Silicon vacancy centers in 4H-silicon carbide (SiC) host a long-lived electronic spin and simultaneously possess spin-resolved optical transitions, making them a great candidate for implementing a spin-photon interface. These interfaces are an important building block of quantum networks, which in turn promise to enable secure communication and distributed quantum computing. To achieve this goal, the rate of coherently scattered photons collected from a single emitter needs to be maximized, which can be achieved by interfacing the emitter with an optical cavity. In this work, we integrate V2 centers inside a SiC membrane into a fiber-based Fabry-Pérot microcavity. We find that SiC lends itself well to membrane fabrication, as evidenced by low surface roughness $σ_{\mathrm{RMS}}$ ~ 400 pm, high reproducibility, and consequentially a high cavity finesse F ~ 40 000. At cryogenic temperatures, we observe individual emitters coupling to cavity modes. We confirm their single-emitter character by measuring the second-order autocorrelation function and investigate the Purcell factor by measuring the optical lifetime as a function of the cavity-emitter detuning. We find a 13.3-fold enhancement of photons scattered into the zero-phonon line (ZPL), which could be further increased by using optimized mirror coatings, potentially opening the path towards deterministic spin-photon interaction.
We study a dispersion-compensated high-finesse optical Fabry-Perot microcavity under high-intensity cw pumping. The Kerr non-linearity in the optical coatings causes a spontaneous four-wave mixing process, which leads to the emission of time-correlated photon pairs. The photon frequencies are shifted by $\pm 1$ free spectral range relative to the pump frequency. This setup allows for constructing a photon-pair source with precisely adjustable frequency difference between the emitted photons, which may have applications in quantum communication.
We present both theoretical and experimental results on fluorescence of single defect centers in diamond nanocrystals embedded in a planar dielectric microcavity. From a theoretical point of view, we show that the overall fluorescence collection efficiency using moderate numerical aperture microscope objective can be enhanced by using a low quality factor microcavity. This could be used in particular for low temperature applications where the numerical aperture of collection microscope objectives is limited due to the experimental constraints. We experimentally investigate the control of the f…
Open Fabry-Perot microcavities represent a promising route for achieving a quantum electrodynamics (cavity-QED) platform with diamond-based emitters. In particular, they offer the opportunity to introduce high purity, minimally fabricated material into a tunable, high quality factor optical resonator. Here, we demonstrate a fiber-based microcavity incorporating a thick (> 10 μm) diamond membrane with a finesse of 17,000, corresponding to a quality factor Q ~ $10^6$. Such minimally fabricated, thick samples can contain optically stable emitters similar to those found in bulk diamond. We observe…
Organic dye molecules have been used in great many scientific and technological applications, but their wider use in quantum optics has been hampered by transitions to short-lived vibrational levels, which limit their coherence properties. To remedy this, one can take advantage of optical resonators. Here we present the first results on coherent molecule-resonator coupling, where a single polycyclic aromatic hydrocarbon molecule extinguishes 38\% of the light entering a microcavity at liquid helium temperature. We also demonstrate four-fold improvement of single-molecule stimulated emission co…
We report on the fabrication and characterization of a scannable Fabry-Perot microcavity, consisting of a curved micromirror at the end of an optical fiber and a planar distributed Bragg reflector. Furthermore, we demonstrate the coupling of single organic molecules embedded in a thin film to well-defined resonator modes. We discuss the choice of cavity parameters that will allow sufficiently high Purcell factors for enhancing the zero-phonon transition between the vibrational ground levels of the electronic excited and ground states.
