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arXiv 2510.02429cond-mat.supr-concond-mat.dis-nncond-mat.mtrl-sciquant-ph
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利用量子传感器揭示La$_3$Ni$_2$O$_7$中异质超导性的起源

Uncovering origins of heterogeneous superconductivity in La$_3$Ni$_2$O$_7$ using quantum sensors

Harvard University(哈佛大学);Boston University(波士顿大学);Massachusetts Institute of Technology(麻省理工学院);Iowa State University(爱荷华州立大学)

Srinivas V. Mandyam, Esther Wang, Zhipan Wang, Bijuan Chen, Nishan C. Jayarama, Anmay Gupta, Eric A. Riesel, Valery I. Levitas, Christopher R. Laumann, Norman Y. Yao

AI总结:

利用量子传感器研究La$_3$Ni$_2$O$_7$中异质超导性的起源,揭示抑制和增强超导的机制。

摘要:

镍酸盐超导体家族长期以来被用作高温杯状体的类比。然而,最近发现某些化学计量比的镍酸盐在高压下可以超导到较高的$T_c$,这令人惊讶。超导态背后的机制仍不清楚。除了高压环境带来的实际挑战外,典型样品表现出异常弱的抗磁响应,这些已被推测反映非均匀的`纤维状'超导态。我们通过宽场、高压、光检测磁共振光谱学来成像原生La$_3$Ni$_2$O$_7$样品的局部抗磁响应,使用嵌入金刚石压裂机中的氮空位量子传感器。这些地图证实了在几微米尺度上功能超导响应的显著不均匀性。通过将抗磁Meissner响应与本地张量应力环境以及化学计量比进行空间相关性分析,我们揭示了抑制和增强超导性的主导机制。我们的宽场技术同时提供了样品行为的广泛视角和出色的局部灵敏度,使能够从亚微米像素尺度观察到的局部结构-功能相关性中快速构建多参数相图。

英文摘要:

The family of nickelate superconductors have long been explored as analogs of the high temperature cuprates. Nonetheless, the recent discovery that certain stoichiometric nickelates superconduct up to high $T_c$ under pressure came as a surprise. The mechanisms underlying the superconducting state remain experimentally unclear. In addition to the practical challenges posed by working in a high pressure environment, typical samples exhibit anomalously weak diamagnetic responses, which have been conjectured to reflect inhomogeneous `filamentary' superconducting states. We perform wide-field, high-pressure, optically detected magnetic resonance spectroscopy to image the local diamagnetic responses of as grown La$_3$Ni$_2$O$_7$ samples \emph{in situ}, using nitrogen vacancy quantum sensors embedded in the diamond anvil cell. These maps confirm significant inhomogeneity of the functional superconducting responses at the few micron scale. By spatially correlating the diamagnetic Meissner response with both the local tensorial stress environment, also imaged \emph{in situ}, and stoichiometric composition, we unravel the dominant mechanisms suppressing and enhancing superconductivity. Our wide-field technique simultaneously provides a broad view of sample behavior and excellent local sensitivity, enabling the rapid construction of multi-parameter phase diagrams from the local structure-function correlations observed at the sub-micron pixel scale.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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