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arXiv 2409.03063cond-mat.str-el
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Kagomé晶格上电荷密度波与磁性的相互作用

Interplay of Charge Density Wave and Magnetism on the Kagomé Lattice

Yu-Han Lin, Jin-Wei Dong, Ruiqing Fu, Xian-Xin Wu, Ziqiang Wang, Sen Zhou

AI总结:

受FeGe中CDW启发,研究kagomé晶格单轨道模型,发现库仑作用驱动键序CDW并增强铁磁序,形成具量子反常霍尔效应的Chern绝缘体。

摘要:

受近期在磁性kagomé金属FeGe中发现电荷密度波(CDW)序的启发,我们研究了kagomé晶格上的单轨道$t$-$U$-$V_1$-$V_2$模型,其中$U$、$V_1$和$V_2$分别代表在位、最近邻和次近邻库仑排斥。当费米能级处于平带中时,在足够大的在位$U$作用下,向铁磁(FM)序演化的不稳定性会产生FM半金属。有趣的是,在能带填充$n=17/24$时,费米能级穿过该半金属自旋少数能带的van Hove奇点。我们证明,由于kagomé晶格在van Hove奇点处的独特几何与子晶格干涉效应,格间库仑相互作用$V_1$和$V_2$分别驱动了实键序和虚键序的$2a_0 \ imes 2a_0$ CDW不稳定性。具有复键序的FM环路电流CDW是一种展示量子反常霍尔效应的自旋极化Chern绝缘体。研究发现,与相应的van Hove填充下的非磁性kagomé金属相比,键涨落得到显著增强,为包括FM环路电流CDW在内的键序CDW优先于在位电荷密度序态出现提供了具体的模型实现。当自旋部分极化时,我们发现键序CDW的形成显著增强了有序磁矩。这些发现为kagomé晶格上环路电流与键序CDW的出现及其与磁性的相互作用提供了物理见解,并可能与磁性kagomé金属FeGe存在联系。

英文摘要:

Motivated by the recent discovery of charge density wave (CDW) order in the magnetic kagomé metal FeGe, we study the single-orbital $t$-$U$-$V_1$-$V_2$ model on the kagomé lattice, where $U$, $V_1$, and $V_2$ are the onsite, nearest neighbor, and next-nearest-neighbor Coulomb repulsions, respectively. When the Fermi level lies in the flat band, the instability toward ferromagnetic (FM) order gives rise to a FM half-metal at sufficiently large onsite $U$. Intriguingly, at band filling $n=17/24$, the Fermi level crosses the van Hove singularity of the spin-minority bands of the half-metal. We show that, due to the unique geometry and sublattice interference on the kagomé lattice at van Hove singularity, the intersite Coulomb interactions $V_1$ and $V_2$ drive a real and an imaginary bond-ordered $2a_0 \times 2a_0$ CDW instability, respectively. The FM loop current CDW with complex bond orders is a spin-polarized Chern insulator exhibiting the quantum anomalous Hall effect. The bond fluctuations are found to be substantially enhanced compared to the corresponding nonmagnetic kagomé metals at van Hove filling, providing a concrete model realization of the bond-ordered CDWs, including the FM loop current CDW, over the onsite charge density ordered states. When the spins are partially polarized, we find that the formation of bond-ordered CDWs enhances substantially the ordered magnetic moments. These findings provide physical insights for the emergence of loop-current and bond-ordered CDW and their interplay with magnetism on the kagomé lattice, with possible connections to the magnetic kagomé metal FeGe.

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