High-finesse, open-geometry microcavities have recently emerged as a versatile tool for enhancing interactions between photons and material systems, with a range of applications in quantum optics and quantum information science. However, mechanical vibrations pose a considerable challenge to their operation within a closed-cycle cryostat, particularly when spatial tunability and free-space optical access are required. Here, we present the design and characterization of a system that can achieve $\sim$16 pm-rms passive mechanical stability between two high-finesse mirrors while permitting both …
We report on the realization of an open plane-concave Fabry-Pérot resonator with a mode volume below $λ^3$ at optical frequencies. We discuss some of the less common features of this new microcavity regime and show that the ultrasmall mode volume allows us to detect cavity resonance shifts induced by single nanoparticles even at quality factors as low as $100$. Being based on low-reflectivity micromirrors fabricated on a silicon cantilever, our experimental arrangement provides broadband operation, tunability of the cavity resonance, lateral scanning and promise for optomechanical studies.
We study the optomechanical coupling of a single-layer graphene with a high-Q Fabry-Perot microcavity in the membrane-in-the-middle configuration. In ordinary dissipative coupling systems, mechanical oscillators modulate the loss associated with the input coupling of the cavity mode; while in our system, the graphene oscillator couples dissipatively with the cavity mode through modulating its absorption loss. By analyzing the effects of the interband transition of a graphene suspended near the node of the cavity field, we obtain strong and tunable dissipative coupling without excessively reduc…
We report on the detection of free nanoparticles in a micromachined, open-access Fabry-Pérot microcavity. With a mirror separation of $130\,μ$m, a radius of curvature of $1.3\,$mm, and a beam waist of $12\,μ$m, the mode volume of our symmetric infrared cavity is smaller than $15\,$pL. The small beam waist, together with a finesse exceeding 34,000, enables the detection of nano-scale dielectric particles in high vacuum. This device allows monitoring of the motion of individual $150\,$nm radius silica nanospheres in real time. We observe strong coupling between the particles and the cavity field…
We report on the fabrication and characterization of a Fabry-Perot microcavity enclosing a thin diamond membrane at cryogenic temperatures. The cavity is designed to enhance resonant emission of single nitrogen-vacancy centers by allowing spectral and spatial tuning while preserving the optical properties observed in bulk diamond. We demonstrate cavity finesse at cryogenic temperatures within the range of F = 4,000-12,000 and find a sub-nanometer cavity stability. Modeling shows that coupling nitrogen-vacancy centers to these cavities could lead to an increase of remote entanglement success ra…
A microfabricated Fabry-Perot optical resonator has been used for atom detection and photon production with less than 1 atom on average in the cavity mode. Our cavity design combines the intrinsic scalability of microfabrication processes with direct coupling of the cavity field to single-mode optical waveguides or fibers. The presence of the atom is seen through changes in both the intensity and the noise characteristics of probe light reflected from the cavity input mirror. An excitation laser passing transversely through the cavity triggers photon emission into the cavity mode and hence int…
Direct laser-written optomechanical double membranes in an optical microcavity
University of Bonn（波恩大学）；Technical University of Munich（慕尼黑工业大学）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）；Chalmers University of Technology（查尔姆斯理工大学）
We describe a method to map the standing-wave pattern inside a Fabry-Perot optical cavity with sub-wavelength resolution by perturbing it with a commercially available scanning near-field optical microscope (SNOM) tip. The method is applied to a fiber Fabry-Perot microcavity. We demonstrate its use to determine the relative position of the antinodes at two different wavelengths. In addition, we use the SNOM tip as a point-like source allowing precise positioning of a microscope objective with respect to the cavity mode.
