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arXiv 2405.09136physics.flu-dyncond-mat.soft
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剪切稀化流体中椭球形颗粒的自扩散泳推进

Self-diffusiophoretic propulsion of a spheroidal particle in a shear-thinning fluid

Guangpu Zhu, Brandon van Gogh, Lailai Zhu, On Shun Pak, Yi Man

AI总结:

本文通过渐近分析与数值模拟发现,剪切稀化流变学可增强椭球形颗粒的自扩散泳推进,这与球形颗粒减速的结论相反,并揭示了互补涂层颗粒对的推进速度新特征。

摘要:

剪切稀化粘度是一种非牛顿行为,活性颗粒在血液和粘液等生物流体中经常遇到。这种普遍存在的非牛顿流变学如何影响活性颗粒的推进这一基本问题引起了广泛关注。特别是,由自扩散泳驱动的球形 Janus 颗粒(合成活性颗粒的主要物理化学推进机制)被证明在剪切稀化流体中总是比在牛顿流体中游得更慢。在这项工作中,我们超越了球形极限,研究了颗粒偏心率对剪切稀化流体中自扩散泳推进的影响。我们结合渐近分析和数值模拟表明,剪切稀化流变学可以增强椭球形颗粒的自扩散泳推进,这与先前关于球形情况的结果形成鲜明对比。对推进速度依赖于颗粒活性表面覆盖率的系统表征,也揭示了一对互补涂层颗粒的推进速度所具有的一个有趣特征,这是以前未曾报道过的。我们提出了对称性论证,以阐明这一新特征如何作为椭球几何各向异性和流体流变学非线性的综合效应而出现。

英文摘要:

Shear-thinning viscosity is a non-Newtonian behaviour that active particles often encounter in biological fluids such as blood and mucus. The fundamental question of how this ubiquitous non-Newtonian rheology affects the propulsion of active particles has attracted substantial interest. In particular, spherical Janus particles driven by self-diffusiophresis, a major physico-chemical propulsion mechanism of synthetic active particles, were shown to always swim slower in a shear-thinning fluid than in a Newtonian fluid. In this work, we move beyond the spherical limit to examine the effect of particle eccentricity on self-diffusiophoretic propulsion in a shear-thinning fluid. We use a combination of asymptotic analysis and numerical simulations to show that shear-thinning rheology can enhance self-diffusiophoretic propulsion of a spheroidal particle, in stark contrast to previous findings for the spherical case. A systematic characterization of the dependence of the propulsion speed on the particle's active surface coverage has also uncovered an intriguing feature associated with the propulsion speeds of a pair of complementarily coated particles not previously reported. Symmetry arguments are presented to elucidate how this new feature emerges as a combined effect of anisotropy of the spheroidal geometry and nonlinearity in fluid rheology.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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