivial electron correlations. Furthermore, our comprehensive investigation across the superconducting dome reveals that the evolution of (thermo)electric normal-state properties - specifically, the sign changes of the Hall and Seebeck coefficients - coincide with the evolution of superconducting anisotropy and pairing strength. This demonstrates a definitive link between electron correlations and strong-coupling superconductivity in (La,Sr)NiO$_2$, contributing to a unified framework for understanding unconventional superconductivity.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