We develop a light-matter interface enabling strong and uniform coupling between a chain of cold atoms and photons of an optical cavity. This interface is a fiber Fabry-Perot cavity, doubly resonant for both the wavelength of the atomic transition and for a geometrically commensurate red-detuned intracavity trapping lattice. Fulfilling the condition of a strong and uniform atom-photon coupling requires optimization of the spatial overlap between the two standing waves in the cavity. In a strong-coupling cavity, where the mode waists and Rayleigh range are small, we derive the expression of the…
Optical microcavities are a powerful tool to enhance spontaneous emission of individual quantum emitters. However, the broad emission spectra encountered in the solid state at room temperature limit the influence of a cavity, and call for ultra-small mode volume. We demonstrate Purcell-enhanced single photon emission from nitrogen-vacancy (NV) centers in nanodiamonds coupled to a tunable fiber-based microcavity with a mode volume down to $1.0\,λ^{3}$. We record cavity-enhanced fluorescence images and study several single emitters with one cavity. The Purcell effect is evidenced by enhanced flu…
Coupling nitrogen-vacancy centers in diamond to optical cavities is a promising way to enhance the efficiency of diamond based quantum networks. An essential aspect of the full toolbox required for the operation of these networks is the ability to achieve microwave control of the electron spin associated with this defect within the cavity framework. Here, we report on the fabrication of an integrated platform for microwave control of an NV center electron spin in an open, tunable Fabry-Perot microcavity. A critical aspect of the measurements of the cavity's finesse reveals that the presented f…
High-cooperativity coupling and spin-resolved extinction of tin-vacancy centers in a diamond-like microcavity
Karlsruhe Institute of Technology (KIT)（卡尔斯鲁厄理工学院）；University of Kassel（卡塞尔大学）；University of Stuttgart（斯图加特大学）；Ulm University（乌尔姆大学）；University of Leipzig（莱比锡大学）；Ferdinand-Braun-Institut (FBH)（费迪南德·布劳恩研究所）；Humboldt-Universität zu Berlin（柏林洪堡大学）；Fraunhofer Institute for Applied Solid State Physics（弗劳恩霍夫应用固态物理研究所）
We present a new approach to incorporate self-assembled quantum dots into a Fabry-Pérot-like microcavity. Thereby a 3$λ$/4 GaAs layer containing quantum dots is epitaxially removed and attached by van der Waals bonding to one of the microcavity mirrors. We reach a finesse as high as 4,100 with this configuration limited by the reflectivity of the dielectric mirrors and not by scattering at the semiconductor - mirror interface, demonstrating that the epitaxial lift-off procedure is a promising procedure for cavity quantum electrodynamics in the solid state. As a first step in this direction, we…
Optical microcavities allow to strongly confine light in small mode volumes and with long photon lifetimes. This confinement significantly enhances the interaction between light and matter inside the cavity, with applications such as optical trapping and cooling of nanoparticles, single-photon emission enhancement, quantum information processing, and sensing. For many applications, open resonators with direct access to the mode volume are necessary. Here we report on a scalable, open-access optical microcavity platform with mode volumes < 30 $λ^3$ and finesse approaching $5x10^5$. This result …
With a highly coherent, optically addressable electron spin, the nitrogen vacancy (NV) centre in diamond is a promising candidate for a node in a quantum network. However, the NV centre is a poor source of coherent single photons owing to a long radiative lifetime, a small branching ratio into the zero-phonon line (ZPL) and a poor extraction efficiency out of the high-index host material. In principle, these three shortcomings can be addressed by resonant coupling to a single mode of an optical cavity. Utilising the weak-coupling regime of cavity electrodynamics, resonant coupling between the …
We present two novel schemes to generate photon polarization entanglement via single electron spins confined in charged quantum dots inside microcavities. One scheme is via entangled remote electron spins followed by negatively-charged exciton emissions, and another scheme is via a single electron spin followed by the spin state measurement. Both schemes are based on giant circular birefringence and giant Faraday rotation induced by a single electron spin in a microcavity. Our schemes are deterministic and can generate an arbitrary amount of multi-photon entanglement. Following similar procedu…
We show that a broadband Fabry-Perot microcavity can assist an emitter coupled to an off-resonant plasmonic nanoantenna to inhibit the nonradiative channels that affect the quenching of fluorescence. We identify the interference mechanism that creates the necessary enhanced couplings and bandwidth narrowing of the hybrid resonance and show that it can assist entering into the strong coupling regime. Our results provide new possibilities for improving the efficiency of solid-state emitters and accessing diverse realms of photophysics with hybrid structures that can be fabricated using existing …
