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arXiv 2403.04515cond-mat.mes-hallphysics.app-ph
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光诱导KTaO3基界面非互易输运的巨增强

Light-induced giant enhancement of nonreciprocal transport at KTaO3-based interfaces

Xu Zhang, Tongshuai Zhu, Shuai Zhang, Zhongqiang Chen, Anke Song, Chong Zhang, Rongzheng Gao, Wei Niu, Yequan Chen, Fucong Fei, Yilin Tai, Guoan Li, Binghui Ge,… 展开作者

Xu Zhang, Tongshuai Zhu, Shuai Zhang, Zhongqiang Chen, Anke Song, Chong Zhang, Rongzheng Gao, Wei Niu, Yequan Chen, Fucong Fei, Yilin Tai, Guoan Li, Binghui Ge, Wenkai Lou, Jie Shen, Haijun Zhang, Kai Chang, Fengqi Song, Rong Zhang, Xuefeng Wang

AI总结:

本研究在CaZrO3/KTaO3(111)超导界面观测到光诱导的非互易输运巨增强,系数提升三个数量级,揭示了紫外光生高迁移率载流子诱导强Rashba自旋轨道耦合的机制,为光整流与自旋轨道器件研发提供了新路径。

摘要:

非线性输运是非中心对称系统的独特功能,反映了自旋轨道相互作用、超导性和能带几何等深刻物理机制。然而,增强非互易输运以开发有前景的整流器件仍极具挑战性。本研究在超导外延CaZrO3/KTaO3 (111)界面上观测到光诱导的非互易输运巨增强现象:非互易输运系数出现三个数量级的大幅提升,最高可达10⁵ A⁻¹T⁻¹。此外,在紫外光照射下,体系产生大量高迁移率光载流子,实现了14.7 T的强Rashba自旋轨道耦合有效场,这是非互易输运系数巨增强的原因。第一性原理计算进一步揭示了光载流子激发过程中更强的Rashba自旋轨道耦合强度和更长的弛豫时间,建立了光与物性之间的定量关系。本研究为提升非中心对称系统的非互易输运性能提供了新途径,并推动了其在光整流器件和自旋轨道电子器件中的潜在应用。

英文摘要:

Nonlinear transport is a unique functionality of noncentrosymmetric systems, which reflects profound physics, such as spin-orbit interaction, superconductivity and band geometry. However, it remains highly challenging to enhance the nonreciprocal transport for promising rectification devices. Here, we observe a light-induced giant enhancement of nonreciprocal transport at the superconducting and epitaxial CaZrO3/KTaO3 (111) interfaces. The nonreciprocal transport coefficient undergoes a giant increase with three orders of magnitude up to 105 A-1T-1. Furthermore, a strong Rashba spin-orbit coupling effective field of 14.7 T is achieved with abundant high-mobility photocarriers under ultraviolet illumination, which accounts for the giant enhancement of nonreciprocal transport coefficient. Our first-principles calculations further disclose the stronger Rashba spin-orbit coupling strength and the longer relaxation time in the photocarrier excitation process, bridging the light-property quantitative relationship. Our work provides an alternative pathway to boost nonreciprocal transport in noncentrosymmetric systems and facilitates the promising applications in opto-rectification devices and spin-orbitronic devices.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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