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arXiv 2407.05798cond-mat.supr-concond-mat.mes-hallcond-mat.mtrl-sci
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拓扑超导体候选材料AuSn$_{4}$中非常规Rashba能带与涡旋零模的可视化

Visualization of Unconventional Rashba Band and Vortex Zero Mode in Topopogical Superconductor Candidate AuSn$_{4}$

Yuhan Ye, Rui Song, Hongqin Xiao, Guoyu Xian, Hui Guo, Haitao Yang, Hui Chen, Hong-Jun Gao

AI总结:

本研究通过扫描隧道显微镜直接观测AuSn4的Au终止表面,发现非常规Rashba能带和类似马约拉纳零模的涡旋零能态,为拓扑超导研究提供新平台。

摘要:

拓扑超导电性(TSC)是承载马约拉纳零模(MZM)以实现拓扑量子计算的有前景平台。最近,贵金属合金AuSn$_{4}$已被确认为一种本征表面拓扑超导体。然而,其非平凡表面态和MZM的原子级可视化仍然难以实现。在此,我们通过超低温度扫描隧道显微镜/谱学报告了在AuSn$_{4}$的金(Au)终止表面上对非常规表面态和涡旋零模的直接观测。与锡(Sn)表面上的平凡金属体态不同,Au终止表面在费米能级附近展现出显著的表面态。我们的密度泛函理论计算表明,这些态源于非常规Rashba能带,其中来自不同能带的两条费米圆共享相同的螺旋自旋纹理、手性和群速度方向。此外,我们发现尽管超导能隙、临界温度、各向异性面内临界场在Au和Sn终止表面上几乎相同,但Abrikosov涡旋核心内的隙内束缚态显示出显著差异。Sn终止表面上的涡旋表现出常规的Caroli-de Gennes-Matricon束缚态,而Au表面则显示出尖锐的零能核心态,具有长的非劈裂距离,类似于非量子极限条件下的MZM。这种差异可能源于Au终止表面费米能级附近非常规Rashba能带的主导贡献。我们的结果为研究超导体中的非常规Rashba能带和MZM提供了新平台。

英文摘要:

Topological superconductivity (TSC) is a promising platform to host Majorana zero mode (MZM) for topological quantum computing. Recently, the noble metal alloy AuSn$_{4}$ has been identified as an intrinsic surface TSC. However, the atomic visualization of its nontrivial surface states and MZM remains elusive. Here, we report the direct observation of unconventional surface states and vortex zero mode at the gold (Au) terminated surfaces of AuSn$_{4}$, by ultra-low scanning tunneling microscope/spectroscopy. Distinct from the trivial metallic bulk states at tin (Sn) surfaces, the Au terminated surface exhibits pronounced surface states near Fermi level. Our density functional theory calculations indicate that these states arise from unconventional Rashba bands, where two Fermi circles from different bands share identical helical spin textures, chiralities, and group velocities in the same direction. Furthermore, we find that although the superconducting gap, critical temperature, anisotropic in-plane critical field are almost identical on Au and Sn terminated surfaces, the in-gap bound states inside Abrikosov vortex cores show significant differences. The vortex on Sn terminated surfaces exhibits a conventional Caroli-de Gennes-Matricon bound state while the Au surface shows a sharp zero-energy core state with a long non-splitting distance, resembling an MZM in a non-quantum-limit condition. This distinction may result from the dominant contribution of unconventional Rashba bands near Fermi energy from Au terminated surface. Our results provide a new platform for studying unconventional Rashba band and MZM in superconductors.

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