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arXiv 2502.03361cond-mat.mtrl-sci
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薄 WSe$_2$ 波导中激子极化激元的光发射电子显微术

Photoemission electron microscopy of exciton-polaritons in thin WSe$_2$ waveguides

Tobias Eul, Miwan Sabir, Victor DeManuel-Gonzalez, Florian Diekmann, Kai Rossnagel, Michael Bauer

AI总结:

本研究利用光发射电子显微术表征薄 WSe$_2$ 波导中激子与横电/横磁光子模式的强耦合,提取色散及 Rabi 分裂,为时间分辨传播研究奠定基础。

摘要:

在强耦合区域由光子与激子相互作用产生的激子极化激元,是一类引人关注的准粒子,因为在光捕获等光-物质相互作用过程中存在潜在的能量交换。这种耦合会在以激子共振为中心的光子色散关系中引起能量反交叉,即在较低和较高能量分支之间形成 Rabi 分裂。该分裂的大小与激子和光子模式之间的耦合强度相关。在本工作中,我们研究了在过渡金属二硫族化合物 WSe$_2$ 的薄膜薄片中同时激发的激子与光子波导模式之间的这种耦合。利用光发射电子显微镜,我们能够提取在这些薄片中传播的横电模式和横磁模式的色散关系,并提取能量分裂。最终,我们的发现为通过时间分辨光发射研究激子极化激元在时间域中的传播提供了基础。

英文摘要:

Exciton-polaritons emerging from the interaction of photons and excitons in the strong coupling regime are intriguing quasiparticles for the potential exchange of energy during light-matter interaction processes such as light harvesting. The coupling causes an energy anti-crossing in the photon dispersion centered around the exciton resonance, i.e., a Rabi splitting between a lower and upper energetic branch. The size of this splitting correlates with the coupling strength between the exciton and the photonic modes. In this work, we investigate this coupling between excitons and photonic waveguide modes excited simultaneously in thin-film flakes of the transition-metal dichalcogenide WSe$_2$. Using a Photoemission electron microscope, we are able to extract the dispersion of the transversal electric and magnetic modes propagating through these flakes as well as extract the energy splitting. Ultimately, our findings provide a basis for the investigation of the propagation of exciton-polaritons in the time-domain via time-resolved photoemission.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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