Up to now, all the works about constructing quantum logic gates, an essential part in quantum computing, are focused on operating on one degree of freedom (DOF) of quantum systems. Here, we investigate the possibility to achieve a scalable photonic quantum computing based on two DOFs of quantum systems and construct a deterministic hyper-controlled-not (hyper-CNOT) gate operating on both spatial-mode and polarization DOFs of a photon pair simultaneously, by using the giant optical Faraday rotation induced by a single-electron spin in a quantum dot inside a one-side optical microcavity as a res…
Assisted with linear optical manipulation, single photon, entangled photon pairs, photon measurement, and classical communication, a scheme for two-spin qubits phase gate and teleportation of a CNOT gate between two electron spins from acting on local qubits to acting on remote qubits using quantum dots in optical microcavities is proposed. The scheme is based on spin selective photon reflection from the cavity and is achieved in a deterministic way by the sequential detection of photons and the single-qubit rotations of a single electron spin in a self-assembled GaAs/InAs quantum dot. The fea…
Whispering-gallery microcavity laser possesses ultralow threshold, whereas convenient free-space optical excitation and collection suffer from low efficiencies due to its rotational symmetry. Here we analytically study a three-dimensional microsphere coupled to a nano-sized scatterer in the framework of quantum optics. It is found that the scatterer is capable of coupling light in and out of the whispering-gallery modes (WGMs) without seriously degrading their high-Q properties, while the microsphere itself plays the role of a lens to focus the input beam on the scatterer and vice versa. Our a…
Quantum key distribution enables secure communication based on the principles of quantum mechanics. The distance in fiber-based quantum communication is limited to about a hundred kilometers due to signal attenuation. Thus, quantum repeaters are required to establish large-scale quantum networks. Ideal quantum repeater nodes possess a quantum memory which is efficiently connected to photons, the carrier of quantum information. Color centers in diamond and, in particular, the negatively-charged silicon-vacancy centers are promising candidates to establish such nodes. The major obstacle is an in…
We analyze a detailed model of a Bose-Einstein condensate trapped in a ring optical resonator and contrast its classical and quantum properties to those of a Fabry-P{é}rot geometry. The inclusion of two counter-propagating light fields and three matter field modes leads to important differences between the two situations. Specifically, we identify an experimentally realizable region where the system's behavior differs strongly from that of a BEC in a Fabry-Pérot cavity, and also where quantum corrections become significant. The classical dynamics are rich, and near bifurcation points in the me…
We propose a quantum non-demolition method - giant Faraday rotation - to detect a single electron spin in a quantum dot inside a microcavity where negatively-charged exciton strongly couples to the cavity mode. Left- and right-circularly polarized light reflected from the cavity feels different phase shifts due to cavity quantum electrodynamics and the optical spin selection rule. This yields giant and tunable Faraday rotation which can be easily detected experimentally. Based on this spin-detection technique, a scalable scheme to create an arbitrary amount of entanglement between two or more …
This chapter reviews the fundamental optical properties and applications of pho-tonic molecules (PMs) - photonic structures formed by electromagnetic coupling of two or more optical microcavities (photonic atoms). Controllable interaction between light and matter in photonic atoms can be further modified and en-hanced by the manipulation of their mutual coupling. Mechanical and optical tunability of PMs not only adds new functionalities to microcavity-based optical components but also paves the way for their use as testbeds for the exploration of novel physical regimes in atomic physics and qu…
We propose an all optical quantum computation scheme, with trapped electron spin qubits, using their Coulomb exchange interaction with optically excited microcavity exciton-polaritons. This paper describes a single qubit rotation, which together with two-qubit controlled-z gate presented in PRB 85, 241403(R) (2012), form a set of universal logic gates. The errors due to finite cavity lifetime and incorrect orientation of the rotation axis are minimized by optimizing pump pulse parameters. With projective homodyne phase measurement and initialization, our scheme is a promising candidate for the…
Programmable cavity QED with a fiber-integrated atomic array
Institute of Science and Technology Austria (ISTA)（奥地利科学技术研究院）；Vienna Center for Quantum Science and Technology, Atominstitut, TU Wien（维也纳量子科学与技术中心，原子物理研究所，维也纳工业大学）
