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arXiv 2404.14697cond-mat.mes-hallcond-mat.mtrl-scicond-mat.str-el
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共振X射线磁散射揭示手性立方磁体Co$_8$Zn$_8$Mn$_4$中的竞争各向异性

Competing anisotropies in the chiral cubic magnet Co$_8$Zn$_8$Mn$_4$ unveiled by resonant x-ray magnetic scattering

Victor Ukleev, Oleg I. Utesov, Chen Luo, Florin Radu, Sebastian Wintz, Markus Weigand, Simone Finizio, Moritz Winter, Alexander Tahn, Bernd Rellinghaus, Kosuke … 展开作者

Victor Ukleev, Oleg I. Utesov, Chen Luo, Florin Radu, Sebastian Wintz, Markus Weigand, Simone Finizio, Moritz Winter, Alexander Tahn, Bernd Rellinghaus, Kosuke Karube, Yoshinori Tokura, Yasujiro Taguchi, Jonathan S. White

AI总结:

本研究利用矢量磁场下的X射线共振磁小角散射,揭示了手性立方磁体Co$_8$Zn$_8$Mn$_4$中磁晶各向异性与交换各向异性的竞争机制,定量阐明了各向异性交换相互作用随温度的变化及其对螺旋螺距的影响。

摘要:

立方$β$-Mn型合金Co$_8$Zn$_8$Mn$_4$是一种手性螺旋磁体,其螺旋螺距表现出奇特的温度依赖行为,从室温下的130 nm减小到20 K以下的70 nm。值得注意的是,这种缩短还伴随着亚稳态skyrmion织构的结构转变,从六角晶格转变为拉长skyrmion的四方晶格。这些转变的潜在机制仍然未知,可能涉及的相互作用包括温度依赖的Dzyaloshinskii-Moriya相互作用、磁晶各向异性和交换各向异性。在此,我们采用矢量磁场下的X射线共振磁小角散射来研究Co$_8$Zn$_8$Mn$_4$中螺旋相各向异性性质的温度依赖性。我们的结果定量地揭示,各向异性交换相互作用的强度在从室温冷却到20 K时增加了4倍,导致20 K时(001)面内螺旋螺距发生5%的变化。尽管各向异性交换相互作用促成了螺旋螺距的缩短,但其强度不足以解释从室温到低温螺旋周期的变化。最后,我们证明了磁晶各向异性和交换各向异性相互竞争,在基态中偏好不同的螺旋矢量取向。

英文摘要:

The cubic $β$-Mn-type alloy Co$_8$Zn$_8$Mn$_4$ is a chiral helimagnet that exhibits a peculiar temperature-dependent behavior in the spiral pitch, which decreases from 130 nm at room temperature to 70 nm below 20 K. Notably, this shortening is also accompanied by a structural transition of the metastable skyrmion texture, transforming from a hexagonal lattice to a square lattice of elongated skyrmions. The underlying mechanism of these transformations remain unknown, with interactions potentially involved including temperature-dependent Dzyaloshinskii-Moriya interaction, magnetocrystalline anisotropy, and exchange anisotropy. Here, x-ray resonant magnetic small-angle scattering in vectorial magnetic fields was employed to investigate the temperature dependence of the anisotropic properties of the helical phase in Co$_8$Zn$_8$Mn$_4$. Our results reveal quantitatively that the magnitude of the anisotropic exchange interaction increases by a factor of 4 on cooling from room temperature to 20 K, leading to a 5% variation in the helical pitch within the (001) plane at 20 K. While anisotropic exchange interaction contributes to the shortening of the spiral pitch, its magnitude is insufficient to explain the variation in the spiral periodicity from room to low temperatures. Finally, we demonstrate that magnetocrystalline and exchange anisotropies compete, favoring different orientations of the helical vector in the ground state.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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