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arXiv 2408.03471cond-mat.mtrl-scicond-mat.mes-hall
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1/3-火、2/3-冰亚铁磁体SmMn$_2$Ge$_2$中具有太赫兹尝试频率的量子自旋弛豫

Quantum Spin Relaxation with THz Attempt Frequency in the 1/3-Fire, 2/3-Ice Ferrimagnet SmMn$_2$Ge$_2$

M. L. McLanahan, A. P. Ramirez

AI总结:

本研究在1/3-火、2/3-冰亚铁磁材料SmMn$_2$Ge$_2$中发现新型单自旋共振,通过交流磁化率测得类德拜共振的Orbach弛豫特性与太赫兹尝试频率,证实该弛豫源于畴界Mn自旋提供翻转场的Sm顺磁自旋,为奇异磁基态研究提供实验支撑。

摘要:

其中一半自旋无序、一半自旋有序的亚铁磁体(即所谓半火半冰态),在理论上被提出是实现奇异磁性基态的一种途径。本文中,我们在1/3-火、2/3-冰材料SmMn$_2$Ge$_2$中观测到了新型单自旋共振。通过0.1 Hz–1 kHz频率范围内的交流磁化率测量,我们发现了具有Orbach弛豫温度依赖特性的类德拜共振,得到能垒$E_B \approx 840$ $k_B$,且尝试频率处于太赫兹范围。这些结果强烈表明,单自旋弛豫发生在顺磁性Sm自旋之间,其翻转场由畴界处铁磁有序的Mn自旋提供,这是1/3-火、2/3-冰态的直接结果。

英文摘要:

Ferrimagnets in which half the spins are disordered and half ordered, so-called half-fire, half-ice state, have been advanced theoretically as a route towards realizing exotic magnetic ground states. Here we demonstrate novel single-spin resonance in SmMn$_2$Ge$_2$, a 1/3-fire, 2/3-ice material. Using ac-susceptibility in the frequency range 0.1 Hz - 1 kHz we find a Debye-like resonance with Orbach relaxation temperature dependence, yielding an energy barrier $E_B \approx 840$ $k_B$ and attempt frequencies in the THz range. These quantities strongly suggest single-spin relaxation among paramagnetic Sm spins where the flipping field is provided by the FM-ordered Mn spins at domain boundaries, a direct outcome of the 1/3-fire, 2/3-ice state.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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